M. H. Szymanska

Bose-Einstein condensation of exciton polaritons

Phase transitions to quantum condensed phases—such as Bose–Einstein condensation (BEC), superfluidity, and superconductivity—have long fascinated scientists, as they bring pure quantum effects to a macroscopic scale. BEC has, for example, famously been demonstrated in dilute atom gas of rubidium atoms at temperatures below 200 nanokelvin. Much effort has been devoted to finding a solid-state system in which BEC can take place. Promising candidate systems are semiconductor microcavities, in which photons are confined and strongly coupled to electronic excitations, leading to the creation of exciton polaritons. These bosonic quasi-particles are 109 times lighter than rubidium atoms, thus theoretically permitting BEC to occur at standard cryogenic temperatures. Here we detail a comprehensive set of experiments giving compelling evidence for BEC of polaritons. Above a critical density, we observe massive occupation of the ground state developing from a polariton gas at thermal equilibrium at 19 K, an increase of temporal coherence, and the build-up of long-range spatial coherence and linear polarization, all of which indicate the spontaneous onset of a macroscopic quantum phase.

Nonequilibrium Quantum Condensation in an Incoherently Pumped Dissipative System

We study spontaneous quantum coherence in an out of an equilibrium system, coupled to multiple baths describing pumping and decay. For a range of parameters describing coupling to, and occupation of the baths, a stable steady-state condensed solution exists. The presence of pumping and decay significantly modifies the spectra of phase fluctuations, leading to correlation functions that differ both from an isolated condensate and from a laser.

Collective coherence in planar semiconductor microcavities

Semiconductor microcavities, in which strong coupling of excitons to confined photon modes leads to the formation of exciton?polariton modes, have increasingly become a focus for the study of spontaneous coherence, lasing and condensation in solid state systems. This review discusses the significant experimental progress to date, the phenomena associated with coherence which have been observed and also discusses in some detail the different theoretical models that have been used to study such systems. We consider both the case of non-resonant pumping, in which coherence may spontaneously arise, and the related topics of resonant pumping, and the optical parametric oscillator.

Power-law decay of the spatial correlation function in exciton-polariton condensates

We create a large exciton-polariton condensate and employ a Michelson interferometer setup to characterize the short- and long-distance behavior of the first order spatial correlation function. Our experimental results show distinct features of both the two-dimensional and nonequilibrium characters of the condensate. We find that the gaussian short-distance decay is followed by a power-law decay at longer distances, as expected for a two-dimensional condensate. The exponent of the power law is measured in the range 0.9–1.2, larger than is possible in equilibrium. We compare the experimental results to a theoretical model to understand the features required to observe a power law and to clarify the influence of external noise on spatial coherence in nonequilibrium phase transitions. Our results indicate that Berezinskii–Kosterlitz–Thouless-like phase order survives in open-dissipative systems.

Polariton condensation with localized excitons and propagating photons.

We estimate the condensation temperature for microcavity polaritons, allowing for their internal structure. We consider polaritons formed from localized excitons in a planar microcavity, using a generalized Dicke model. At low densities, we find a condensation temperature T(c) proportional, rho, as expected for a gas of structureless polaritons. However, as T(c) becomes of the order of the Rabi splitting, the structure of the polaritons becomes relevant, and the condensation temperature is that of a BCS-like mean-field theory. We also calculate the excitation spectrum, which is related to observable quantities such as the luminescence and absorption spectra.

BCS-BEC crossover in a system of microcavity polaritons

We investigate the thermodynamics and signatures of a polariton condensate over a range of densities, using a model of microcavity polaritons with internal structure. We determine a phase diagram for this system including fluctuation corrections to the mean-field theory. At low densities the condensation temperature T{sub c} behaves like that for point bosons. At higher densities, when T{sub c} approaches the Rabi splitting, T{sub c} deviates from the form for point bosons, and instead approaches the result of a BCS-like mean-field theory. This crossover occurs at densities much less than the Mott density. We show that current experiments are in a density range where the phase boundary is described by the BCS-like mean-field boundary. We investigate the influence of inhomogeneous broadening and detuning of excitons on the phase diagram.

Excitons in T-shaped quantum wires

We calculate energies, oscillator strengths for radiative recombination, and two-particle wave functions for the ground-state exciton and around 100 excited states in a T-shaped quantum wire. We include the single-particle potential and the Coulomb interaction between the electron and hole on an equal footing, and perform exact diagonalization of the two-particle problem within a finite-basis set. We calculate spectra for all of the experimentally studied cases of T-shaped wires including symmetric and asymmetric

Models of coherent exciton condensation

{\mathrm{G}\mathrm{a}\mathrm{A}\mathrm{s}/\mathrm{A}\mathrm{l}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}

Conventional character of the BCS-BEC crossover in ultracold gases of {sup 40}K

and

Mean-field theory and fluctuation spectrum of a pumped decaying Bose-Fermi system across the quantum condensation transition

{\mathrm{In}}_{y}{\mathrm{Ga}}_{1\ensuremath{-}y}{\mathrm{A}\mathrm{s}/\mathrm{A}\mathrm{l}}_{x}{\mathrm{Ga}}_{1\ensuremath{-}x}\mathrm{As}