L. Lamaignère

Polishing-induced contamination of fused silica optics and laser induced damage density at 351 nm

In this paper we study the effect of contamination induced by fabrication process on laser damage density of fused silica polished parts at 351 nm in nanosecond regime. We show, owing to recent developments of our raster scan metrology, that a good correlation exists between damage density and concentration of certain contaminants for the considered parts.

An accurate, repeatable, and well characterized measurement of laser damage density of optical materials.

Known for more than 40 years, laser damage phenomena have not been measured reproducibly up to now. Laser resistance of optical components is decreased by the presence of material defects, the distribution of which can initiate a distribution of damage sites. A raster scan test procedure has been used for several years in order to determine laser damage density of large aperture UV fused silica optics. This procedure was improved in terms of accuracy and repeatability. We describe the equipment, test procedure, and data analysis to perform this damage test of large aperture optics with small beams. The originality of the refined procedure is that a shot to shot correlation is performed between the damage occurrence and the corresponding fluence by recording beam parameters of hundreds of thousands of shots during the test at 10 Hz. We characterize the distribution of damaging defects by the fluence at which they cause damage. Because tests are realized with small Gaussian beams (about 1 mm at 1e), beam overlap and beam shape are two key parameters which have to be taken into account in order to determine damage density. After complete data analysis and treatment, we reached a repeatable metrology of laser damage performance. The measurement is destructive for the sample. However, the consideration of error bars on defect distributions in a series of parts allows us to compare data with other installations. This will permit to look for reproducibility, a necessary condition in order to test theoretical predictions.

The impact of laser damage on the lifetime of optical components in fusion lasers

The purpose of this paper is to gather experimental elements allowing for the prediction of laser damage on full size components installed on high power Nd-glass laser lines. Damage can initiated on material defects, which aren’t known in their nature, but the density of which can be measured. On transmissive optics, depending on the component thickness, and on the intensity distribution at the front surface, rear surface damage can also appear due to self-focusing of hot spots. These two contributions produce damage sites that are prone to grow. The growth rate has been shown to be proportional to the damaged area. The resulting exponential growth is the major limitation to the lifetime of optics. A representation of these phenomena in the plane Intensity/Fluence gives a practical description of the impact of laser damage on the lifetime of optical components. It also enlightens the comparison between different operating conditions.

Parametric study of laser-induced surface damage density measurements: Toward reproducibility

In the range of nanosecond pulse lengths, the mechanisms of surface laser damage to dielectric materials are still unclear. A large amount of experimental and theoretical work has been performed over recent years. In order to test theoretical predictions and compare experimental results, reproducibility is essential whatever the beam parameters and experimental conditions. The rasterscan procedure, previously developed to test large components, is an efficient method that allows measuring extremely low surface damage site density (until 0.01 site/cm2 for large optics). In this paper, we show that by suitable data reduction, error bar calculation, and attention paid to beam analysis, laser-induced surface damage density of fused silica optics can be measured with high accuracy and repeatability in the range of pulse durations from 2 to 16 ns. This procedure provides a straightforward means of comparing the experimental results obtained from several facilities using different lasers.

Parametric study of the growth of damage sites on the rear surface of fused silica windows

The growth of damage sites on the rear surface of fused silica plates was studied as a function of fluence and angle of incidence. At 1053 nm, a 70 J beam, 3 ns in pulselength, was directed to a 5 cm2 zone on a bare fused silica window. Initiation and growth was observed. The growth of previously initiated sites was also studied. Growth is exponential in nature. The experiments allow for the determination of the growth coefficient as a function of fluence. At 355 nm, damage sites were irradiated at various angles of incidence, with a tripled Nd:Yag laser, spatially Gaussian, 2.5 ns in pulselength. By fitting growth with an exponential law, it was determined that the relevant fluence for growth was that taken inside the material.

Influence of longitudinal mode beating on laser-induced damage in fused silica

In our study, the laser-induced damage densities on a fused silica surface produced by multiple longitudinal mode (MLM) pulses are found to be higher than those produced by single longitudinal mode pulses at 1064 nm. This behavior is explained by the enhancement of the three-photon absorption due to the intensity spikes related to longitudinal mode beating. At 355 nm, the absorption is linear and an opposite behavior occurs. It can be explained with the help of a process involving thermomechanics coupled with the fine time structure of MLM pulses, leading to the possible annealing of part of the absorbent defects.

Laser damage phenomena relevant to the design and operation of an ICF laser driver

Laser damage performance of optical components is a defect related material characteristic. Recent advances were made to realize repeatable and accurate measurements of surface density of damage initiation due to pulses of nanosecond duration. This new measurement technique was used to guide the improvement of surface damage resistance. Fractures must be eliminated from surfaces, in order not to suffer a damage growth phenomenon, whose exponential character will endanger the optical component. A dedicated set-up was mounted on ALISě laser. With it, laser damage growth was measured accurately, as well as its dependence on parameters like pulse length and pulse shape. Using data from LIL, a prototype of Laser Megajoule (LMJ), and from a specific set-up, we can estimate the effect of multi wavelength illumination on damage growth. High intensity hot spots due to beam modulations can also cause surface damage. New measurements of self-focusing were obtained. The predictions derived from this laboratory work were cross checked with LIL data. They are also useful to predict damage events during the operation of a large laser facility.

Impact of two CO(2) laser heatings for damage repairing on fused silica surface.

CO(2) laser is an interesting tool to repair defects on silica optics. We studied UV nanosecond laser-induced damage in fused silica after CO(2) laser heating. The localization of damage sites and the laser damage threshold are closely related to stress area in silica induced by heating. By applying a suitable second laser heating, we managed to eliminate the debris issued from redeposited silica and to modify the stress area. As a consequence, a significant increase of laser resistance has been observed. This process offers the possibility to improve damage repairing sufficiently to extend the lifetime of the silica components.

Removal of scratches on fused silica optics by using a CO 2 laser

We investigate the efficiency of local CO₂laser processing of scratches on silica optics in order to enhance the nanosecond UV-laser damage resistance. The surface deformations induced by the process have been measured for different CO₂laser parameters and then the pulse duration and the beam diameter have been chosen accordingly to limit those deformations below 1 µm. From the study of the laser damage resistance as a function of different material modifications we identify a range of optimal radiation parameters allowing a complete elimination of scratches associated with a high threshold of laser damage. Calculation of the temperature of silica using a two-dimensional axi-symmetric code was compared with experiment, supporting an optimization of the laser parameter as a function of the maximal dimensions of scratches that could be removed by this process.

Self-focusing and rear surface damage in a fused silica window at 1064 nm and 355 nm

Rear surface damage is known to occur preferentially to front surface damage on silica lenses and windows transmitting 1ω or 3ω light of a Nd:Yag or Nd:glass laser. Lab-scale Experiments were performed to assess the contribution of self-focusing to the measurement of damage statistics. The occurrence of filamentation in the bulk and the statistics of rear surface damage were studied at 1064 nm and 355 nm, for a pulse length around 3 ns. The measurements were performed on synthetic fused silica samples, 4 to 5 cm thick. The laser beam had dimensions around 0.6 mm at the sample. The results are interpreted with the help of the calculations made by J. H. Marburger et al. They are also compared with other experimental results.