Jacob Baron

Order of Magnitude Smaller Limit on the Electric Dipole Moment of the Electron

Stubbornly Spherical The shape of the electrons charge distribution reflects the degree to which switching the direction of time impacts the basic ingredients of the universe. The Standard Model (SM) of particle physics predicts a very slight asphericity of the charge distribution, whereas SM extensions such as supersymmetry posit bigger and potentially measurable, but still tiny, deviations from a perfect sphere. Polar molecules have been identified as ideal settings for measuring this asymmetry, which should be reflected in a finite electric dipole moment (EDM) because of the extremely large effective electric fields that act on an electron inside such molecules. Using electron spin precession in the molecule ThO, Baron et al. (p. 269, published online 19 December; see the cover; see the Perspective by Brown) measured the EDM of the electron as consistent with zero. This excludes some of the extensions to the SM and sets a bound to the search for a nonzero EDM in other facilities, such as the Large Hadron Collider. Spin precession measurements in the polar molecule thorium monoxide indicate a nearly spherical charge distribution of an electron. [Also see Perspective by Brown] The Standard Model of particle physics is known to be incomplete. Extensions to the Standard Model, such as weak-scale supersymmetry, posit the existence of new particles and interactions that are asymmetric under time reversal (T) and nearly always predict a small yet potentially measurable electron electric dipole moment (EDM), de, in the range of 10−27 to 10−30 e·cm. The EDM is an asymmetric charge distribution along the electron spin (S→) that is also asymmetric under T. Using the polar molecule thorium monoxide, we measured de = (–2.1 ± 3.7stat ± 2.5syst) × 10−29 e·cm. This corresponds to an upper limit of | de | < 8.7 × 10−29 e·cm with 90% confidence, an order of magnitude improvement in sensitivity relative to the previous best limit. Our result constrains T-violating physics at the TeV energy scale.

Methods, Analysis, and the Treatment of Systematic Errors for the Electron Electric Dipole Moment Search in Thorium Monoxide

We recently set a new limit on the electric dipole moment of the electron (eEDM) (J Baron et al and ACME collaboration 2014 Science 343 269–272), which represented an order-of-magnitude improvement on the previous limit and placed more stringent constraints on many charge-parity-violating extensions to the standard model. In this paper we discuss the measurement in detail. The experimental method and associated apparatus are described, together with the techniques used to isolate the eEDM signal. In particular, we detail the way experimental switches were used to suppress effects that can mimic the signal of interest. The methods used to search for systematic errors, and models explaining observed systematic errors, are also described. We briefly discuss possible improvements to the experiment.

STIRAP preparation of a coherent superposition of ThO

Experimental searches for the electron electric dipole moment (EDM) probe new physics beyond the Standard Model. The current best EDM limit was set by the ACME Collaboration [Science \textbf{343}, 269 (2014)], constraining time reversal symmetry (

H^3\Delta_1

T

states for an improved electron EDM measurement

) violating physics at the TeV energy scale. ACME used optical pumping to prepare a coherent superposition of ThO

Measurement of the 4S1/2→6S1/2 transition frequency in atomic potassium via direct frequency-comb spectroscopy

H^3\Delta_1

Invariances in a Combinatorial Olfactory Receptor Code

states that have aligned electron spins. Spin precession due to the molecules internal electric field was measured to extract the EDM. We report here on an improved method for preparing this spin-aligned state of the electron by using STIRAP. We demonstrate a transfer efficiency of

Improved Thermochemical Beam Source of ThO for Measuring the Electric Dipole Moment of the Electron

75\pm5\%

Future Improvements to the ACME Electric Dipole Moment Experiment

, representing a significant gain in signal for a next generation EDM experiment. We discuss the particularities of implementing STIRAP in systems such as ours, where molecular ensembles with large phase-space distributions are transfered via weak molecular transitions with limited laser power and limited optical access.

Electron EDM measurement in a beam of ThO: Demonstrated and planned upgrades

We present an experimental determination of the 4 S1/2 → 6 S1/2 transition frequency in atomic potassium, K, using direct frequency comb spectroscopy. The output of a stabilized optical frequency comb was used to excite a thermal atomic vapor. The repetition rate of the frequency comb was scanned and the transitions were excited using step-wise two-photon excitation. The center of gravity frequency for the transition was found to be νcog = 822 951 698.09(13) MHz and the measured hyperfine A coefficient of the 6 S1/2 state was 21.93(11) MHz. The measurements are in agreement with previous values and represent an improvement by a factor of 700 in the uncertainty of the center of gravity measurement.