Dirk Bouwmeester

Self-tuned quantum dot gain in photonic crystal lasers

We demonstrate that very few (2-4) quantum dots as a gain medium are sufficient to realize a photonic-crystal laser based on a high-quality nanocavity. Photon correlation measurements show a transition from a thermal to a coherent light state proving that lasing action occurs at ultralow thresholds. Observation of lasing is unexpected since the cavity mode is in general not resonant with the discrete quantum dot states and emission at those frequencies is suppressed. In this situation, the quasicontinuous quantum dot states become crucial since they provide an energy-transfer channel into the lasing mode, effectively leading to a self-tuned resonance for the gain medium.

Sub-kelvin optical cooling of a micromechanical resonator

Micromechanical resonators, when cooled down to near their ground state, can be used to explore quantum effects such as superposition and entanglement at a macroscopic scale. Previously, it has been proposed to use electronic feedback to cool a high frequency (10 MHz) resonator to near its ground state. In other work, a low frequency resonator was cooled from room temperature to 18 K by passive optical feedback. Additionally, active optical feedback of atomic force microscope cantilevers has been used to modify their response characteristics, and cooling to approximately 2 K has been measured. Here we demonstrate active optical feedback cooling to 135 ± 15 mK of a micromechanical resonator integrated with a high-quality optical resonator. Additionally, we show that the scheme should be applicable at cryogenic base temperatures, allowing cooling to near the ground state that is required for quantum experiments—near 100 nK for a kHz oscillator.

CNOT and Bell-state analysis in the weak-coupling cavity QED regime

We propose an interface between the spin of a photon and the spin of an electron confined in a quantum dot embedded in a microcavity operating in the weak-coupling regime. This interface, based on spin selective photon reflection from the cavity, can be used to construct a CNOT gate, a multiphoton entangler and a photonic Bell-state analyzer. Finally, we analyze experimental feasibility, concluding that the schemes can be implemented with current technology.

Evidence for Rod‐Shaped DNA‐Stabilized Silver Nanocluster Emitters

Fluorescent DNA-stabilized silver nanoclusters contain both cationic and neutral silver atoms. The absorbance spectra of compositionally pure solutions follow the trend expected for rod-shaped silver clusters, consistent with the polarized emission measured from individual nanoclusters. The data suggest a rod-like assembly of silver atoms, with silver cations mediating attachment to the bases.

Dynamic modulation of photonic crystal nanocavities using gigahertz acoustic phonons

The authors demonstrate dynamic tuning of a photonic-crystal cavity by surface acoustic waves at frequencies exceeding 1.7 GHz. The tuning is claimed to preserve the quality factor and to be an order of magnitude faster than alternative approaches.

Deterministic nanoassembly of a coupled quantum emitter–photonic crystal cavity system

Controlling the interaction of a single quantum emitter with its environment is a key challenge in quantum optics. Here, we demonstrate deterministic coupling of single nitrogen-vacancy (NV) centers to high-quality photonic crystal cavities. We preselect single NV centers and position their 50-nm-sized host nanocrystals into the mode maximum of photonic crystal S1 cavities with few-nanometer accuracy. The coupling results in a strong enhancement of NV center emission at the cavity wavelength.

Strong coupling through optical positioning of a quantum dot in a photonic crystal cavity

crystal cavities have relied largely on random chance 5,6 and often required the measurement of many devices before finding a cavity in which a quantum dot is both spectrally and spatially in resonance with the cavity mode. These devices have the additional complication that the photonic crystal cavity typically interacts with many emitters due to the large quantum dot density required to find a strongly coupled device. A deterministic coupling method based on using atomic force microscopy to locate the strain sites of buried quantum dots has previously been demonstrated. 7,8 Here, we present an all-optical method for measuring the positions of individual quantum dots that allows us to deterministically achieve strong coupling between a quantum dot and a photonic crystal cavity. This versatile method can be performed in the measurement setup at a very low quantum dot density and could be applied to many emitter-cavity systems. Our technique relies on the precise determination of the optical

Quantum entanglement of a large number of photons

A bipartite multiphoton entangled state is created through stimulated parametric down-conversion of strong laser pulses in a nonlinear crystal. It is shown how detectors that do not resolve the photon number can be used to analyze such multiphoton states. Entanglement of up to 12 photons is detected using both the positivity of the partially-transposed density matrix and a newly derived criteria. Furthermore, evidence is provided for entanglement of up to 100 photons. The multiparticle quantum state is such that even in the case of an overall photon collection and detection efficiency as low as a few percent, entanglement remains and can be detected.

Photon statistics from coupled quantum dots

We present an optical study of two closely stacked self-assembled InAs/GaAs quantum dots. The energy spectrum and correlations between photons subsequently emitted from a single pair provide not only clear evidence of coupling between the quantum dots but also insight into the coupling mechanism. Our results are in agreement with recent theories predicting that tunneling is largely suppressed between nonidentical quantum dots and that the interaction is instead dominated by dipole-dipole coupling and phonon-assisted energy transfer processes.

Frequency control of photonic crystal membrane resonators by monolayer deposition

We study the response of GaAs photonic crystal membrane resonators to thin-film deposition. Slow spectral shifts of the cavity mode of several nanometers are observed at low temperatures, caused by cryo-gettering of background molecules. Heating the membrane resets the drift and shielding will prevent drift altogether. In order to explore the drift as a tool to detect surface layers, or to intentionally shift the cavity resonance frequency, we studied the effect of self-assembled monolayers of polypeptide molecules attached to the membranes. The 2-nm-thick monolayers lead to a discrete step in the resonance frequency and partially passivate the surface.