E. F. Talantsev

TEM observation of the microstructure of metal-organic deposited YBa2Cu3O7−δ with Dy additions

The microstructure of metal-organic deposited YBa2Cu3O7−δ with dysprosium (Dy) additions has been investigated by transmission electron microscopy (TEM). Dy additions which increase the density of normal-state nanoparticles in the YBCO have been demonstrated to enhance the critical current densities in moderate magnetic fields. The influence of nanoparticles, stacking faults and other planar defects on flux pinning is discussed. We observed a high density of nanoparticles in the size range of 10–50 nm, which may act as flux pinning centres to enhance the critical current density of the material. Stacking faults and planar defects are observed which may also be effective flux pinning centres in YBCO samples with and without Dy addition.

Universal self-field critical current for thin-film superconductors

For any practical superconductor the magnitude of the critical current density, Jc, is crucially important. It sets the upper limit for current in the conductor. Usually Jc falls rapidly with increasing external magnetic field, but even in zero external field the current flowing in the conductor generates a self-field that limits Jc. Here we show for thin films of thickness less than the London penetration depth, λ, this limiting Jc adopts a universal value for all superconductors—metals, oxides, cuprates, pnictides, borocarbides and heavy Fermions. For type-I superconductors, it is Hc/λ where Hc is the thermodynamic critical field. But surprisingly for type-II superconductors, we find the self-field Jc is Hc1/λ where Hc1 is the lower critical field. Jc is thus fundamentally determined and this provides a simple means to extract absolute values of λ(T) and, from its temperature dependence, the symmetry and magnitude of the superconducting gap.

On the origin of critical temperature enhancement in atomically thin superconductors

Recent experiments showed that thinning gallium, iron selenide and 2H tantalum disulfide to single/several monoatomic layer(s) enhances their superconducting critical temperatures. Here, we characterize these superconductors by extracting the absolute values of the London penetration depth, the superconducting energy gap, and the relative jump in specific heat at the transition temperature from their self-field critical currents. Our central finding is that the enhancement in transition temperature for these materials arises from the opening of an additional superconducting gap, while retaining a largely unchanged bulk superconducting gap. Literature data reveals that ultrathin niobium films similarly develop a second superconducting gap. Based on the available data, it seems that, for type-II superconductors, a new superconducting band appears when the film thickness becomes smaller than the out-of-plane coherence length. The same mechanism may also be the cause of enhanced interface superconductivity.

Flux Pinning by Barium Stannate Nanoparticles in MOD YBCO Coated Conductors

Tin-based nanoparticles, proposed to be barium stannate, have been formed in YBCO films fabricated by metal-organic deposition, through modification of the precursor solution. These randomly-oriented 30-50 nm particles are dispersed throughout the film thickness, providing an enhancement in the isotropic flux pinning relative to undoped YBCO. For a low level of nanoparticle addition of 2 vol%, a flux-pinning force enhancement of up to 32% is achieved. We report field and field-angle dependence of the transport critical current, transmission electron microscopy, and X-ray diffraction of our YBCO films on RABiTS substrates, and compare with similar barium zirconate additions.

The scaling of transport AC losses in Roebel cables with varying strand parameters

A Roebel cable is a good candidate for low-voltage windings in a high-temperature superconductor (HTS) transformer because of its high current-carrying capability and low AC loss. Transport AC loss measurements were carried out in 1.8 m long 15/5 (fifteen 5 mm wide strands) and 15/4 Roebel cables. The results were compared with those in many Roebel cables composed of 2 mm wide Roebel strands. Comparison of the AC losses hinted that the intrinsic difference in normalized transport AC losses is due to differences in the g/w (ratio of the horizontal gap between the Roebel strands over the Roebel strand width) values. The intrinsic difference was confirmed by measuring transport AC loss in a series of horizontally arranged parallel conductor pairs with various g values. A method to scale transport AC losses in Roebel cables with varying strand parameters was developed. The scaling method will be useful for a rough assessment of AC loss in one-layer solenoid winding coils, such as in a HTS transformer.

