Eiji Saitoh

Observation of the spin Seebeck effect

The generation of electric voltage by placing a conductor in a temperature gradient is called the Seebeck effect. Its efficiency is represented by the Seebeck coefficient, S, which is defined as the ratio of the generated electric voltage to the temperature difference, and is determined by the scattering rate and the density of the conduction electrons. The effect can be exploited, for example, in thermal electric-power generators and for temperature sensing, by connecting two conductors with different Seebeck coefficients, a device called a thermocouple. Here we report the observation of the thermal generation of driving power, or voltage, for electron spin: the spin Seebeck effect. Using a recently developed spin-detection technique that involves the spin Hall effect, we measure the spin voltage generated from a temperature gradient in a metallic magnet. This thermally induced spin voltage persists even at distances far from the sample ends, and spins can be extracted from every position on the magnet simply by attaching a metal. The spin Seebeck effect observed here is directly applicable to the production of spin-voltage generators, which are crucial for driving spintronic devices. The spin Seebeck effect allows us to pass a pure spin current, a flow of electron spins without electric currents, over a long distance. These innovative capabilities will invigorate spintronics research.

Conversion of spin current into charge current at room temperature: Inverse spin-Hall effect

The inverse process of the spin-Hall effect (ISHE), conversion of a spin current into an electric current, was observed at room temperature. A pure spin current was injected into a Pt thin film using spin pumping, and it was observed to generate electromotive force transverse to the spin current. By changing the spin-current polarization direction, the magnitude of this electromotive force varies critically, consistent with the prediction of ISHE.

Transmission of electrical signals by spin-wave interconversion in a magnetic insulator

The energy bandgap of an insulator is large enough to prevent electron excitation and electrical conduction. But in addition to charge, an electron also has spin, and the collective motion of spin can propagate—and so transfer a signal—in some insulators. This motion is called a spin wave and is usually excited using magnetic fields. Here we show that a spin wave in an insulator can be generated and detected using spin-Hall effects, which enable the direct conversion of an electric signal into a spin wave, and its subsequent transmission through (and recovery from) an insulator over macroscopic distances. First, we show evidence for the transfer of spin angular momentum between an insulator magnet Y3Fe5O12 and a platinum film. This transfer allows direct conversion of an electric current in the platinum film to a spin wave in the Y3Fe5O12 via spin-Hall effects. Second, making use of the transfer in a Pt/Y3Fe5O12/Pt system, we demonstrate that an electric current in one metal film induces voltage in the other, far distant, metal film. Specifically, the applied electric current is converted into spin angular momentum owing to the spin-Hall effect in the first platinum film; the angular momentum is then carried by a spin wave in the insulating Y3Fe5O12 layer; at the distant platinum film, the spin angular momentum of the spin wave is converted back to an electric voltage. This effect can be switched on and off using a magnetic field. Weak spin damping in Y3Fe5O12 is responsible for its transparency for the transmission of spin angular momentum. This hybrid electrical transmission method potentially offers a means of innovative signal delivery in electrical circuits and devices.

Spin Seebeck insulator

Thermoelectric generation is an essential function in future energy-saving technologies. However, it has so far been an exclusive feature of electric conductors, a situation which limits its application; conduction electrons are often problematic in the thermal design of devices. Here we report electric voltage generation from heat flowing in an insulator. We reveal that, despite the absence of conduction electrons, the magnetic insulator LaY(2)Fe(5)O(12) can convert a heat flow into a spin voltage. Attached Pt films can then transform this spin voltage into an electric voltage as a result of the inverse spin Hall effect. The experimental results require us to introduce a thermally activated interface spin exchange between LaY(2)Fe(5)O(12) and Pt. Our findings extend the range of potential materials for thermoelectric applications and provide a crucial piece of information for understanding the physics of the spin Seebeck effect.

Current-induced resonance and mass determination of a single magnetic domain wall.

