J. E. Sonier

Evidence for static magnetism in the vortex cores of ortho-II YBa2Cu3O6.50.

Evidence for static alternating magnetic fields in the vortex cores of underdoped YBa2Cu3O6+x is reported. Muon spin rotation measurements of the internal magnetic field distribution of the vortex state of YBa2Cu3O6.50 in applied fields of H = 1 T and H = 4 T reveal a feature in the high-field tail of the field distribution which is not present in optimally doped YBa2Cu3O6.95 and which fits well to a model with static magnetic fields in the vortex cores. The magnitude of the fields is estimated to be 18(2) G and decreases above T = 10 K. We discuss possible origins of the additional vortex core magnetism within the context of existing theories.

Field Induced Reduction of the Low-Temperature Superfluid Density in YBa{sub 2}Cu{sub 3}O{sub 6.95}

A novel high magnetic field (8 T) spectrometer for muon spin rotation has been used to measure the temperature dependence of the in-plane magnetic penetration depth {lambda}{sub ab} in YBa{sub 2}Cu {sub 3}O{sub 6.95} . At low H and low T , {lambda}{sub ab} exhibits the characteristic linear T dependence associated with the energy gap of a d{sub x{sup 2}-y{sup 2}}-wave superconductor. However, at higher fields {lambda}{sub ab} is essentially temperature independent at low T . We discuss possible interpretations of this surprising new feature in the low-energy excitation spectrum. (c) 1999 The American Physical Society.

Glassy Spin Dynamics in Non-Fermi-Liquid UCu5xPdx, x = 1.0 and 1.5

Local f-electron spin dynamics in the non-Fermi-liquid heavy-fermion alloys UCu5-xPdx, x = 1.0 and 1.5, have been studied using muon spin-lattice relaxation. The sample-averaged asymmetry function G(t) indicates strongly inhomogeneous spin fluctuations and exhibits the scaling G(t,H) = G(t/H(gamma)) expected from glassy dynamics. At 0.05 K gamma(x = 1.0) = 0.35+/-0.1, but gamma(x = 1.5) = 0.7+/-0.1. This is in contrast to inelastic neutron scattering results, which yield gamma = 0.33 for both concentrations. There is no sign of static magnetism approximately greater than 10(-3)(B)/U ion in either material above 0.05 K. Our results strongly suggest that both alloys are quantum spin glasses.

Detection of the unusual magnetic orders in the pseudogap region of a high-temperature superconducting YBa2Cu3O6.6 crystal by muon-spin relaxation.

We present muon-spin relaxation (muSR) measurements on a large YBa2Cu3O6.6 single crystal in which two kinds of unusual magnetic order have been detected in the pseudogap region by neutron scattering. A comparison is made to measurements on smaller, higher quality YBa2Cu3Oy single crystals. One type of magnetic order is observed in all samples, but does not evolve significantly with hole doping. A second type of unusual magnetic order is observed only in the YBa2Cu3O6.6 single crystal. This magnetism has an ordered magnetic moment that is quantitatively consistent with the neutron experiments, but is confined to just a small volume of the sample ( approximately 3%). Our findings do not support theories that ascribe the pseudogap to a state characterized by loop-current order, but instead indicate that dilute impurity phases are the source of the unusual magnetic orders in YBa2Cu3Oy.

Inhomogeneous magnetic-field response of YBa2Cu3Oy and La2-xSrxCuO4 persisting above the bulk superconducting transition temperature.

We report that in YBa2Cu3Oy and La2-xSrxCuO4 there is a spatially inhomogeneous response to the magnetic field for temperatures T extending well above the bulk-superconducting transition temperature Tc. An inhomogeneous magnetic response is observed above Tc even in ortho-II YBa2Cu3O6.50, which has highly ordered doping. The degree of the field inhomogeneity above Tc tracks the hole-doping dependences of both Tc and the density of the superconducting carriers below Tc, and therefore is apparently coupled to superconductivity.

