E. R. Eliel

Production and characterization of spiral phase plates for optical wavelengths

We describe the fabrication and characterization of a high-quality spiral phase plate as a device to generate optical vortices of low (3-5) specified charge at visible wavelengths. The manufacturing process is based on a molding technique and allows for the production of high-precision, smooth spiral phase plates as well as for their replication. An attractive feature of this process is that it permits the fabrication of nominally identical spiral phase plates made from different materials and thus yielding different vortex charges. When such a plate is inserted in the waist of a fundamental Gaussian beam, the resultant far-field intensity profile shows a rich vortex structure, in excellent agreement with diffraction calculations based on ideal spiral phase plates. Using a simple optical test, we show that the reproducibility of the manufacturing process is excellent.

Observation of Goos-Hänchen shifts in metallic reflection

We report the first observation of the Goos-Hänchen shift of a light beam incident on a bare metal surface. This phenomenon is particularly interesting because the Goos-Hänchen shift for p polarized light in metals is negative and much bigger than the positive shift for s polarized light. The experimental result for the measured shifts as a function of the angle of incidence is in excellent agreement with theoretical predictions. In an energy-flux interpretation, our measurement shows the existence of a backward energy flow at the bare metal surface when this is excited by a p polarized beam of light.

Experimental demonstration of fractional orbital angular momentum entanglement of two photons.

The singular nature of a noninteger spiral phase plate allows easy manipulation of spatial degrees of freedom of photon states. Using two such devices, we have observed very high-dimensional spatial entanglement of twin photons generated by spontaneous parametric down-conversion.

Self-dispersive sum-frequency generation at interfaces.

We employ the self-dispersive nature of infrared-visible sum-frequency generation at interfaces to record sumfrequency spectra of molecular monolayers with a spectral resolution of a few inverse centimeters, using IR light with a spectral content of approximately 50 cm(-1).

Full-field quantum correlations of spatially entangled photons.

Spatially entangled twin photons allow the study of high-dimensional entanglement, and the Laguerre-Gauss modes are the most commonly used basis to discretize the single-photon mode spaces. In this basis, to date only the azimuthal degree of freedom has been investigated experimentally due to its fundamental and experimental simplicity. We show that the full spatial entanglement is indeed accessible experimentally; i.e., we have found practicable radial detection modes with negligible cross correlations. This allows us to demonstrate hybrid azimuthal-radial quantum correlations in a Hilbert space with more than 100 dimensions per photon.

Shannon dimensionality of quantum channels and its application to photon entanglement.

We introduce the concept of Shannon dimensionality D as a new way to quantify bipartite entanglement as measured in an experiment. This is applied to orbital-angular-momentum entanglement of two photons, using two state analyzers composed of a rotatable angular-sector phase plate that is lens coupled to a single-mode fiber. We can deduce the value of D directly from the observed two-photon coincidence fringe. In our experiment, D varies between 2 and 6, depending on the experimental conditions. We predict how the Shannon dimensionality evolves when the number of angular sectors imprinted in the phase plate is increased and anticipate that D approximately 50 is experimentally within reach.

Sum-frequency generation from thiophenol on silver in the mid and far-IR

Sum-frequency (SF) spectra of a monolayer of thiophenol on silver are reported in the mid and far-IR (infrared). The free-electron laser FELIX was used to reach wavelengths up to 54 μm. Molecular vibrations of thiophenol are observed at wavelengths near 10 μm (three modes), 14 μm (1 mode), and 24 μm (1 mode). The appearance of the different vibrational modes in the spectra varies dramatically due to interference between the resonant sum-frequency signal and the nonresonant sum-frequency signal from silver. The standard model used to describe line shapes in SF spectra is shown to be insufficient to explain the different line shapes for the various vibrational modes of thiophenol on silver.

Transport of orbital-angular-momentum entanglement through a turbulent atmosphere

We demonstrate experimentally how orbital-angular-momentum entanglement of two photons evolves under the influence of atmospheric turbulence. Experimental results are in excellent agreement with our theoretical model, which combines the formalism of two-photon coincidence detection with a Kolmogorov description of atmospheric turbulence. We express the robustness to turbulence in terms of the dimensionality of the measured correlations. This dimensionality is surprisingly robust: scaling up our system to real-life dimensions, a horizontal propagation distance of 2 km seems viable.

Creating and verifying a quantum superposition in a micro-optomechanical system

Micro-optomechanical systems are central to a number of recent proposals for realizing quantum mechanical effects in relatively massive systems. Here, we focus on a particular class of experiments which aim to demonstrate massive quantum superpositions, although the obtained results should be generalizable to similar experiments. We analyze in detail the effects of finite temperature on the interpretation of the experiment, and obtain a lower bound on the degree of non-classicality of the cantilever. Although it is possible to measure the quantum decoherence time when starting from finite temperature, an unambiguous demonstration of a quantum superposition requires the mechanical resonator to be in or near the ground state. This can be achieved by optical cooling of the fundamental mode, which also provides a method to measure the mean phonon number in that mode. We also calculate the rate of environmentally induced decoherence and estimate the timescale for gravitational collapse mechanisms as proposed by Penrose and Diosi. In view of recent experimental advances, practical considerations for the realization of the described experiment are discussed.

Intrinsic orbital angular momentum of paraxial beams with off-axis imprinted vortices.

We investigate the orbital angular momentum (OAM) of paraxial beams containing off-axis phase dislocations and put forward a simple method to calculate the intrinsic orbital angular momentum of an arbitrary paraxial beam. Using this approach we find that the intrinsic OAM of a fundamental Gaussian beam with a vortex imprinted off axis has a Gaussian dependence on the vortex displacement, implying that the expectation value of the intrinsic OAM of a photon can take on a continuous range of values (i.e., integer and noninteger values in units of h). Finally, we investigate, both numerically and experimentally, the far-field profiles of beams carrying half-integer OAM per photon, these beams having been created by the method of imprinting off-axis vortices.