Jean-Michel Melkonian

High spectral purity and tunable operation of a continuous singly resonant optical parametric oscillator emitting in the red.

Continuous-wave oscillation of a singly resonant optical parametric oscillator operating from 619 to 640 nm has been obtained. Parametric gain is created in a MgO-doped periodically poled stoichiometric lithium tantalate crystal pumped at 532 nm. 100 mW of single-frequency red light have been generated. The signal frequency is tunable, and its frequency stabilization on an external reference has been achieved.

Multispecies high-energy emitter for CO 2 , CH 4 , and H 2 O monitoring in the 2 μm range

We demonstrate the first emitter, based on a single optical source device, capable of addressing three species of interest (CO₂, CH₄, and H₂O) for differential absorption Lidar remote sensing of atmospheric greenhouse gases from space in the 2 μm region. It is based on an amplified nested cavity optical parametric oscillator. The single frequency source shows a total conversion efficiency of 37% and covers the 2.05-2.3 μm range.

Passive mode locking of optical parametric oscillators: an efficient technique for generating sub-picosecond pulses

We show that optical parametric generation in a nonlinear crystal with a large group velocity mismatch between the pump and nearly-degenerate signal and idler is analogous to laser amplification in the medium with a gain recovery time comparable to the walk-off time. Based on this conclusion we propose to combine an OPO with a nonlinear saturable absorber or Kerr lens to generate directly high peak power sub-picosecond pulses using pump pulses ranging from tens of picoseconds to quasi-CW. Our analytical model predicts better than 80% photon conversion efficiency and pulse lengths that are of the order of a few hundred femtoseconds. Numerical simulations confirm our predictions and show that repetitive passive mode locking is feasible with a quasi-CW pump.

Spectrotemporal dynamics of a picosecond OPO based on chirped quasi-phase-matching

We report on the first experimental investigation of the spectral dynamics of a synchronously pumped optical parametric oscillator (OPO) by use of dispersive Fourier transformation. For standard pumping rates, we observe a reproducible steady-state pulse-to-pulse spectrum. However, at high pumping levels, the OPO delivers pulse trains with nontrivial oscillatory spectral patterns. So as to benefit from a tailored broadband gain spectrum, the investigated OPO contains a chirped quasi-phase matching (QPM) nonlinear crystal. We explore the specific impacts of using such a remarkable parametric amplification medium where nonlinearly coupled frequencies vary with position. Depending on the QPM chirp rate sign, a red- or blue-shift of the emitted wavelength occurs when the OPO is switched on, leading to different spectral steady-states. These singular spectrotemporal dynamics are evidenced and explained for the first time.

Longwave infrared, single-frequency, tunable, pulsed optical parametric oscillator based on orientation-patterned GaAs for gas sensing.

We demonstrate a nanosecond single-frequency nested cavity optical parametric oscillator (NesCOPO) based on orientation-patterned GaAs (OP-GaAs). Its low threshold energy of 10 μJ enables to pump it with a pulsed single-frequency Tm:YAP microlaser. Stable single-longitudinal-mode emission is obtained owing to Vernier spectral filtering provided by the dual-cavity doubly-resonant NesCOPO scheme. Crystal temperature tuning covers the 10.3-10.9 μm range with a quasi-phase-matching period of 72.6 μm. A first step toward the implementation of this device in a differential absorption lidar is demonstrated by carrying out short-range standoff detection of ammonia vapor around 10.4 μm. Owing to the single-frequency emission, interferences due to absorption by atmospheric water vapor can be discriminated from the analyte signal.

Active mode locking of continuous-wave doubly and singly resonant optical parametric oscillators

We report on what we believe to be the first active mode locking of near-degenerate, doubly and singly resonant cw-pumped optical parametric oscillators (OPOs). We show experimentally that a steady-state regime of short pulses is reached in a few tens of microseconds under cw pumping. The oscillation buildup dynamics of both OPOs is also explored, evidencing an unusual transient behavior in the mode-locking process.

Microsecond fiber laser pumped, single-frequency optical parametric oscillator for trace gas detection

We report on the first microsecond doubly resonant optical parametric oscillator (OPO). It is based on a nested cavity OPO architecture allowing single longitudinal mode operation and low oscillation threshold (few microjoule). The combination with a master oscillator-power amplifier fiber pump laser provides a versatile optical source widely tunable in the 3.3-3.5 μm range with an adjustable pulse repetition rate (from 40 to 100 kHz), high duty cycle (~10(-2)) and mean power (up to 25 mW in the idler beam). The potential for trace gas sensing applications is demonstrated through photoacoustic detection of atmospheric methane.

Dual-wavelength source from 5%MgO:PPLN cylinders for the characterization of nonlinear infrared crystals

We conceived a unique fully parametric source based on two independent cylindrical OPOs simultaneously pumped by the same Nd:YAG laser. Each OPO delivers more than 2 mJ and is continuously tunable between 1.41 µm and 4.3 µm. This source is of particular interest for the study of the generation of infrared parametric light in nonlinear crystals. It was validated by performing difference frequency generation experiments in CdSe crystals with output in the range 8 - 10 µm.

Analysis of cavity-length detuning in diffraction-grating narrowed picosecond optical parametric oscillators

We report on the detailed investigation of picosecond synchronously pumped optical parametric oscillators (OPOs) with a Littrow-mounted diffraction grating as the tuning element, operating close to and far from degeneracy. In addition to the expected line-narrowing effect, we observe a fivefold increase of the resonator-length detuning tolerance when compared to conventional mirror-based OPOs. When the OPO resonator length is altered, we also measure reproducible variations of the emitted wavelength associated with lateral beam displacements that were not reported before. We show that all of these effects can be explained by a geometric adaptation of the resonant beam path within the cavity to maintain a constant cavity round-trip time.

Rapidly tunable optical parametric oscillator based on aperiodic quasi-phase matching.

A new optical parametric oscillator (OPO) architecture with high tuning speed capability is demonstrated. This device exploits the versatility offered by aperiodic quasi-phase matching (QPM) to provide a broad parametric gain spectrum without changing the temperature, angle, or position of the nonlinear crystal. Rapid tuning is then straightforwardly achieved using a fast intracavity spectral filter. This concept is demonstrated here for a picosecond synchronously pumped OPO containing an aperiodically poled MgO-doped LiNbO3 crystal and a rapidly tunable spectral filter based on a diffraction grating. Tuning over 160 nm around 3.86 μm is achieved at fixed temperature and a fast tuning over 30 nm in 40 μs is demonstrated. Different configurations are tested and compared. The cavity length detuning is analyzed and discussed. This device is successfully used to detect N2O by absorption. This approach could be generalized to other spectral ranges (e.g., visible) and temporal regimes (e.g., continuous-wave or nanosecond).