Ken-ichi Uchida

Observation of the spin Seebeck effect

The generation of electric voltage by placing a conductor in a temperature gradient is called the Seebeck effect. Its efficiency is represented by the Seebeck coefficient, S, which is defined as the ratio of the generated electric voltage to the temperature difference, and is determined by the scattering rate and the density of the conduction electrons. The effect can be exploited, for example, in thermal electric-power generators and for temperature sensing, by connecting two conductors with different Seebeck coefficients, a device called a thermocouple. Here we report the observation of the thermal generation of driving power, or voltage, for electron spin: the spin Seebeck effect. Using a recently developed spin-detection technique that involves the spin Hall effect, we measure the spin voltage generated from a temperature gradient in a metallic magnet. This thermally induced spin voltage persists even at distances far from the sample ends, and spins can be extracted from every position on the magnet simply by attaching a metal. The spin Seebeck effect observed here is directly applicable to the production of spin-voltage generators, which are crucial for driving spintronic devices. The spin Seebeck effect allows us to pass a pure spin current, a flow of electron spins without electric currents, over a long distance. These innovative capabilities will invigorate spintronics research.

Transmission of electrical signals by spin-wave interconversion in a magnetic insulator

The energy bandgap of an insulator is large enough to prevent electron excitation and electrical conduction. But in addition to charge, an electron also has spin, and the collective motion of spin can propagate—and so transfer a signal—in some insulators. This motion is called a spin wave and is usually excited using magnetic fields. Here we show that a spin wave in an insulator can be generated and detected using spin-Hall effects, which enable the direct conversion of an electric signal into a spin wave, and its subsequent transmission through (and recovery from) an insulator over macroscopic distances. First, we show evidence for the transfer of spin angular momentum between an insulator magnet Y3Fe5O12 and a platinum film. This transfer allows direct conversion of an electric current in the platinum film to a spin wave in the Y3Fe5O12 via spin-Hall effects. Second, making use of the transfer in a Pt/Y3Fe5O12/Pt system, we demonstrate that an electric current in one metal film induces voltage in the other, far distant, metal film. Specifically, the applied electric current is converted into spin angular momentum owing to the spin-Hall effect in the first platinum film; the angular momentum is then carried by a spin wave in the insulating Y3Fe5O12 layer; at the distant platinum film, the spin angular momentum of the spin wave is converted back to an electric voltage. This effect can be switched on and off using a magnetic field. Weak spin damping in Y3Fe5O12 is responsible for its transparency for the transmission of spin angular momentum. This hybrid electrical transmission method potentially offers a means of innovative signal delivery in electrical circuits and devices.

Spin Seebeck insulator

Thermoelectric generation is an essential function in future energy-saving technologies. However, it has so far been an exclusive feature of electric conductors, a situation which limits its application; conduction electrons are often problematic in the thermal design of devices. Here we report electric voltage generation from heat flowing in an insulator. We reveal that, despite the absence of conduction electrons, the magnetic insulator LaY(2)Fe(5)O(12) can convert a heat flow into a spin voltage. Attached Pt films can then transform this spin voltage into an electric voltage as a result of the inverse spin Hall effect. The experimental results require us to introduce a thermally activated interface spin exchange between LaY(2)Fe(5)O(12) and Pt. Our findings extend the range of potential materials for thermoelectric applications and provide a crucial piece of information for understanding the physics of the spin Seebeck effect.

Observation of longitudinal spin-Seebeck effect in magnetic insulators

We propose a longitudinal spin-Seebeck effect (SSE), in which a magnon-induced spin current is injected parallel to a temperature gradient from a ferromagnet into an attached paramagnetic metal. The longitudinal SSE is measured in a simple and versatile system composed of a ferrimagnetic insulator Y3Fe5O12 slab and a Pt film by means of the inverse spin-Hall effect. The experimental results highlight the intriguing character of the longitudinal SSE due to its own geometric configuration.

Theory of the spin Seebeck effect

The spin Seebeck effect refers to the generation of a spin voltage caused by a temperature gradient in a ferromagnet, which enables the thermal injection of spin currents from the ferromagnet into an attached nonmagnetic metal over a macroscopic scale of several millimeters. The inverse spin Hall effect converts the injected spin current into a transverse charge voltage, thereby producing electromotive force as in the conventional charge Seebeck device. Recent theoretical and experimental efforts have shown that the magnon and phonon degrees of freedom play crucial roles in the spin Seebeck effect. In this paper, we present the theoretical basis for understanding the spin Seebeck effect and briefly discuss other thermal spin effects.

