Kenji Nishihara

Neutronics Design of Accelerator-Driven System for Power Flattening and Beam Current Reduction

In the present neutronics design of the Accelerator-Driven System (ADS) cooled by lead-bismuth eu-tectic (LBE), we investigated several methods to reduce the power peak and beam current, and estimated the temperature reductions of the cladding tube and beam window from the conventional design. The methods are adjustment of inert matrix ratio in fuel in each burn-up cycle, multiregion design in terms of pin radius or inert matrix content, and modification of the level of the beam window position and the height of the central fuel assemblies. As a result, we optimized the ADS combined with the adjustment of the inert matrix ratio in each burn-up cycle, multiregion design in terms of inert matrix content and deepened window level. The maximum temperatures of the optimized ADS at the surface of the cladding tube and the beam window were reduced by 91 and 38°C, respectively. The maximum beam current was improved from 20.3 to 15.6 mA.

Research and Development Program on Accelerator Driven Subcritical System in JAEA

For a dedicated transmutation system, Japan Atomic Energy Agency (JAEA) has been proceeding with the research and development on an accelerator-driven subcritical system (ADS). The ADS proposed by JAEA is a lead-bismuth eutectic (LBE) cooled fast subcritical core with 800 MWth. JAEA has started a comprehensive research and development (R&D) program since the fiscal year of 2002 to acquire knowledge and elemental technology that are necessary for the validation of engineering feasibility of the ADS. In this paper, the outline and the results in the first three-year stage of the program are reported. Items of R&D were concentrated on three technical areas peculiar to the ADS: (1) a superconducting linear accelerator (SC-LINAC), (2) the LBE as spallation target and core coolant, and (3) a subcritical core design and reactor physics of the ADS. For R&D on the accelerator, a prototype cryomodule was built and its good performance in electric field was examined. For R&D on the LBE, various technical data for material corrosion, thermal-hydraulics and radioactive impurity were obtained by loop tests and reactor irradiation. For R&D on the subcritical core, engineering feasibility for the LBE cooled tank-type ADS was discussed using thermal-hydraulic and structural analysis not only in normal operation but also in transient situations. Reactor physics experiments for subcritical monitoring and physics parameters of the ADS were also performed at critical assemblies.

Impact of Partitioning and Transmutation on LWR High-Level Waste Disposal

Partitioning and/or transmutation (PT) technology affects the disposal concept of high-level radioactive waste (HLW). We studied how cooling in the predisposal storage period may affect the design of the emplacement area in a repository for radioactive wastes produced by a light-water-reactor nuclear system that uses PT technology. Three different fuel cycle scenarios involving PT technology were analyzed: 1) partitioning process only (separation of some fission products), 2) transmutation process only (separation and transmutation of minor actinides), and 3) both partitioning and transmutation. The necessary predisposal storage periods for some predefined emplacement configurations were determined through transient thermal analysis, and the relation between the storage period and the emplacement area was obtained. For each scenario, we also estimated the storage capacity required for the dry storage of the heat-generating waste forms. The contributions of PT technology on the storage and disposal were discussed holistically, and we noted that the coupled introduction of partitioning and transmutation processes can bring an appreciable reduction in waste management size.

Radionuclide release to stagnant water in the Fukushima-1 nuclear power plant1

After the severe accident at the Fukushima-1 nuclear power plant, large amounts of contaminated stagnant water have accumulated in turbine buildings and their surroundings. This rapid communication reports calculation of the radionuclide inventory in the core, collection of measured inventory in the stagnant water, and estimation of radionuclide release ratios from the core to the stagnant water. This evaluation is based on data obtained before 3 June 2011. The release ratios of tritium, iodine, and cesium were several tens of percent, whereas those of strontium and barium were smaller by one or two orders of magnitude. The release ratios in the Fukushima accident were equivalent to those in the accident of the Three Mile Island, Unit 2 (TMI-2).

Sensitivity and uncertainty analysis for an accelerator-driven system with JENDL-4.0

A sensitivity and uncertainty analysis was performed for the accelerator-driven system (ADS) proposed by the Japan Atomic Energy Agency (JAEA) with the latest version of the Japanese Evaluated Nuclear Data Library (JENDL-4.0). Significant discrepancies have been found between the reactor physics parameters of JENDL-4.0 and those of JENDL-3.3. An analysis with the sensitivity coefficients showed that the major contributors to these discrepancies are the differences in the inelastic scattering cross sections of 206Pb and 207Pb, and the capture and inelastic scattering cross sections and ν value of 241Am. The uncertainty analysis with the JENDL-4.0 covariance data found that the covariances of the fission neutron spectrum of minor actinides (MAs) have a considerable impact on the uncertainties of the reactor physics parameters.

Parametric survey for benefit of partitioning and transmutation technology in terms of high-level radioactive waste disposal

Benefit of implementing Partitioning and Transmutation (P&T) technology was parametrically surveyed in terms of high-level radioactive waste (HLW) disposal by discussing possible reduction of the geological repository area. First, the amount and characteristics of HLWs caused from UO2 and MOX spent fuels of light-water reactors (LWR) were evaluated for various reprocessing schemes and cooling periods. The emplacement area in the repository site required for the disposal of these HLWs was then estimated with considering the temperature constrain in the repository. The results showed that, by recycling minor actinides (MA), the emplacement area could be reduced by 17–29% in the case of UO2-LWR and by 63–85% in the case of MOX-LWR in comparison with the conventional PUREX reprocessing. This significant impact in MOX fuel was caused by the recycle of 241Am which was a long-term heat source. Further 70–80% reduction of the emplacement area in comparison with the MA-recovery case could be expected by partitioning the fission products (FP) into several groups for both fuel types. To achieve this benefit of P&T, however, it is necessary to confirm the engineering feasibility of these unconventional disposal concepts.

