Irnis Kubat

Multi-milliwatt mid-infrared supercontinuum generation in a suspended core chalcogenide fiber

A low-loss suspended core As(38)Se(62) fiber with core diameter of 4.5 μm and a zero-dispersion wavelength of 3.5 μm was used for mid-infrared supercontinuum generation. The dispersion of the fiber was measured from 2.9 to 4.2 μm and was in good correspondence with the calculated dispersion. An optical parametric amplifier delivering 320 fs pulses with a peak power of 14.8 kW at a repetition rate of 21 MHz was used to pump 18 cm of suspended core fiber at different wavelengths from 3.3 to 4.7 μm. By pumping at 4.4 μm with a peak power of 5.2 kW coupled to the fiber a supercontinuum spanning from 1.7 to 7.5 μm with an average output power of 15.6 mW and an average power >5.0 μm of 4.7 mW was obtained.

Thulium pumped mid-infrared 0.9-9μm supercontinuum generation in concatenated fluoride and chalcogenide glass fibers.

We theoretically demonstrate a novel approach for generating Mid-InfraRed SuperContinuum (MIR SC) by using concatenated fluoride and chalcogenide glass fibers pumped with a standard pulsed Thulium (Tm) laser (T(FWHM)=3.5ps, P0=20kW, ν(R)=30MHz, and P(avg)=2W). The fluoride fiber SC is generated in 10m of ZBLAN spanning the 0.9-4.1μm SC at the -30dB level. The ZBLAN fiber SC is then coupled into 10cm of As2Se3 chalcogenide Microstructured Optical Fiber (MOF) designed to have a zero-dispersion wavelength (λ(ZDW)) significantly below the 4.1μm InfraRed (IR) edge of the ZBLAN fiber SC, here 3.55μm. This allows the MIR solitons in the ZBLAN fiber SC to couple into anomalous dispersion in the chalcogenide fiber and further redshift out to the fiber loss edge at around 9μm. The final 0.9-9μm SC covers over 3 octaves in the MIR with around 15mW of power converted into the 6-9μm range.

Mid-infrared supercontinuum generation to 12.5μm in large NA chalcogenide step-index fibres pumped at 4.5μm

We present numerical modeling of mid-infrared (MIR) supercontinuum generation (SCG) in dispersion-optimized chalcogenide (CHALC) step-index fibres (SIFs) with exceptionally high numerical aperture (NA) around one, pumped with mode-locked praseodymium-doped (Pr(3+)) chalcogenide fibre lasers. The 4.5um laser is assumed to have a repetition rate of 4MHz with 50ps long pulses having a peak power of 4.7kW. A thorough fibre design optimisation was conducted using measured material dispersion (As-Se/Ge-As-Se) and measured fibre loss obtained in fabricated fibre of the same materials. The loss was below 2.5dB/m in the 3.3-9.4μm region. Fibres with 8 and 10μm core diameters generated an SC out to 12.5 and 10.7μm in less than 2m of fibre when pumped with 0.75 and 1kW, respectively. Larger core fibres with 20μm core diameters for potential higher power handling generated an SC out to 10.6μm for the highest NA considered but required pumping at 4.7kW as well as up to 3m of fibre to compensate for the lower nonlinearities. The amount of power converted into the 8-10μm band was 7.5 and 8.8mW for the 8 and 10μm fibres, respectively. For the 20μm core fibres up to 46mW was converted.

Refractive index dispersion of chalcogenide glasses for ultra-high numerical-aperture fiber for mid-infrared supercontinuum generation

We select a chalcogenide core glass, AsSe, and cladding glass, GeAsSe, for their disparate refractive indices yet sufficient thermal-compatibility for fabricating step index fiber (SIF) for mid-infrared supercontinuum generation (MIR-SCG). The refractive index dispersion of both bulk glasses is measured over the 0.4 µm–33 µm wavelength-range, probing the electronic and vibrational behavior of these glasses. We verify that a two-term Sellmeier model is unique and sufficient to describe the refractive index dispersion over the wavelength range for which the experimentally determined extinction coefficient is insignificant. A SIF composed of the glasses is fabricated and calculated to exhibit an ultra-high numerical aperture >0.97 over the entire wavelength range 0.4-33 µm suggesting that the SIF glass pair is a promising candidate for MIR-SCG. Material dispersion characteristics and the zero dispersion wavelength, both critical design parameters for SIF for MIR-SCG, are derived.

