Jean-Pierre Likforman

Measurement of photon echoes by use of femtosecond Fourier-transform spectral interferometry

Using Fourier-transform spectral interferometry, we demonstrate the measurement of both amplitude and phase of photon echoes in GaAs multiple-quantum-well structures. The complete measurement of the electric field thus achieved makes possible the determination of the corresponding Wigner spectrograms.

Double-lambda microscopic model for entangled light generation by four-wave-mixing

Motivated by recent experiments, we study four-wave-mixing in an atomic double-{Lambda} system driven by a far-detuned pump. Using the Heisenberg-Langevin formalism, and based on the microscopic properties of the medium, we calculate the classical and quantum properties of seed and conjugate beams beyond the linear amplifier approximation. A continuous-variable approach gives us access to relative-intensity noise spectra that can be directly compared with experiments. Restricting ourselves to the cold-atom regime, we predict the generation of quantum-correlated beams with a relative-intensity noise spectrum well below the standard quantum limit (down to -6 dB). Moreover, entanglement between seed and conjugate beams measured by an inseparability down to 0.25 is expected. This work opens the way to the generation of entangled beams by four-wave mixing in a cold-atom sample.

Coherent broadband pulse shaping in the mid infrared

We demonstrate broadband infrared pulse shaping by difference-frequency mixing of two visible phase-locked linearly chirped pulses in GaAs. Control of the temporal profile of the emitted field is achieved through this direct tailoring of the exciting visible intensity. The results are in agreement with a simulation with no adjustable parameter.

Conversion of high-power 15-fs visible pulses to the mid infrared

We measure the efficiency of converting high-power 15-fs 0.8-mum pulses to the mid infrared in GaAs and GaSe as well as the pulse duration and the spectrum of the infrared radiation that is produced. Free-carrier production limits the conversion efficiency in GaAs to approximately 5x10(-7) , allowing us to produce 2.5-pJ, 30-fs pulses spanning the spectral range from 6 to 14 mum . In GaSe we obtain, in a moderately saturated regime, a conversion efficiency of 7.5x10(-5) , limited by two-photon absorption, allowing us to produce pulses of 100-fs duration containing 10 nJ of energy.

Amplitude and phase measurements of femtosecond pulses shaped by use of spectral hole burning in free-base naphthalocyanine-doped films

We performed pulse-shaping and time-reversal experiments using spectral holography based on persistent spectral hole burning in free-base naphthalocyanine-doped films. We demonstrate that we can control the pulses diffracted from the hologram by shaping and then by characterizing these pulses in both amplitude and phase. A dephasing time of 29 ps (i.e., a homogeneous linewidth of 69 GHz) was measured from a photon-echo experiment in the chemically accumulated regime.

Generation and complete characterization of intense mid-infrared ultrashort pulses

Intense mid-infrared pulses tunable between 5 and 14 µm with pulse energies of several microjoules were generated by difference-frequency mixing (DFM) in a GaSe crystal. Longer wavelengths (up to 18 µm) were achieved by DFM in a CdSe crystal. The infrared pulses were then characterized using various techniques: The spectrum was measured using a Fourier-transform spectrometer, which was then modified to determine the interferometric second-order autocorrelation. The electric field spectral phase was measured using the same setup, thus leading to a full characterization of the mid-infrared pulses. The spectral phase was measured using the time-domain homodyne optical technique for spectral phase interferometry for direct electric field reconstruction, where spectral interferometry was replaced with time-domain interferometry. The measured pulse duration was 100 fs, nearly transform limited.

Trapping and cooling of Sr+ ions: strings and large clouds

This paper reports on trapping and laser cooling of singly ionized strontium ions in a linear Paul trap. We describe the loading technique based on two-photon absorption of femtosecond pulses at a wavelength of 431 nm and we compare this technique to electron-bombardment ionization. We perform Doppler cooling of the ions in the few-ions regime as well as in the case of large clouds. The analysis of the fluorescence spectra and direct imaging of the cloud allows us to identify the Coulomb-crystal regime. These experiments open the way to the use of a large cold trapped-ion cloud as a medium for quantum optics and quantum information experiments.

Broadband ultrafast spectroscopy using a photonic crystal fiber: application to the photophysics of malachite green

Femtosecond single-pulsed supercontinua (SC) are produced in a short sub-cm piece of photonic crystal fiber. The SC span from 450 nm to more than 1.1 mum with 1-nJ energy injection. UV light down to 340 nm is observed with increased injection power. Using such a single-pulsed SC we implemented a compact transient absorption spectrometer with broadband detection and 150-fs FWHM time resolution to monitor the ultrafast dynamics of the electronic states of malachite green in ethanol excited to the S(2) state. The full spectral evolution is observed from 450 nm to 1050 nm, with high sensitivity and a signal-to-noise ratio as high as 1000.

Large two dimensional Coulomb crystals in a radio frequency surface ion trap

We designed and operated a surface ion trap with an ion-substrate distance of 500 μm, realized with standard printed-circuit-board techniques. The trap has been loaded with up to a few thousand Sr+ ions in the Coulomb-crystal regime. An analytical model of the pseudo-potential allowed us to determine the parameters that drive the trap into anisotropic regimes in which we obtain large (N>150) purely two dimensional (2D) ion Coulomb crystals. These crystals may open a simple and reliable way to experiments on quantum simulations of large 2D systems.

Excitonic dynamics in CdTe/ZnTe quantum dots

Abstract We study the dephasing and population dynamics of excitons at low temperature, in self-organized CdTe/ZnTe islands grown by atomic layer epitaxy. Using a pump–probe technique, we probe the relaxation dynamics of the electron-hole population after an excitation of the ZnTe barriers. After a fast transfer (