Jonathan Keeling

Bose-Einstein condensation of exciton polaritons

Phase transitions to quantum condensed phases—such as Bose–Einstein condensation (BEC), superfluidity, and superconductivity—have long fascinated scientists, as they bring pure quantum effects to a macroscopic scale. BEC has, for example, famously been demonstrated in dilute atom gas of rubidium atoms at temperatures below 200 nanokelvin. Much effort has been devoted to finding a solid-state system in which BEC can take place. Promising candidate systems are semiconductor microcavities, in which photons are confined and strongly coupled to electronic excitations, leading to the creation of exciton polaritons. These bosonic quasi-particles are 109 times lighter than rubidium atoms, thus theoretically permitting BEC to occur at standard cryogenic temperatures. Here we detail a comprehensive set of experiments giving compelling evidence for BEC of polaritons. Above a critical density, we observe massive occupation of the ground state developing from a polariton gas at thermal equilibrium at 19 K, an increase of temporal coherence, and the build-up of long-range spatial coherence and linear polarization, all of which indicate the spontaneous onset of a macroscopic quantum phase.

Spontaneous Rotating Vortex Lattices in a Pumped Decaying Condensate

Injection and decay of particles in an inhomogeneous quantum condensate can significantly change its behavior. We model trapped, pumped, decaying condensates by a complex Gross-Pitaevskii equation and analyze the density and currents in the steady state. With homogeneous pumping, rotationally symmetric solutions are unstable. Stability may be restored by a finite pumping spot. However if the pumping spot is larger than the Thomas-Fermi cloud radius, then rotationally symmetric solutions are replaced by solutions with spontaneous arrays of vortices. These vortex arrays arise without any rotation of the trap, spontaneously breaking rotational symmetry.

Nonequilibrium Quantum Condensation in an Incoherently Pumped Dissipative System

We study spontaneous quantum coherence in an out of an equilibrium system, coupled to multiple baths describing pumping and decay. For a range of parameters describing coupling to, and occupation of the baths, a stable steady-state condensed solution exists. The presence of pumping and decay significantly modifies the spectra of phase fluctuations, leading to correlation functions that differ both from an isolated condensate and from a laser.

Minimal Excitation States of Electrons in One-Dimensional Wires

A strategy is proposed to excite particles from a Fermi sea in a noise-free fashion by electromagnetic pulses with realistic parameters. We show that by using quantized pulses of simple form one can suppress the particle-hole pairs which are created by a generic excitation. The resulting many-body states are characterized by one or several particles excited above the Fermi surface accompanied by no disturbance below it. These excitations carry charge which is integer for noninteracting electron gas and fractional for Luttinger liquid. The operator algebra describing these excitations is derived, and a method of their detection which relies on noise measurement is proposed.

Collective coherence in planar semiconductor microcavities

Semiconductor microcavities, in which strong coupling of excitons to confined photon modes leads to the formation of exciton?polariton modes, have increasingly become a focus for the study of spontaneous coherence, lasing and condensation in solid state systems. This review discusses the significant experimental progress to date, the phenomena associated with coherence which have been observed and also discusses in some detail the different theoretical models that have been used to study such systems. We consider both the case of non-resonant pumping, in which coherence may spontaneously arise, and the related topics of resonant pumping, and the optical parametric oscillator.

Collective Dynamics of Bose-Einstein Condensates in Optical Cavities

Experiments on Bose-Einstein condensates in optical cavities have observed a coherent state of the matter-light system-superradiance. The nature of these experiments demands consideration of collective dynamics. Including cavity leakage and the backreaction of the cavity field on the condensate, we find a rich phase diagram including multiphase coexistence regions, and persistent optomechanical oscillations. The proximity of the phase boundaries results in a critical slowing down of the decay of many-body oscillations, which can be enhanced by large cavity loss.

Dynamics of nonequilibrium Dicke models

Motivated by experiments observing self-organization of cold atoms in optical cavities, we investigate the collective dynamics of the associated nonequilibrium Dicke model. The model displays a rich semiclassical phase diagram of long-time attractors including distinct superradiant fixed points, bistable and multistable coexistence phases, and regimes of persistent oscillations. We explore the intrinsic time scales for reaching these asymptotic states and discuss the implications for finite-duration experiments. On the basis of a semiclassical analysis of the effective Dicke model, we find that sweep measurements over 200 ms may be required in order to access the asymptotic regime. We briefly comment on the corrections that may arise due to quantum fluctuations and states outside of the effective two-level Dicke model description.

Nonequilibrium model of photon condensation.

We develop a nonequilibrium model of condensation and lasing of photons in a dye filled microcavity. We examine in detail the nature of the thermalization process induced by absorption and emission of photons by the dye molecules, and investigate when the photons are able to reach a thermal equilibrium Bose-Einstein distribution. At low temperatures, or large cavity losses, the absorption and emission rates are too small to allow the photons to reach thermal equilibrium and the behavior becomes more like that of a conventional laser.

Nonequilibrium Dynamics of Coupled Qubit-Cavity Arrays

We study the coherence and fluorescence properties of the coherently pumped and dissipative Jaynes-Cummings-Hubbard model describing polaritons in a coupled-cavity array. At weak hopping we find strong signatures of photon blockade similar to single-cavity systems. At strong hopping the state of the photons in the array depends on its size. While the photon blockade persists in a dimer consisting of two coupled cavities, a coherent state forms on an extended lattice, which can be described in terms of a semiclassical model.

Power-law decay of the spatial correlation function in exciton-polariton condensates

We create a large exciton-polariton condensate and employ a Michelson interferometer setup to characterize the short- and long-distance behavior of the first order spatial correlation function. Our experimental results show distinct features of both the two-dimensional and nonequilibrium characters of the condensate. We find that the gaussian short-distance decay is followed by a power-law decay at longer distances, as expected for a two-dimensional condensate. The exponent of the power law is measured in the range 0.9–1.2, larger than is possible in equilibrium. We compare the experimental results to a theoretical model to understand the features required to observe a power law and to clarify the influence of external noise on spatial coherence in nonequilibrium phase transitions. Our results indicate that Berezinskii–Kosterlitz–Thouless-like phase order survives in open-dissipative systems.