Hybrid polymer photonic crystal fiber with integrated chalcogenide glass nanofilms

The combination of chalcogenide glasses with polymer photonic crystal fibers (PCFs) is a difficult and challenging task due to their different thermo-mechanical material properties. Here we report the first experimental realization of a hybrid polymer-chalcogenide PCF with integrated As2S3 glass nanofilms at the inner surface of the air-channels of a poly-methyl-methacrylate (PMMA) PCF. The integrated high refractive index glass films introduce distinct antiresonant transmission bands in the 480–900 nm wavelength region. We demonstrate that the ultra-high Kerr nonlinearity of the chalcogenide glass makes the polymer PCF nonlinear and provides a possibility to shift the transmission band edges as much as 17 nm by changing the intensity. The proposed fabrication technique constitutes a new highway towards all-fiber nonlinear tunable devices based on polymer PCFs, which at the moment is not possible with any other fabrication method.

Multimode supercontinuum generation in chalcogenide glass fibres.

Mid-infrared supercontinuum generation is considered in chalcogenide fibres when taking into account both polarisations and the necessary higher order modes. In particular we focus on high pulse energy supercontinuum generation with long pump pulses. The modeling indicates that when only a single polarisation in the fundamental mode is considered the obtainable supercontinuum bandwidth is substantially exaggerated compared to when both polarisations are taken into account. Our modeling shows that if the pump pulse is short enough (≤ 10 ps) then higher order modes are not important because of temporal walk-off. In contrast long pump pulses (≥ 40 ps) will efficiently excite higher order modes through Raman scattering, which will deplete the fundamental mode of energy and limit the possibility of obtaining a broadband supercontinuum.

High average power mid-infrared supercontinuum generation in a suspended core chalcogenide fiber

Mid-infrared supercontinuum spanning from 2.0 to 6.1 μm is generated in a 9 cm suspended core chalcogenide fiber by pumping close to the fiber zero-dispersion wavelength at 3.5 μm with an OPA system.

Towards the mid-infrared optical biopsy

We are establishing a new paradigm in mid-infrared molecular sensing, mapping and imaging to open up the midinfrared spectral region for in vivo (i.e. in person) medical diagnostics and surgery. Thus, we are working towards the mid-infrared optical biopsy (‘opsy’ look at, bio the biology) in situ in the body for real-time diagnosis. This new paradigm will be enabled through focused development of devices and systems which are robust, functionally designed, safe, compact and cost effective and are based on active and passive mid-infrared optical fibers. In particular, this will enable early diagnosis of external cancers, mid-infrared detection of cancer-margins during external surgery for precise removal of diseased tissue, in one go during the surgery, and mid-infrared endoscopy for early diagnosis of internal cancers and their precision removal. The mid-infrared spectral region has previously lacked portable, bright sources. We set a record in demonstrating extreme broad-band supercontinuum generated light 1.4 to 13.3 microns in a specially engineered, high numerical aperture mid-infrared optical fiber. The active mid-infrared fiber broadband supercontinuum for the first time offers the possibility of a bright mid-infrared wideband source in a portable package as a first step for medical fiber-based systems operating in the mid-infrared. Moreover, mid-infrared molecular mapping and imaging is potentially a disruptive technology to give improved monitoring of the environment, energy efficiency, security, agriculture and in manufacturing and chemical processing. This work is in part supported by the European Commission: Framework Seven (FP7) Large-Scale Integrated Project MINERVA: MId-to-NEaR- infrared spectroscopy for improVed medical diAgnostics (317803; www.minerva-project.eu).

Nonlinear Kerr effect in a hybrid polymer/chalcogenide photonic crystal fiber

We fabricated and characterized a hybrid As2S3/PMMA photonic crystal fiber. The high index chalcogenide glass films provide the possibility to red-shift the transmission windows as much as ~ 17 nm with power

Mid-infrared supercontinuum generation spanning more than 11 μm in a chalcogenide step-index fiber

Supercontinuum generation covering an ultra-broad spectrum from 1.5-11.7μm and 1.4-13.3μm is experimentally demonstrated by pumping an 85mm chalcogenide step-index fiber with 100fs pulses at a wavelength of 4.5μm and 6.3μm, respectively.