D. Ursescu

Optimization toward a high-average-brightness soft-x-ray laser pumped at grazing incidence

We report the near-field imaging characterization of a 10 Hz Ni-like 18.9 nm molybdenum soft-x-ray laser pumped in a grazing incidence pumping (GRIP) geometry with a table-top laser driver. We investigate the effect of varying the GRIP angle on the spatial behavior of the soft-x-ray laser source. After multiparameter optimization, we were able to find conditions to generate routinely a high-repetition-rate soft-x-ray laser with an energy level of up to 3 microJ/pulse and to 6x10(17) photons/s/mm2/mrad2/(0.1% bandwidth) average brightness and 1x10(28) photons/s/mm2/mrad2/(0.1% bandwidth) peak brightness.

Extreme Light Infrastructure: Architecture and major challenges

Extreme Light Infrastructure (ELI), the first research facility hosting an exawatt class laser will be built with a joint international effort and form an integrated infrastructure comprised at last three branches: Attosecond Science (in Szeged, Hungary) designed to make temporal investigation at the attosecond scale of electron dynamics in atoms, molecules, plasmas and solids. High Field Science will be mainly focused on producing ultra intense and ultra short sources of electons, protons and ions, coherent and high energetic X rays (in Prague, Czech Republic) as well as laserbased nuclear physics (in Magurele, Romania). The location of the fourth pillar devoted to Extreme Field Science, which will explore laser-matter interaction up to the non linear QED limit including the investigation of vacuum structure and pair creation, will be decided after 2012. The research activities will be based on an incremental development of the light sources starting from the current high intensity lasers (APOLLON, GEMINI, Vulcan and PFS) as prototypes to achieve unprecedented peak power performance, from tens of petawatt up to a fraction of exawatt (1018 W). This last step will depend on the laser technology development in the above three sites as well as in current high intensity laser facilities.

Optimization of the non-normal incidence, transient pumped plasma X-ray laser for laser spectroscopy and plasma diagnostics at the facility for antiproton and ion research (FAIR)

Intense and stable laser operation with Ni-like Zr and Ag was demonstrated at pump energies between 2 J and 5 J energy from the PHELIX pre-amplifier section. A novel single mirror focusing scheme for the TCE x-ray laser ~XRL! has been successfully implemented by the LIXAM0MBI0GSI collaboration under different pump geometries. This shows potential for an extension to shorter XRL wavelength. Generation of high quality XRL beams for XRL spectroscopy of highly charged ions is an important issue within the scientific program of PHELIX. Long range perspective is the study of nuclear properties of radioactive isotopes within the FAIR project.

Extreme Light Infrastructure – Nuclear Physics

The Extreme Light Infrastructure (ELI) is an ESFRI-listed distributed facility that entered the implementation phase. The Romanian pillar will focus on the field of nuclear physics research, performed with the help of an ultra-short-pulse, multi-petawatt scale laser system and a brilliant, tuneable and highly collimated gamma beam system. ELI-Nuclear Physics, an open-access facility, shall become operational and receive the first visiting research teams in 2017. We report herein on the status of the implementation and some of the research topics proposed for ELI-NP.

An improved double-pulse non-normal incidence pumping geometry for transient collisionally excited soft X-ray lasers

An optimized pumping geometry for transient collisionally excited soft X-ray lasers is presented, similar to the geometry proposed by [1]. In contrast to usual approaches, where a nanosecond pre-pulse is assumed to provide the optimal plasma preparation and a picosecond pulse performs the final heating- and excitation process, two pulses of equal duration in the range around 10 picoseconds are applied. Both pulses are produced in the front end of the CPA pump laser. They are focused onto the target with the same spherical mirror under non-normal incidence geometry, optimized for efficient traveling wave excitation for the main-pulse. A first experiment was performed on Ni-like palladium (14.7 nm) at less than 500mJ total pulse energy on the target. This proves that this configuration is at least as favorable as the standard GRIP scheme, providing much simpler and more reliable operation.

Spectroscopic study of gold nanoparticle formation through high intensity laser irradiation of solution

A spectroscopic study of the gold nanoparticle (NP) formation by high-intensity femtosecond laser irradiation of a gold ion solution was reported. The effect of varying energy density of the laser on the formation of gold NPs was also investigated. The surface plasmon resonance (SPR) peak of the gold nanocolloid in real-time UV-visible absorption spectra during laser irradiation showed a distinctive progress; the SPR absorption peak intensity increased after a certain irradiation time, reached a maximum and then gradually decreased. During this absorption variation, at the same time, the peak wavelength changed from 530 to 507 nm. According to an empirical equation derived from a large volume of experimental data, the estimated mean size of the gold NPs varied from 43.4 to 3.2 nm during the laser irradiation. The mean size of gold NPs formed at specific irradiation times by transmission electron microscopy showed the similar trend as that obtained in the spectroscopic analysis. From these observations, th...

Pump energy reduction for a high gain Ag X-ray laser using one long and two short pump pulses

A pump scheme with one long and two short pump pulses is proposed, in a grazing incidence pumping x-ray laser (XRL) configuration. A 360 ps long pulse, prepares a plasma in a low charge state. Then, an initial short pulse ionizes the plasma to an optimal charge state, while the second short pulse induces strong collisional excitation in the gain region. With only 200 mJ of pump energy on target, a compact Ag XRL at 13.9 nm with a gain coefficient of 55u2009u2009cm(-1) was achieved.

Thin film beam splitter multiple short pulse generation for enhanced Ni-like Ag x-ray laser emission

An alternative, novel multiple pulse generation scheme was implemented directly after the optical compressor output of an x-ray pump laser. The new method uses a polarization sensitive thin film beam splitter and a half-wavelength wave plate for tuning the energy ratio in the multiple short pulses. Based on this method, an extensive study was made of the running parameters for a grazing incidence pumped silver x-ray laser (XRL) pumped with a long pulse of 145xa0mJ in 6xa0ns at 532xa0nm and up to 1.45xa0J in few picoseconds at 810xa0nm. Fivefold enhancement in the emission of the silver XRL was demonstrated using the new pump method.

Spectral combination of ultrashort laser pulses

An ultrashort and ultraintense pulses combination method is proposed, based on the spectral combination of parallel laser pulses, with complementary spectra, in chirped pulse amplification (CPA) laser systems. In a proof-of-principle experiment, it is demonstrated that two long pulses of 330u2009fs can be overlapped in a collinear way, to produce a shorter pulse, of 190u2009fs. As a consequence, it is shown that the power for the combined pulse obtained is up to a factor of 1.7 larger than the sum of the peak powers of each individual pulse. The spectral phase of the combined pulse was characterized with λ/10 accuracy, using spectral interferometry. A way to implement the method at parallel CPA laser facilities, using no transmission optics, is indicated.

Quantitative study of 10 Hz operation of a soft x-ray laser-energy stability and target considerations

A soft x-ray laser from Ni-like Mo, pumped in grazing incidence (GRIP), is analyzed with regard to high repetition rate operation. Reliable lasing is obtained, but with significant energy fluctuations attributed mainly to beam pointing jitter from the pump laser. Two modes of operation are compared: continuously moving target and stationary target. With a moving target the soft X-ray output is constant on average, whereas the repeated use of the same target position leads to a pulse energy which increases for several tens of shots. This effect might be caused by improved guiding of the pump laser in the formed groove and the removal, through laser ablation, of the oxide layer on the target surface.