Kazufumi Tsujimoto

Neutronics Design of Accelerator-Driven System for Power Flattening and Beam Current Reduction

In the present neutronics design of the Accelerator-Driven System (ADS) cooled by lead-bismuth eu-tectic (LBE), we investigated several methods to reduce the power peak and beam current, and estimated the temperature reductions of the cladding tube and beam window from the conventional design. The methods are adjustment of inert matrix ratio in fuel in each burn-up cycle, multiregion design in terms of pin radius or inert matrix content, and modification of the level of the beam window position and the height of the central fuel assemblies. As a result, we optimized the ADS combined with the adjustment of the inert matrix ratio in each burn-up cycle, multiregion design in terms of inert matrix content and deepened window level. The maximum temperatures of the optimized ADS at the surface of the cladding tube and the beam window were reduced by 91 and 38°C, respectively. The maximum beam current was improved from 20.3 to 15.6 mA.

Research and Development Program on Accelerator Driven Subcritical System in JAEA

For a dedicated transmutation system, Japan Atomic Energy Agency (JAEA) has been proceeding with the research and development on an accelerator-driven subcritical system (ADS). The ADS proposed by JAEA is a lead-bismuth eutectic (LBE) cooled fast subcritical core with 800 MWth. JAEA has started a comprehensive research and development (R&D) program since the fiscal year of 2002 to acquire knowledge and elemental technology that are necessary for the validation of engineering feasibility of the ADS. In this paper, the outline and the results in the first three-year stage of the program are reported. Items of R&D were concentrated on three technical areas peculiar to the ADS: (1) a superconducting linear accelerator (SC-LINAC), (2) the LBE as spallation target and core coolant, and (3) a subcritical core design and reactor physics of the ADS. For R&D on the accelerator, a prototype cryomodule was built and its good performance in electric field was examined. For R&D on the LBE, various technical data for material corrosion, thermal-hydraulics and radioactive impurity were obtained by loop tests and reactor irradiation. For R&D on the subcritical core, engineering feasibility for the LBE cooled tank-type ADS was discussed using thermal-hydraulic and structural analysis not only in normal operation but also in transient situations. Reactor physics experiments for subcritical monitoring and physics parameters of the ADS were also performed at critical assemblies.

Sensitivity and uncertainty analysis for an accelerator-driven system with JENDL-4.0

A sensitivity and uncertainty analysis was performed for the accelerator-driven system (ADS) proposed by the Japan Atomic Energy Agency (JAEA) with the latest version of the Japanese Evaluated Nuclear Data Library (JENDL-4.0). Significant discrepancies have been found between the reactor physics parameters of JENDL-4.0 and those of JENDL-3.3. An analysis with the sensitivity coefficients showed that the major contributors to these discrepancies are the differences in the inelastic scattering cross sections of 206Pb and 207Pb, and the capture and inelastic scattering cross sections and ν value of 241Am. The uncertainty analysis with the JENDL-4.0 covariance data found that the covariances of the fission neutron spectrum of minor actinides (MAs) have a considerable impact on the uncertainties of the reactor physics parameters.

Analytical Validation of Uncertainty in Reactor Physics Parameters for Nuclear Transmutation Systems

To confirm the reliability of calculated reactor physics parameters for the nuclear transmutation systems, the uncertainty deduced from the covariance data prepared in JENDL-3.3 is compared with the differences in the reactor physicsparameters in the Monte-Carlo calculation using different nuclear data libraries, ENDF/B-VII.0 and JEFF-3.1.1. The Accelerator-Driven System (ADS) and the Minor Actinide (MA)-loaded Fast Reactor (FR) are selected as the representative transmutation systems. The criticality and void reactivity of these systems are discussed. The results show that the uncertainties deduced from the JENDL-3.3 covariance data are smaller than the differences in the reactor physics parameters among the nuclear data libraries. The cause of this discrepancy is that the covariance data of main nuclides and reactions in JENDL-3.3 are smaller than the relative differences in the cross sections among the nuclear data libraries. It is required to verify the uncertainty of the reactor physics parameters by integral experiments and to discuss the uncertainty utilization for the nuclear design accuracy.

Validation of Pb nuclear data by Monte Carlo analyses of sample reactivity experiments at Kyoto University Critical Assembly

Sample reactivity experiments on the uncertainty analyses of Pb nuclear data are carried out by substituting Al plates for Pb ones at the Kyoto University Critical Assembly, as part of basic research on Pb–Bi for the coolant. Numerical simulations of sample reactivity experiments are performed with the Monte Carlo calculation code MCNP6.1 together with four nuclear data libraries JENDL-3.3, JENDL-4.0, ENDF/B-VII.0 and JEFF-3.1, to examine the accuracy of cross-section uncertainties of Pb isotopes by comparing measured and calculated sample reactivities. A library update from JENDL-3.3 to JENDL-4.0 is demonstrated by the fact that the difference between Pb isotopes of the two JENDL libraries is dominant in the comparative study, through the experimental analyses of sample reactivity by the MCNP approach. In addition, JENDL-4.0 reveals a slight difference from ENDF/B-VII.0 in all Pb isotopes and 27Al, and from JEFF-3.1 in 238U and 27Al. Based on these results, further experiments are needed to investigate the uncertainties of Bi isotopes with the use of the Pb–Bi and Bi plates.

