Harald Sinn

Nanofocusing of hard X-ray free electron laser pulses using diamond based Fresnel zone plates

A growing number of X-ray sources based on the free-electron laser (XFEL) principle are presently under construction or have recently started operation. The intense, ultrashort pulses of these sources will enable new insights in many different fields of science. A key problem is to provide x-ray optical elements capable of collecting the largest possible fraction of the radiation and to focus into the smallest possible focus. As a key step towards this goal, we demonstrate here the first nanofocusing of hard XFEL pulses. We developed diamond based Fresnel zone plates capable of withstanding the full beam of the worlds most powerful x-ray laser. Using an imprint technique, we measured the focal spot size, which was limited to 320 nm FWHM by the spectral band width of the source. A peak power density in the focal spot of 4×1017 W/cm2 was obtained at 70 fs pulse length.

Coherence properties of the European XFEL

The European x-ray free-electron laser (XFEL) provides x-ray self-amplified spontaneous emission (SASE) FEL radiation in the wavelength range from 0.1 to 3 nm using three undulator systems. The SASE mode of operation at the European XFEL defines specific behavior of longitudinal and transverse coherence properties. In this paper, we describe the evolution of the temporal and transverse correlation functions along the undulator length, and we extract the corresponding evolution of coherence time and degree of transverse coherence as typical figures of merit. Generation of coherent radiation inside the FEL undulators is followed by beam transport to the experiments. During transport, the total number of coherent modes is preserved, but the wavefront can be disturbed, and we analyze the conditions under which this occurs. It is emphasized that the development of experimental observables for the degree of coherence and wavefront properties will be important for experiments using coherent x-ray radiation.

Exploring the wavefront of hard X-ray free-electron laser radiation

The high photon flux and femtosecond pulse duration of hard X-ray free-electron lasers have spurred a large variety of novel and fascinating experiments in physical, chemical and biological sciences. Many of these experiments depend fundamentally on a clean, well-defined wavefront. Here we explore the wavefront properties of hard X-ray free-electron laser radiation by means of a grating interferometer, from which we obtain shot-to-shot wavefront information with an excellent angular sensitivity on the order of ten nanoradian. The wavefront distortions introduced by optical elements are observed in-situ and under operational conditions. The source-point position and fluctuations are measured with unprecedented accuracy in longitudinal and lateral direction, both during nominal operation and as the X-ray free-electron laser is driven into saturation.

Damage of amorphous carbon induced by soft x-ray femtosecond pulses above and below the critical angle

We present results of damage studies conducted at the Free Electron LASer in Hamburg (FLASH) facility with 13.5 nm (91.8 eV) and 7 nm (177.1 eV) radiations. The laser beam was focused on a sample of 890-nm-thick amorphous carbon coated on a silicon wafer mimicking a x-ray mirror. The fluence threshold for graphitization was determined for different grazing angles above and below the critical angle. The observed angular dependence of Fth is explained by the variation in absorption depth and reflectivity. Moreover, the absorbed local dose needed for the phase transition leading to graphitization is shown to vary with the radiation wavelength.

Requirements on Hard X-ray Grazing Incidence Optics for European XFEL: Analysis and Simulation of Wavefront Transformations

Analytical and numerical simulations were carried out for both, surface profiles measured on a real ultra precise mirror by use of the BESSY-NOM slope measuring profiler as well as for model local surface distortions. The effect of mirror imperfections could be properly handled in the frame of the wave optics approach. In spite of the large distances, for hard X-rays one still needs to carry out full-scale calculations surpassing the far field approximation. It is shown that the slope errors corresponding to medium spatial frequency components are of a special importance for the properties of coherent beam reflection from ultra smooth mirrors. The typical height errors for this component should not exceed 1-2 nm. Calculations show that reflection on such a mirror surface still imposes substantial wave field distortions at distances of several hundred meters from the mirror relevant for European XFEL beamlines. Requirements and trade-off for high precision mirrors and demands to coherent beams propagations are discussed.

New developments in fabrication of high-energy-resolution analyzers for inelastic X-ray spectroscopy.