A magnetic domain wall (DW) is a spatially localized change of magnetization configuration in a magnet. This topological object has been predicted to behave at low energy as a composite particle with finite mass. This particle will couple directly with electric currents as well as magnetic fields, and its manipulation using electric currents is of particular interest with regard to the development of high-density magnetic memories. The DW mass sets the ultimate operation speed of these devices, but has yet to be determined experimentally. Here we report the direct observation of the dynamics of a single DW in a ferromagnetic nanowire, which demonstrates that such a topological particle has a very small but finite mass of 6.6 × 10-23 kg. This measurement was realized by preparing a tunable DW potential in the nanowire, and detecting the resonance motion of the DW induced by an oscillating current. The resonance also allows low-current operation, which is crucial in device applications; a DW displacement of 10 µm was induced by a current density of 1010 A m-2.

Observation of longitudinal spin-Seebeck effect in magnetic insulators

We propose a longitudinal spin-Seebeck effect (SSE), in which a magnon-induced spin current is injected parallel to a temperature gradient from a ferromagnet into an attached paramagnetic metal. The longitudinal SSE is measured in a simple and versatile system composed of a ferrimagnetic insulator Y3Fe5O12 slab and a Pt film by means of the inverse spin-Hall effect. The experimental results highlight the intriguing character of the longitudinal SSE due to its own geometric configuration.

Theory of the spin Seebeck effect

The spin Seebeck effect refers to the generation of a spin voltage caused by a temperature gradient in a ferromagnet, which enables the thermal injection of spin currents from the ferromagnet into an attached nonmagnetic metal over a macroscopic scale of several millimeters. The inverse spin Hall effect converts the injected spin current into a transverse charge voltage, thereby producing electromotive force as in the conventional charge Seebeck device. Recent theoretical and experimental efforts have shown that the magnon and phonon degrees of freedom play crucial roles in the spin Seebeck effect. In this paper, we present the theoretical basis for understanding the spin Seebeck effect and briefly discuss other thermal spin effects.

Theory of magnon-driven spin Seebeck effect

The spin Seebeck effect is a spin-motive force generated by a temperature gradient in a ferromagnet that can be detected via normal metal contacts through the inverse spin Hall effect [K. Uchida et al., Nature (London) 455, 778 (2008)]. We explain this effect by spin pumping at the contact that is proportional to the spin-mixing conductance of the interface, the inverse of a temperature-dependent magnetic coherence volume, and the difference between the magnon temperature in the ferromagnet and the electron temperature in the normal metal [D. J. Sanders and D. Walton, Phys. Rev. B 15, 1489 (1977)].

Theory of spin Hall magnetoresistance

We present a theory of the spin Hall magnetoresistance (SMR) in multilayers made from an insulating ferromagnet F, such as yttrium iron garnet (YIG), and a normal metal N with spin-orbit interactions, such as platinum (Pt). The SMR is induced by the simultaneous action of spin Hall and inverse spin Hall effects and therefore a nonequilibrium proximity phenomenon. We compute the SMR in F|N and F|N|F layered systems, treating N by spin-diffusion theory with quantum mechanical boundary conditions at the interfaces in terms of the spin-mixing conductance. Our results explain the experimentally observed spin Hall magnetoresistance in N|F bilayers. For F|N|F spin valves we predict an enhanced SMR amplitude when magnetizations are collinear. The SMR and the spin-transfer torques in these trilayers can be controlled by the magnetic configuration.

Inverse spin-Hall effect induced by spin pumping in metallic system

The inverse spin-Hall effect (ISHE) induced by the spin pumping has been investigated systematically in simple ferromagnetic/paramagnetic bilayer systems. The spin pumping driven by ferromagnetic resonance injects a spin current into the paramagnetic layer, which gives rise to an electromotive force transverse to the spin current using the ISHE in the paramagnetic layer. In a Ni81Fe19/Pt film, we found an electromotive force perpendicular to the applied magnetic field at the ferromagnetic resonance condition. The spectral shape of the electromotive force is well reproduced using a simple Lorentz function, indicating that the electromotive force is due to the ISHE induced by the spin pumping; extrinsic magnetogalvanic effects are eliminated in this measurement. The electromotive force varies systematically by changing the microwave power, magnetic-field angle, and film size, being consistent with the prediction based on the Landau–Lifshitz–Gilbert equation combined with the models of the ISHE and spin pump...