Correlations between charge ordering and local magnetic fields in overdoped YBa2Cu3O6+x

Zero-field muon spin-relaxation (ZF-μSR) measurements were undertaken on under- and overdoped samples of superconducting YBa 2 Cu 3 O 6 + x to determine the origin of the weak static magnetism recently reported in this system. The temperature dependence of the muon spin-relaxation rate in overdoped crystals displays an unusual behavior in the superconducting state. A comparison to the results of NQR and lattice structure experiments on highly doped samples provides compelling evidence for strong coupling of charge, spin, and structural inhomogeneities.

Hole-doping dependence of the magnetic penetration depth and vortex core size in YBa2Cu3Oy : Evidence for stripe correlations near 1/8 hole doping

We report on muon spin rotation measurements of the internal magnetic field distribution n(B) in the vortex solid phase of YBa2Cu3Oy (YBCO) single crystals, from which we have simultaneously determined the hole doping dependences of the in-plane Ginzburg-Landau (GL) length scales in the underdoped regime. We find that Tc has a sublinear dependence on 1/lambda_{ab}^2, where lambda_{ab} is the in-plane magnetic penetration depth in the extrapolated limits T -> 0 and H -> 0. The power coefficient of the sublinear dependence is close to that determined in severely underdoped YBCO thin films, indicating that the same relationship between Tc and the superfluid density is maintained throughout the underdoped regime. The in-plane GL coherence length (vortex core size) is found to increase with decreasing hole doping concentration, and exhibit a field dependence that is explained by proximity-induced superconductivity on the CuO chains. Both the magnetic penetration depth and the vortex core size are enhanced near 1/8 hole doping, supporting the belief by some that stripe correlations are a universal property of high-Tc cuprates.

m(+) knight shift measurements in U0.965Th0.035Be13 single crystals

Muon spin rotation ( &mgr;SR) measurements of the temperature dependence of the &mgr;(+) Knight shift in single crystals of U0. 965Th0.035Be13 have been used to study the static spin susceptibility chi(s) below the transition temperatures T(c1) and T(c2). While an abrupt reduction of chi(s) with decreasing temperature is observed below T(c1), chi(s) does not change below T(c2) and remains at a value below the normal-state susceptibility chi(n). In the normal state we find an anomalous anisotropic temperature dependence of the transferred hyperfine coupling between the &mgr;(+) spin and the U 5f electrons.

Slow spin dynamics in non-fermi-liquid UCu5-xPdx, x = 1.0 and 1.5

Abstract Low-temperature muon spin-lattice relaxation measurements in the non-Fermi-liquid heavy-fermion alloys UCu 5− x Pd x , x =1.0 and 1.5, indicate inhomogeneously distributed f-electron spin fluctuation rates, and exhibit a time-field scaling of the muon relaxation function indicative of long-lived spin correlations. In UCu 4 Pd the scaling exponent γ is small and temperature independent. In UCu 3.5 Pd 1.5 γ varies with temperature, increasing with decreasing temperature similar to spin-glass AgMn. This suggests that the spin-glass state found for x ≳2 in UCu 5− x Pd x modifies the low-frequency spin dynamics in UCu 3.5 Pd 1.5 .

Signatures of new d-wave vortex physics in overdoped Tl2Ba2CuO(6+x) revealed by TF-µ(+)SR.

The spontaneous expulsion of applied magnetic field, the Meissner effect, is a defining feature of superconductors; in Type-II superconductors above the lower critical field, this screening takes the form of a lattice of magnetic flux vortices. Using implanted spin-1/2 positive muons, one can measure the vortex lattice field distribution through the spin precession and deduce key parameters of the superconducting ground state, and thereby fundamental properties of the superconducting pairing. Muon spin rotation/relaxation (µSR) experiments have indeed revealed much interesting physics in the underdoped cuprates, where superconductivity is closely related to, or coexistent with, disordered or fluctuating magnetic and charge excitations. Such complications should be absent in overdoped cuprates, which are believed to exhibit conventional Fermi liquid behaviour. These first transverse field (TF)-µ+SR experiments on heavily-overdoped single crystals reveal a superfluid density exhibiting a clear inflection point near 0.5Tc , with a striking doping-independent scaling. This reflects hitherto unrecognized physics intrinsic to d-wave vortices, evidently generic to the cuprates, and may offer fundamentally new insights into their still-mysterious superconductivity.