S. S. R. Oemrawsingh

CNOT and Bell-state analysis in the weak-coupling cavity QED regime

We propose an interface between the spin of a photon and the spin of an electron confined in a quantum dot embedded in a microcavity operating in the weak-coupling regime. This interface, based on spin selective photon reflection from the cavity, can be used to construct a CNOT gate, a multiphoton entangler and a photonic Bell-state analyzer. Finally, we analyze experimental feasibility, concluding that the schemes can be implemented with current technology.

Production and characterization of spiral phase plates for optical wavelengths

We describe the fabrication and characterization of a high-quality spiral phase plate as a device to generate optical vortices of low (3-5) specified charge at visible wavelengths. The manufacturing process is based on a molding technique and allows for the production of high-precision, smooth spiral phase plates as well as for their replication. An attractive feature of this process is that it permits the fabrication of nominally identical spiral phase plates made from different materials and thus yielding different vortex charges. When such a plate is inserted in the waist of a fundamental Gaussian beam, the resultant far-field intensity profile shows a rich vortex structure, in excellent agreement with diffraction calculations based on ideal spiral phase plates. Using a simple optical test, we show that the reproducibility of the manufacturing process is excellent.

Experimental demonstration of fractional orbital angular momentum entanglement of two photons.

The singular nature of a noninteger spiral phase plate allows easy manipulation of spatial degrees of freedom of photon states. Using two such devices, we have observed very high-dimensional spatial entanglement of twin photons generated by spontaneous parametric down-conversion.

Evidence for Rod‐Shaped DNA‐Stabilized Silver Nanocluster Emitters

Fluorescent DNA-stabilized silver nanoclusters contain both cationic and neutral silver atoms. The absorbance spectra of compositionally pure solutions follow the trend expected for rod-shaped silver clusters, consistent with the polarized emission measured from individual nanoclusters. The data suggest a rod-like assembly of silver atoms, with silver cations mediating attachment to the bases.

Shannon dimensionality of quantum channels and its application to photon entanglement.

We introduce the concept of Shannon dimensionality D as a new way to quantify bipartite entanglement as measured in an experiment. This is applied to orbital-angular-momentum entanglement of two photons, using two state analyzers composed of a rotatable angular-sector phase plate that is lens coupled to a single-mode fiber. We can deduce the value of D directly from the observed two-photon coincidence fringe. In our experiment, D varies between 2 and 6, depending on the experimental conditions. We predict how the Shannon dimensionality evolves when the number of angular sectors imprinted in the phase plate is increased and anticipate that D approximately 50 is experimentally within reach.

Intrinsic orbital angular momentum of paraxial beams with off-axis imprinted vortices.

We investigate the orbital angular momentum (OAM) of paraxial beams containing off-axis phase dislocations and put forward a simple method to calculate the intrinsic orbital angular momentum of an arbitrary paraxial beam. Using this approach we find that the intrinsic OAM of a fundamental Gaussian beam with a vortex imprinted off axis has a Gaussian dependence on the vortex displacement, implying that the expectation value of the intrinsic OAM of a photon can take on a continuous range of values (i.e., integer and noninteger values in units of h). Finally, we investigate, both numerically and experimentally, the far-field profiles of beams carrying half-integer OAM per photon, these beams having been created by the method of imprinting off-axis vortices.

Half-integral spiral phase plates for optical wavelengths

We have fabricated high-quality, half-integral spiral phase plates for generating optical vortices at visible and near-infrared wavelengths. When inserted in the waist of a fundamental Gaussian beam, such a device gives rise to a rich vortex structure in the far field. The near-perfect cancellation of the effect induced by two nominally identical phase plates shows that we have excellent control of the manufacturing process.

Dual-color nanoscale assemblies of structurally stable, few-atom silver clusters, as reported by fluorescence resonance energy transfer.

We develop approaches to hold fluorescent silver clusters composed of only 10-20 atoms in nanoscale proximity, while retaining the individual structure of each cluster. This is accomplished using DNA clamp assemblies that incorporate a 10 atom silver cluster and a 15 or 16 atom silver cluster. Thermally modulated fluorescence resonance energy transfer (FRET) verifies assembly formation. Comparison to Förster theory, using measured spectral overlaps, indicates that the DNA clamps hold clusters within roughly 5 to 6 nm separations, in the range of the finest resolutions achievable on DNA scaffolds. The absence of spectral shifts in dual-cluster FRET pairs, relative to the individual clusters, shows that select few-atom silver clusters of different sizes are sufficiently stable to retain structural integrity within a single nanoscale DNA construct. The spectral stability of the cluster persists in a FRET pair with an organic dye molecule, in contrast to the blue-shifted emission of the dye.

Diffraction-limited high-finesse optical cavities

High-quality optical cavities with wavelength-sized end mirrors are important to the growing field of micro-optomechanical systems. We present a versatile method for calculating the modes of diffraction limited optical cavities and show that it can be used to determine the effect of a wide variety of cavity geometries and imperfections. Additionally, we show these calculations agree remarkably well with FDTD simulations for wavelength-sized optical modes, even though our method is based on the paraxial approximation.

Fiber-connectorized micropillar cavities

We present a cryogenically compatible method for permanently connecting and coupling a single mode fiber to a single mode of a micropillar cavity with embedded quantum dots (QDs). Efficient coupling of up to 40% was measured which requires a 300 nm positioning accuracy that remains preserved during the fiber attachment procedure and during cool-down to 4 K. Fiber coupling, as opposed to conventional free space coupling, makes it possible to connect many such QD-cavity systems within the same cryostat which can interact through an external optical network, facilitating the implementation of hybrid photon/confined-electron schemes for quantum communication and information processing.