D. Comtois

Laser-Induced Electron Tunneling and Diffraction

Molecular structure is usually determined by measuring the diffraction pattern the molecule impresses on x-rays or electrons. We used a laser field to extract electrons from the molecule itself, accelerate them, and in some cases force them to recollide with and diffract from the parent ion, all within a fraction of a laser period. Here, we show that the momentum distribution of the extracted electron carries the fingerprint of the highest occupied molecular orbital, whereas the elastically scattered electrons reveal the position of the nuclear components of the molecule. Thus, in one comprehensive technology, the photoelectrons give detailed information about the electronic orbital and the position of the nuclei.

Filamentation of ultrashort pulse laser beams resulting from their propagation over long distances in air

The propagation of high-power short-pulse laser beams over considerable distances in air is studied both experimentally and via numerical simulations. Filaments are formed after 5–10 m and their propagation over distances in excess of 200 m is reported for the first time. The lateral dimensions of the filaments are found to range from about 100 μm to a few millimeters in diameter. The early values of plasma electron density have been inferred to be a few times 1016 cm−3 using longitudinal spectral interferometry. For 500 fs pulses and a wavelength of 1053 nm, the energy in the filament can be quite high initially (∼8 mJ) and is found to stabilize at about 1.5–2 mJ, after about 35 m. A simple model based on the nonlinear Schrodinger equation coupled to a multiphoton ionization law appears to describe several experimental results quite well.

Triggering and guiding high-voltage large-scale leader discharges with sub-joule ultrashort laser pulses*

The triggering and guiding of leader discharges using a plasma channel created by a sub-joule ultrashort laser pulse have been studied in a megavolt large-scale electrode configuration (3–7 m rod-plane air gap). By focusing the laser close to the positive rod electrode it has been possible, with a 400 mJ pulse, to trigger and guide leaders over distances of 3 m, to lower the leader inception voltage by 50%, and to increase the leader velocity by a factor of 10. The dynamics of the breakdown discharges with and without the laser pulse have been analyzed by means of a streak camera and of electric field and current probes. Numerical simulations have successfully reproduced many of the experimental results obtained with and without the presence of the laser plasma channel.

Modeling the triggering of streamers in air by ultrashort laser pulses

The physical processes involved in the triggering of ionization waves (streamers) by ultrashort laser pulses, focused in air at 350 Torr and in a uniform electric field, are investigated by means of a one-dimensional (1-D) numerical model. The model describes the interaction of the laser pulse with air and takes into account many of the reactions in the laser-created plasma as well as the radial expansion of the plasma. Consequences of the model are that the threshold electric field for the appearance of streamers is an increasing function of the delay between the laser pulse and the electric field pulse and a decreasing function of the laser energy. Also, it appears that the electron temperature, the plasma density and radius, and the conduction of heat across the plasma boundaries play major roles in the capacity of the laser-created plasma to trigger streamers. The results of the model are compared with the available experimental data.

Guiding large-scale spark discharges with ultrashort pulse laser filaments

Using the nonlinear propagation properties of ultrashort laser pulses in air, we were able to produce long ionized filaments that served to guide spark discharges. With a laser pulse energy of 20 mJ, one or two ionized filaments were created and could guide streamer discharges over 2 m air gaps, where the electric field was fairly uniform and had an average value of 0.6 MV/m. Such a guiding effect was observed for times of 1–3 μs after the laser pulse created the ionized filaments. Longer delays (10–15 μs) were recorded at higher laser pulse energy, with a larger number of filaments. Images of the early stages of the discharge of a uniform air gap show that the laser-produced ionized filaments do not initiate the discharge process but act rather as preferred channels where the leader growth is accelerated. In the end, these straight conductive channels carry the arc current as the voltage in the gap breaks down.