Impact of Partitioning and Transmutation on High-Level Waste Disposal for the Fast Breeder Reactor Fuel Cycle

The impact of partitioning and/or transmutation (PT) technology on high-level waste management was investigated for the equilibrium state of several potential fast breeder reactor (FBR) fuel cycles. Three different fuel cycle scenarios involving PT technology were analyzed: 1) partitioning process only (separation of some fission products), 2) transmutation process only (separation and transmutation of minor actinides), and 3) both partitioning and transmutation processes. The conventional light water reactor (LWR) fuel cycle without PT technology, on which the current repository design is based, was also included for comparison. We focused on the thermal constraints in a geological repository and determined the necessary predisposal storage quantities and time periods (by defining a storage capacity index) for several predefined emplacement configurations through transient thermal analysis. The relation between this storage capacity index and the required repository emplacement area was obtained. We found that the introduction of the FBR fuel cycle without PT can yield a 35% smaller repository per unit electricity generation than the LWR fuel cycle, although the predisposal storage period is prolonged from 50 years for the LWR fuel cycle to 65 years for the FBR fuel cycle without PT. The introduction of the partitioning-only process does not result in a significant reduction of the repository emplacement area from that for the FBR fuel cycle without PT, but the introduction of the transmutation-only process can reduce the emplacement area by a factor of 5 when the storage period is extended from 65 to 95 years. When a coupled partitioning and transmutation system is introduced, the repository emplacement area can be reduced by up to two orders of magnitude by assuming a predisposal storage of 60 years for glass waste and 295 years for calcined waste containing the Sr and Cs fraction. The storage period of 295 years for the calcined waste does not require a large storage capacity because the number of waste packages produced is significantly reduced by a factor of 5 from that of the glass waste package in the FBR fuel cycle without PT.

Conceptual Design Study of Beam Window for Accelerator-Driven System

The conceptual design study of the beam window of the spallation target is one of the critical issues in the R&D of the accelerator-driven system (ADS). In this study, the investigation to create a feasible concept of the beam window for the ADS was performed by changing the proton beam profile from the Gaussian distribution to the parabolic and the flat distributions. Detailed analyses were performed by considering the particle transport of protons and neutrons in the spallation target region, the thermal hydraulics of lead bismuth eutectic (LBE) around the beam window, and the structural strength of the beam window. The calculation results showed that the difference in the temperature between the inner and outer surfaces at the top of the beam window was reduced by changing the beam profile from the Gaussian to the parabolic and the flat distributions. By this reduction, in the parabolic case, the thermal stress at the top position was also reduced and the buckling pressure increased by about 20%. On the other hand, in the flat case, the thermal stress at the peripheral region instead of at the central position increased and the buckling pressure slightly deteriorated. The buckling mode was also changed in the flat case. From these calculation results and discussions, it was confirmed that all three cases, the Gaussian, the parabolic, and the flat, were feasible and it was concluded that the concept with the parabolic distribution would be the most feasible under the current ADS design condition.

Analytical Validation of Uncertainty in Reactor Physics Parameters for Nuclear Transmutation Systems

To confirm the reliability of calculated reactor physics parameters for the nuclear transmutation systems, the uncertainty deduced from the covariance data prepared in JENDL-3.3 is compared with the differences in the reactor physicsparameters in the Monte-Carlo calculation using different nuclear data libraries, ENDF/B-VII.0 and JEFF-3.1.1. The Accelerator-Driven System (ADS) and the Minor Actinide (MA)-loaded Fast Reactor (FR) are selected as the representative transmutation systems. The criticality and void reactivity of these systems are discussed. The results show that the uncertainties deduced from the JENDL-3.3 covariance data are smaller than the differences in the reactor physics parameters among the nuclear data libraries. The cause of this discrepancy is that the covariance data of main nuclides and reactions in JENDL-3.3 are smaller than the relative differences in the cross sections among the nuclear data libraries. It is required to verify the uncertainty of the reactor physics parameters by integral experiments and to discuss the uncertainty utilization for the nuclear design accuracy.

Validation of Pb nuclear data by Monte Carlo analyses of sample reactivity experiments at Kyoto University Critical Assembly

Sample reactivity experiments on the uncertainty analyses of Pb nuclear data are carried out by substituting Al plates for Pb ones at the Kyoto University Critical Assembly, as part of basic research on Pb–Bi for the coolant. Numerical simulations of sample reactivity experiments are performed with the Monte Carlo calculation code MCNP6.1 together with four nuclear data libraries JENDL-3.3, JENDL-4.0, ENDF/B-VII.0 and JEFF-3.1, to examine the accuracy of cross-section uncertainties of Pb isotopes by comparing measured and calculated sample reactivities. A library update from JENDL-3.3 to JENDL-4.0 is demonstrated by the fact that the difference between Pb isotopes of the two JENDL libraries is dominant in the comparative study, through the experimental analyses of sample reactivity by the MCNP approach. In addition, JENDL-4.0 reveals a slight difference from ENDF/B-VII.0 in all Pb isotopes and 27Al, and from JEFF-3.1 in 238U and 27Al. Based on these results, further experiments are needed to investigate the uncertainties of Bi isotopes with the use of the Pb–Bi and Bi plates.