Universal scaling of the self-field critical current in superconductors: from sub-nanometre to millimetre size

Universal scaling behaviour in superconductors has significantly elucidated fluctuation and phase transition phenomena in these materials. However, universal behaviour for the most practical property, the critical current, was not contemplated because prevailing models invoke nucleation and migration of flux vortices. Such migration depends critically on pinning, and the detailed microstructure naturally differs from one material to another, even within a single material. Through microstructural engineering there have been ongoing improvements in the field-dependent critical current, thus illustrating its non-universal behaviour. But here we demonstrate the universal size scaling of the self-field critical current for any superconductor, of any symmetry, geometry or band multiplicity. Key to our analysis is the huge range of sample dimensions, from single-atomic-layer to mm-scale. These have widely variable microstructure with transition temperatures ranging from 1.2 K to the current record, 203 K. In all cases the critical current is governed by a fundamental surface current density limit given by the relevant critical field divided by the penetration depth.

Relating Critical Currents to Defect Populations in Superconductors

Analyzing critical currents from an information theoretic or statistical point of view allows one to identify distinct populations of microstates contributing to the critical current under particular conditions of temperature and applied field. We show how this knowledge can be correlated with the known microstructure of a sample to identify how different physical populations of pinning centers are contributing to these statistical populations of microstates. We will then show that by tracking the variation of critical current with temperature, field, and field angle we can construct a picture of the relative contributions of different defect populations under different conditions. We particularly focus our analysis on YBCO thin film coated conductors with potential commercial application.

Effective Low-Temperature Flux Pinning by Au Ion Irradiation in HTS Coated Conductors

We report the effects of heavy-ion irradiation on critical currents in (Y,Dy)Ba₂Cu₃O_7-δ coated conductors made by a commercial metal organic deposition process. Irradiation with 185 MeV Au ions is investigated and contrasted with previous results on 74 MeV Ag ions. The change in critical current (I_c) is reported as a function of temperature (30-77 K), magnetic field (0-7 T) and magnetic-field angle (full angle dependence). Significant improvements are seen particularly at 30-40 K where I_c can be enhanced over a wide angular range and the minimum of I_c(θ) has been enhanced by up to 60%. This contrasts with the data for the commonly utilized regime of 77 K, 1 T where the I_c enhancements are small or limited to a narrow angular range. This data also serves to illustrate the need to measure Ic in all of the temperature and field regimes of technical interest and to measure the complete field-angular dependence I_c(θ).

Current distribution across type II superconducting films: a new vortex-free critical state

The current distribution across the thickness of a current-carrying rectangular film in the Meissner state was established long ago by the London brothers. The distribution across the width is more complicated but was later shown to be highly non-uniform, diverging at the edges. Accordingly, the standard view for type II superconductors is that vortices enter at the edges and, with increasing current, are driven inwards until they self-annihilate at the centre, causing dissipation. This condition is presumed to define the critical current. However we have shown that, under self-field (no external field), the transport critical current is a London surface current where the surface current density equals the critical field divided by λ, across the entire width. The critical current distribution must therefore be uniform. Here we report studies of the current and field distribution across commercial YBa2Cu3 O7 conductors and confirm the accepted non-uniform distribution at low current but demonstrate a radical crossover to a uniform distribution at critical current. This crossover ends discontinuously at a singularity and calculations quantitatively confirm these results in detail. The onset of self-field dissipation is, unexpectedly, thermodynamic in character and the implied vortex-free critical state seems to require new physics.

The onset of dissipation in high-temperature superconductors: Self-field experiments

The transport critical current, Ic, is usually defined in terms of a threshold electric field criterion, Ec, with the convention Ec = 1 μV/cm chosen somewhat arbitrarily to provide “reasonably small” electric power dissipation in practical devices. Thus Ic is not fundamentally determined. However, recently it has been shown that the self-field critical current of thin-film superconductors is indeed a fundamental property governed only by the London penetration depth of the material. Here we reconsider the definition of the critical current and resolve this apparent contradiction. We measure the field distribution across the width of both first-generation and second-generation high-temperature superconducting tapes as the transport current is increased from zero to Ic. We identify a threshold current, Ic,surfB, at which the local surface magnetic flux density, Bsurf, abruptly crosses over from a non-linear to a linear dependence on the transport current, as measured at any point on the superconductor surfa...