Triggering and guiding leader discharges using a plasma channel created by an ultrashort laser pulse

In a 2.8 m positive rod–plane air gap, we have studied how a plasma channel produced by focusing a 200 mJ ultrashort laser beam is able to trigger and guide a leader discharge. We have observed that the plasma channel allowed the lowering of the leader inception voltage by 50% and the guiding of the leader propagation on a distance of up to 2.3 m, with a tenfold increase of its speed. This led to an effective 40% reduction of the breakdown voltage. For the conditions studied here, the laser energy per unit length required to guide a leader is between 60 and 100 mJ/m.

The influence of electron density on the formation of streamers in electrical discharges triggered with ultrashort laser pulses

In an ongoing program using ultrashort laser pulses to provoke discharges in air over considerable distances at electric fields below breakdown threshold, we have studied the conditions for the onset of streamers in such laser-produced plasmas, both experimentally and through numerical simulations. The results demonstrate the importance of the electron density and of its gradient on the generation of streamers. Also, a significant reduction of the breakdown voltage for a 30 cm plane-plane gap in air was observed with a laser pulse energy of 15 mJ. Finally, a direct comparison of laser-induced breakdown in air and in nitrogen shows the influence of electron attachment to oxygen on the discharge process.

Triggering and guiding of an upward positive leader from a ground rod with an ultrashort laser pulse. I. Experimental results

Using a plasma channel produced by an ultrashort laser pulse, we have studied the laser triggering and guiding of a positive leader from the tip of a 2-m vertical rod standing on the bottom plane of a 7-m plane-plane gap. The purpose of this setup was to reproduce in the laboratory the electric field conditions leading to the onset of a positive upward leader from a ground rod as a downward negative leader is approaching during a thunderstorm, in order to demonstrate the working principle of a possible future laser lightning rod. The leader triggering properties of the laser-created plasma channel have been studied as a function of the synchronization of the laser pulse with the voltage impulse applied to the gap. We show that the laser pulse reduces the inception voltage of the leader compared to its normal value and that the laser plasma channel guides the propagation of the upward leader at a velocity ten times higher than that of an ordinary leader, with a significantly lower charge per unit length. We show that laser guiding of the leader significantly reduces the breakdown voltage of the gap and that the effect of the laser channel at the end of a lightning rod can be compared quite favorably with the effect of an additional metal rod of the same length.

Spectroscopic study of ultrashort pulse laser-breakdown plasmas in air

Time-resolved visible spectroscopy of plasmas produced by laser breakdown of air using femtosecond Nd laser pulses (50–300 mJ, 500 fs) reveals features not observed with nanosecond laser pulses. Emission is initially dominated by molecular lines, specifically the second positive system of N2 and the first negative system of N2+. This is followed by continuum emission with a growth time of ∼3 ns and a decay time of ∼30 ns. Atomic lines of N and O emerge from the decay of the continuum and last up to 1 μs; only faint ionization lines are observed. Several of the atomic lines are initially strongly broadened, narrowing over a period of 100 ns.

Triggering and guiding of an upward positive leader from a ground rod with an ultrashort laser pulse. II. Modeling

We have used the Bondio-Gallimberti model of positive leader propagation to simulate laboratory experiments of laser triggering and guiding of upward leaders initiated from a ground rod. The model proves to be capable of reproducing all the important features of laser-guided leader propagation that have been observed experimentally. The leader guiding effect of the laser-created plasma channel is taken into account in the model by adjusting the value of the charge per unit length of the leader, which has been measured in the laboratory to be lower for a laser-guided leader than for an ordinary one. The charge per unit length of the leader is related in the model to the critical temperature at which the air in the transition region at the leader tip must be heated to be conductive enough to become a new leader portion. For an ordinary leader, this critical temperature is 1500 K, at which the electrons all detach from the negative ions in the leader corona, increasing the air conductivity. We give the interpretation that in the case of the laser-guided leaders, because of the relatively high density of negative ions per unit length in the laser-ionized channel, the right conditions of conductivity can be met in the transition region without the electrons being all detached from the ions, allowing a reduction of the critical temperature and of the charge per unit length.