J.-F. Daigle

Advances in intense femtosecond laser filamentation in air

This is a review of some recent development in femtosecond filamentation science with emphasis on our collective work. Previously reviewed work in the field will not be discussed. We thus start with a very brief description of the fundamental physics of single filamentation of powerful femtosecond laser pulses in air. Intensity clamping is emphasized. One consequence is that the peak intensity inside one or more filaments would not increase significantly even if one focuses the pulse at very high peak power even up to the peta-watt level. Another is that the clamped intensity is independent of pressure. One interesting outcome of the high intensity inside a filament is filament fusion which comes from the nonlinear change of index of refraction inside the filament leading to cross beam focusing. Because of the high intensity inside the filament, one can envisage nonlinear phenomena taking place inside a filament such as a new type of Raman red shift and the generation of very broad band supercontinuum into the infrared through four-wave-mixing. This is what we call by filamentation nonlinear optics. It includes also terahertz generation from inside the filament. The latter is discussed separately because of its special importance to those working in the field of safety and security in recent years. When the filamenting pulse is linearly polarized, the isotropic nature of air becomes birefringent both electronically (instantaneous) and through molecular wave packet rotation and revival (delayed). Such birefringence is discussed in detailed. Because, in principle, a filament can be projected to a long distance in air, applications to pollution measurement as well as other atmospheric science could be earned out. We call this filamentation atmospheric science. Thus, the following subjects are discussed briefly, namely, lightning control, rain making, remote measurement of electric field, microwave guidance and remote sensing of pollutants. A discussion on the higher order Kerr effect on the physics of filamentation is also given. This is a new hot subject of current debate. This review ends on giving our view of the prospect of progress of this field of filamentation in the future. We believe it hinges upon the development of the laser technology based upon the physical understanding of filamentation and on the reduction in price of the laser system.

Arrest of self-focusing collapse in femtosecond air filaments: higher order Kerr or plasma defocusing?

Experimentally measured conical emission rings on the blue side of the filament supercontinuum of a 800 nm 50 fs pulse in air are reproduced in simulations with plasma and the third-order Kerr as the nonlinear terms. This agreement indicates plasma as the dominant mechanism arresting the self-focusing collapse. The higher order Kerr terms with the recently measured coefficients stop the collapse at a lower intensity than the plasma does and lead to the spherical angle-wavelength spectrum without blueshifted rings.

Multioctave infrared supercontinuum generation in large-core As2S3 fibers

We report on infrared supercontinuum (SC) generation through laser filamentation and subsequent nonlinear propagation in a step-index As2S3 fiber. The 100 μm core and high-purity As2S3 fiber used exhibit zero-dispersion wavelength around 4.5 μm, a mid-infrared background loss of 0.2  dB/m, and a maximum loss of only 0.55  dB/m at the S-H absorption peak around 4.05 μm. When pumping with ultrashort laser pulses slightly above the S-H absorption band, broadband infrared supercontinua were generated with a 20 dB spectral flatness spanning from 1.5 up to 7 μm. The efficiency and spectral shape of the SC produced by ultrashort pulses in large-core As2S3 fiber are mainly determined by its dispersion, the S-H contaminant absorption, and the mid-infrared nonlinear absorption.

Mid-infrared supercontinuum generation in fluoroindate fiber

We report the generation of mid-infrared supercontinua in a step-index fluoroindate-based fiber. The large core of the fluoroindate fiber allows the guiding of multiwatt laser power over a broad spectral range. These fibers exhibit zero dispersion at 1.83 μm, minimal loss of 0.1 dB/m at 3.2 μm up to only 0.8 dB/m at 5 μm. These specifications enable mid-infrared supercontinuum generation and propagation with low loss. By using mid-infrared ultrashort laser pulses from an optical parametric amplifier, we demonstrate generation of a 20 dB spectral flatness supercontinua from 2.7 to 4.7 μm in the fluoroindate fiber, which is twice the spectral broadening compared to a ZBLAN fiber under similar conditions.

Self-seeded forward lasing action from a femtosecond Ti:sapphire laser filament in air

428 nm forward lasing action was observed from a femtosecond laser filament in air created by Ti:sapphire laser pulses. The 800 nm femtosecond laser filament not only provides a source for population inversion between two vibrational levels ( and ) of N2+ but also generates a 428 nm seed from filament-induced white light. This simple technique will find more applications in standoff spectroscopy.

Toward remote high energy terahertz generation

Remote terahertz (THz) generation from a two-color femtosecond laser-induced filament in air was experimentally demonstrated. A record of remote THz emission at 16 m was achieved. THz pulse energy more than 250 nJ in the frequency range below 5.5 THz was recorded; this is two orders of magnitude stronger than that from single-color excitation. Back-scattered nitrogen (N2) fluorescence signal remotely measured with a lidar is linearly proportional to the THz emission, which would provide a more practical method to characterize the THz pulses.

Remote THz generation from two-color filamentation: long distance dependence.

Remote terahertz (THz) generation from two-color filamentation is investigated as a function of the onset position of filaments. THz signals emitted by filaments produced at distances up to 55 m from the laser source were measured. However, from 9 m to 55 m, the THz signal decayed monotonically for increasing onset positions. With a simple calculation, the dominant factors associated to this decay were identified as group velocity mismatch of the two-color pulses and linear diffraction induced by focusing and propagating the second harmonic pulse.

Laser guiding of Tesla coil high voltage discharges.

We have investigated the guiding and triggering of discharges from a Tesla coil type 280 kHz AC high voltage source using filaments created by a femtosecond Terawatt laser pulse. Without the laser the discharges were maximum 30 cm long. With the laser straight, guided discharges up to 110 cm length were detected. The discharge length was limited by the voltage amplitude of the Tesla coil.

Remote generation of high-energy terahertz pulses from two-color femtosecond laser filamentation in air

We experimentally investigated the dynamic behavior of remote terahertz (THz) generation from two-color femtosecond laser-induced filamentation in air. A record-high THz pulse energy of 570 nJ at frequency below 5.5 THz was measured by optimizing the pump parameters at a controllable remote distance of 16 m, while super-broadband THz (<300 THz) pulse energy was up to 2.8 {mu}J. A further energy-scaling possibility was proposed. By analyzing simultaneously the fluorescence from both neutral N{sub 2} and N{sub 2}{sup +} in the filament, we found that the enhancement of THz radiation was due principally to guiding of the weak second-harmonic pulse inside the filament of the first strong fundamental pulse.

Laser-guided energetic discharges over large air gaps by electric-field enhanced plasma filaments.

Recent works on plasma channels produced during the propagation of ultrashort and intense laser pulses in air demonstrated the guiding of electric discharges along the laser path. However, the short plasma lifetime limits the length of the laser-guided discharge. In this paper, the conductivity and lifetime of long plasma channels produced by ultrashort laser pulses is enhanced efficiently over many orders of magnitude by the electric field of a hybrid AC-DC high-voltage source. The AC electric pulse from a Tesla coil allowed to stimulate and maintain the highly conductive channel during few milliseconds in order to guide a subsequent 500 times more energetic discharge from a 30-kV DC source. This DC discharge was laser-guided over an air gap length of two metres, which is more than two orders of magnitude longer than the expected natural discharge length. Long plasma channel induced by laser pulses and stimulated by an external high-voltage source opens the way for wireless and efficient transportation of energetic current pulses over long air gaps and potentially for guiding lightning.