New improvements related to the fabrication of spherical bent analyzers for 1 meV energy-resolution inelastic X-ray scattering spectroscopy are presented.

Fluence thresholds for grazing incidence hard x-ray mirrors

X-ray Free Electron Lasers (XFELs) have the potential to contribute to many fields of science and to enable many new avenues of research, in large part due to their orders of magnitude higher peak brilliance than existing and future synchrotrons. To best exploit this peak brilliance, these XFEL beams need to be focused to appropriate spot sizes. However, the survivability of X-ray optical components in these intense, femtosecond radiation conditions is not guaranteed. As mirror optics are routinely used at XFEL facilities, a physical understanding of the interaction between intense X-ray pulses and grazing incidence X-ray optics is desirable. We conducted single shot damage threshold fluence measurements on grazing incidence X-ray optics, with coatings of ruthenium and boron carbide, at the SPring-8 Angstrom compact free electron laser facility using 7 and 12 keV photon energies. The damage threshold dose limits were found to be orders of magnitude higher than would naively be expected. The incorporation of energy transport and dissipation via keV level energetic photoelectrons accounts for the observed damage threshold.

Recent development of thin diamond crystals for X-ray FEL beam-sharing

The recent success of the X-ray Free Electron Lasers has generated great interests from the user communities of a wide range of scientific disciplines including physics, chemistry, structural biology and material science, creating tremendous demand on FEL beamtime access. Due to the serial nature of FEL operation, various beam-sharing techniques have been investigated in order to potentially increase the FEL beamtime capacity. Here we report the recent development in using thin diamond single crystals for spectrally splitting the FEL beam at the Linac Coherent Light Source, thus potentially allowing the simultaneous operation of multiple instruments. Experimental findings in crystal mounting and its thermal performance, position and pointing stabilities of the reflected beam, and impact of the crystal on the FEL transmitted beam profile are presented.

Design of an x-ray split- and delay-unit for the European XFEL

For the European XFEL [1] an x-ray split- and delay-unit (SDU) is built covering photon energies from 5 keV up to 20 keV. This SDU will enable time-resolved x-ray pump / x-ray probe experiments as well as sequential diffractive imaging [2] on a femtosecond to picosecond time scale. Further, direct measurements of the temporal coherence properties will be possible by making use of a linear autocorrelation. The set-up is based on geometric wavefront beam splitting, which has successfully been implemented at an autocorrelator at FLASH [3]. The x-ray FEL pulses will be split by a sharp edge of a silicon mirror coated with Mo/B4C multi layers. Both partial beams will then pass variable delay lines. For different wavelengths the angle of incidence onto the multilayer mirrors will be adjusted in order to match the Bragg condition. For a photon energy of hν = 20 keV a grazing angle of θ = 0.57° has to be set, which results in a footprint of the beam (6σ) on the mirror of l = 345 mm. At this photon energy the reflectance of a Mo/B4C multi layer coating with a multi layer period of d = 3 nm and N = 200 layers amounts to R = 0.92. For a photon energy of hν = 5 keV a smaller size of the footprint of l = 244 mm is calculated due to the steeper grazing angle of θ = 2.28°. In order to enhance the maximum transmission for photon energies of hν = 8 keV and below, a Ni/B4C multilayer coating can be applied beside the Mo/B4C coating for this spectral region. Because of the different incidence angles, the path lengths of the beams will differ as a function of wavelength. Hence, maximum delays between +/- 3.7 ps at hν = 20 keV and up to +/- 44 ps at hν = 5 keV will be possible.

Investigating the interaction of x-ray free electron laser radiation with grating structure.

The interaction of free electron laser pulses with grating structure is investigated using 4.6±0.1 nm radiation at the FLASH facility in Hamburg. For fluences above 63.7±8.7 mJ/cm2, the interaction triggers a damage process starting at the edge of the grating structure as evidenced by optical and atomic force microscopy. Simulations based on solution of the Helmholtz equation demonstrate an enhancement of the electric field intensity distribution at the edge of the grating structure. A procedure is finally deduced to evaluate damage threshold.