Theory of magnon-driven spin Seebeck effect

The spin Seebeck effect is a spin-motive force generated by a temperature gradient in a ferromagnet that can be detected via normal metal contacts through the inverse spin Hall effect [K. Uchida et al., Nature (London) 455, 778 (2008)]. We explain this effect by spin pumping at the contact that is proportional to the spin-mixing conductance of the interface, the inverse of a temperature-dependent magnetic coherence volume, and the difference between the magnon temperature in the ferromagnet and the electron temperature in the normal metal [D. J. Sanders and D. Walton, Phys. Rev. B 15, 1489 (1977)].

Longitudinal spin Seebeck effect free from the proximity Nernst effect.

This Letter provides evidence for intrinsic longitudinal spin Seebeck effects (LSSEs) that are free from the anomalous Nernst effect (ANE) caused by an extrinsic proximity effect. We report the observation of LSSEs in Au/Y(3)Fe(5)O(12) (YIG) and Pt/Cu/YIG systems, showing that the LSSE appears even when the mechanism of the proximity ANE is clearly removed. In the conventional Pt/YIG structure, furthermore, we separate the LSSE from the ANE by comparing the voltages in different magnetization and temperature-gradient configurations; the ANE contamination was found to be negligibly small even in the Pt/YIG structure.

Observation of the spin Seebeck effect in epitaxial Fe3O4 thin films

We report the experimental observation of the spin Seebeck effect in magnetite thin films. The signal observed at temperatures above the Verwey transition is a contribution from both the anomalous Nernst (ANE) and spin Seebeck (SSE) effects. The contribution from the ANE of the Fe3O4 layer to the SSE is found to be negligible due to the resistivity difference between Fe3O4 and Pt layers. Below the Verwey transition, the SSE is free from the ANE of the ferromagnetic layer and it is also found to dominate over the ANE due to magnetic proximity effect on the Pt layer.

Longitudinal spin-Seebeck effect in sintered polycrystalline (Mn,Zn)Fe2O4

This paper reports that the longitudinal spin-Seebeck effect appears even in a sintered polycrystalline Mn-Zn ferrite [(Mn,Zn)Fe2O4] slab. The effect drives a spin current flowing across an interface between the (Mn,Zn)Fe2O4 slab and an attached Pt film along a temperature gradient and it generates electric voltage via the inverse spin-Hall effect in the Pt film. Since the observed phenomenon enables thermal generation of electric voltage from commonly used polycrystalline insulators, it can be used as a versatile and low-cost thermoelectric generator.

Thermal spin pumping and magnon-phonon-mediated spin-Seebeck effect

The spin-Seebeck effect (SSE) in ferromagnetic metals and insulators has been investigated systematically by means of the inverse spin-Hall effect (ISHE) in paramagnetic metals. The SSE generates a spin voltage as a result of a temperature gradient in a ferromagnet, which injects a spin current into an attached paramagnetic metal. In the paramagnet, this spin current is converted into an electric field due to the ISHE, enabling the electric detection of the SSE. The observation of the SSE is performed in longitudinal and transverse configurations consisting of a ferromagnet/paramagnet hybrid structure, where thermally generated spin currents flowing parallel and perpendicular to the temperature gradient are detected, respectively. Our results explain the SSE in terms of a two-step process: (1) the temperature gradient creates a non-equilibrium state in the ferromagnet governed by both magnon and phonon propagations and (2) the non-equilibrium between magnons in the ferromagnet and electrons in the paramagnet at the contact interface leads to “thermal spin pumping” and the ISHE signal. The non-equilibrium state of metallic magnets (e.g., Ni81Fe19) under a temperature gradient is governed mainly by the phonons in the sample and the substrate, while in insulating magnets (e.g., Y3Fe5O12), both magnon and phonon propagations appear to be important. The phonon-mediated non-equilibrium that drives the thermal spin pumping is confirmed also by temperature-dependent measurements, giving rise to a giant enhancement of the SSE signals at low temperatures.