Development of three-dimensional reactor analysis code system for accelerator-driven system, ADS3D and its application with subcriticality adjustment mechanism

ABSTRACT In order to perform the parametric survey for an accelerator-driven system (ADS) core with the subcriticality adjustment mechanism, a new calculation code system, ADS3D, was developed on MARBLE which is a comprehensive and versatile framework for reactor analysis. The application of ADS3D was also demonstrated on the neutronics design of ADS operated by control rod (CR) movement. Through the neutronics calculation, it was shown that the maximum proton beam current was decreased from 20.5 to 11.6 mA due to the switch from beam-operated to CR-operated core.

Estimation of acceptable beam-trip frequencies of accelerators for accelerator-driven systems and comparison with existing performance data

Frequent beam trips as experienced in the existing high-power proton accelerators may cause thermal fatigue in accelerator-driven system (ADS) components, which may lead to degradation of their structural integrity and reduction of their lifetime. In this study, acceptable beam-trip frequencies of the ADS accelerator were evaluated and compared with the performance of the ADS accelerator, which was estimated based on the operational data on existing accelerators. Thermal transient analyses were performed to investigate the effects of beam trips on the reactor components, with the objective of determining the feasibility of engineering the ADS and the reliability of the accelerator. These analyses were based on the thermal responses of the following reactor components: the beam window, the fuel cladding, the inner barrel and the reactor vessel. Assuming that the annual plant availability was 70%, our results indicated three acceptable beam-trip frequencies, depending on the beam-trip duration, τ b : 2 × 104 times per year for 0 10 s; 2 × 103 times per year for 10 s 5 min; and 42 times per year for τ b > 5 min. In order to consider methods to reduce beam-trip frequency, we compared the acceptable beam-trip frequency with the performance of the ADS accelerator, which was estimated based on the operational data on existing accelerators. The comparison showed that for beam trips with a duration of 10 s or less, the beam-trip frequency was acceptable. On the other hand, for beam trips with durations of 10 s 5 min and τ b > 5 min, it was necessary to reduce the beam-trip frequencies to about 1/6 and 1/35, respectively.

Sensitivity and Uncertainty Analyses of Lead Sample Reactivity Experiments at Kyoto University Critical Assembly

Abstract Sensitivity and uncertainty analyses of lead (Pb) isotope cross sections are conducted with the use of sample reactivity experiments at the Kyoto University Critical Assembly (KUCA). With the combined use of the SRAC2006 and MARBLE code systems, attempts are made to precisely examine the contributions of the reactions and energy regions of Pb isotope cross sections to reactivity based on the covariance data of JENDL-4.0. Moreover, the effect of decreasing uncertainty is discussed in terms of the accuracy of sample reactivity by applying the cross-section adjustment method to the uncertainty analyses. From the results of the sensitivity and uncertainty analyses, the reliability of Pb isotope cross sections, such as the Pb isotope covariance data of JENDL-4.0, is compared with the JENDL-3.3, ENDF/B-VII.0, and JEFF-3.1 libraries. Additionally, the numerical results reveal the applicability of the sensitivity and uncertainty analyses to the thermal neutron spectrum cores, such as the KUCA core, and demonstrate the improvement in the calculation results generated by the cross-section adjustment.

Measurement of Activation Reaction Rate Distributions in a Lead Assembly Bombarded with 500-MeV Protons

Abstract Reaction rate distributions of various activation detectors such as the natNi(n,x)58Co, 197Au(n,2n)196Au, and 197Au(n,4n)194Au reactions were measured to study the production and the transport of spallation neutrons in a lead assembly bombarded with protons of 500 MeV. The measured data were analyzed with the nucleon-meson transport code NMTC/JAERI combined with the MCNP4A code using the nuclide production cross sections based on the JENDL Dosimetry File and those calculated with the ALICE-F code. It was found that the NMTC/JAERI-MCNP4A calculations agreed well with the experiments for the low-energy-threshold reaction of natNi(n,x)58Co. With the increase of threshold energy, however, the calculation underestimated the experiments, especially above 20 MeV. The reason for the disagreement can be attributed to the underestimation of the neutron yield in the tens of mega-electron-volt regions by the NMTC/JAERI code.

Lead Void Reactivity Worth in Two Critical Assembly Cores with Differing Uranium Enrichments

Abstract To validate lead (Pb) nuclear cross sections, a series of integral experiments to measure lead void reactivity worths was conducted in a high-enriched uranium (HEU)/Pb system and a low-enriched uranium (LEU)/Pb system using the Comet Critical Assembly at the National Criticality Experiments Research Center. There is a follow-on experiment to measure the lead void reactivity worths in a plutonium/Pb system that is currently under investigation. The critical experiments in the two uranium systems were designed to provide complementary data sets having different sensitivities to scattering cross sections of lead. The larger amount of the 238U present in the LEU/Pb core increases the neutron importance above 1 MeV compared with the HEU/Pb core. Since removal of lead from the core shifts the neutron spectrum to the higher energy region, positive lead void reactivity worths were observed in the LEU/Pb core while negative values were observed in the HEU/Pb core. This technical note is a preliminarily report of the experimental analysis results for the lead void reactivity worths with the Monte Carlo calculation code MCNP® version 6.1 together with nuclear data libraries JENDL-4.0 and ENDF/B-VII.1. The calculation values were found to overestimate the negative reactivity worths for the HEU/Pb core while being consistent for the LEU/Pb core.