M. E. Foord

Ultraviolet surprise: Efficient soft x-ray high-harmonic generation in multiply ionized plasmas.

Short wavelengths birth shorter ones The shortest laser pulses—with durations measured in attoseconds—arise from a process termed high-harmonic generation (HHG). Essentially, a longer, “driving” pulse draws electrons out of gaseous atoms like a slingshot, and, when they ricochet back, light emerges at shorter wavelengths. Most HHG has been carried out using light near the visible/infrared boundary for the driving pulse. Popmintchev et al. used an ultraviolet driving pulse instead, which yielded an unexpectedly efficient outcome. These results could presage a more generally efficient means of creating x-ray pulses for fundamental dynamics studies as well as technological applications. Science, this issue p. 1225 Ultraviolet pulses show unexpected efficiency in generating the higher-frequency emission underlying attosecond spectroscopy. High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Because of reduced quantum diffusion of the radiating electron wave function, the emission from each species is highest when a short-wavelength ultraviolet driving laser is used. However, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams in the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.

Radiation science using Z-pinch x rays

Present-day Z-pinch experiments generate 200 TW peak power, 5–10 ns duration x-ray bursts that provide new possibilities to advance radiation science. The experiments support both the underlying atomic and plasma physics, as well as inertial confinement fusion and astrophysics applications. A typical configuration consists of a sample located 1–10 cm away from the pinch, where it is heated to 10–100 eV temperatures by the pinch radiation. The spectrally-resolved sample-plasma absorption is measured by aiming x-ray spectrographs through the sample at the pinch. The pinch plasma thus both heats the sample and serves as a backlighter. Opacity measurements with this source are promising because of the large sample size, the relatively long radiation duration, and the possibility to measure opacities at temperatures above 100 eV. Initial opacity experiments are under way with CH-tamped NaBr foil samples. The Na serves as a thermometer and absorption spectra are recorded to determine the opacity of Br with a pa...

Neon Photoionization Experiments Driven By Z-Pinch Radiation

Abstract Present-day Z-pinch experiments generate ∼2×10 21 erg / s peak power, ∼6 ns full-width at half-maximum X-ray bursts that provide new possibilities to study radiation-heated matter. This source is being used to investigate the production of plasmas in which photoionization dominates collisional ionization. Spectroscopic measurements of such plasmas can serve to benchmark atomic physics models of the photoionized plasmas. Beyond intrinsic interest in the atomic physics, these models will be applied to the interpretation of data from the new generation of satellite X-ray spectrographs that will promote the understanding of accretion-powered objects such as X-ray binaries and active galactic nuclei. Moreover, this information is needed for X-ray laser research. Our experiments use a 1-cm-scale neon gas cell to expose 10 18 atoms / cm 3 to an X-ray flux of ∼5×10 18 erg / cm 2 / s . Thin mylar ( 1.5 μm ) windows confine the gas and allow the radiation to flow into the cell. The ionization is monitored with absorption spectra recorded with crystal spectrometers, using the pinch as a backlight source. In initial experiments we acquired an absorption spectrum from Li- and He-like Ne, confirming the ability to produce a highly ionized neon plasma.

Accurate determination of the charge state distribution in a well characterized highly ionized Au plasma

Abstract The density, temperature and charge state distribution are accurately determined in a highly ionized non-LTE Au sample. Laser heated Au microdots buried in a thin Be foil, reach temperatures of 2 keV and ionize into the M-shell. During expansion, the tamped Au samples remain uniform and in near steady-state ionization equilibrium. The electron temperature is measured with time and space resolved Thomson scattering while the density is determined from time-gated X-ray imaging the expanded Au sample. The charge state distribution is obtained from analysis of emission measurements of Au 5f–3d transition arrays in the wavelength range 3.3–3.9 A, allowing the average charge to be determined to within ∼1% accuracy.

Calculation of photoionized plasmas with an average-atom model

We use a simple average-atom model (NIMP) to calculate the distribution of ionization in a photoionization-dominated plasma, for comparison with recent experimental measurements undertaken on the Z-machine at the Sandia National Laboratory. The agreement between theory and experiment is found to be as good for calculations with an average-atom model as for those generated by more detailed models.

Plasma diagnostics for x-ray driven foils at Z

We report the development of techniques to diagnose plasmas produced by x-ray photoionization of thin foils placed near the Z-pinch on the Sandia Z Machine. The development of 100+ TW x-ray sources enables access to novel plasma regimes, such as the photoionization equilibrium. To diagnose these plasmas one must simultaneously characterize both the foil and the driving pinch. The desired photoionized plasma equilibrium is only reached transiently for a 2-ns window, placing stringent requirements on diagnostic synchronization. We have adapted existing Sandia diagnostics and fielded an additional gated three-crystal Johann spectrometer with dual lines of sight to meet these requirements. We present sample data from experiments using 1-cm, 180-eV tungsten pinches to photoionize foils made of 200 A Fe and 300 A NaF co-mixed and sandwiched between 1000 A layers of Lexan (C16H14O3), and discuss the application of this work to benchmarking astrophysical models.

Relativistic allowed and forbidden transition probabilities for fluorine-like Fe XVIII

Energy levels and the corresponding transition probabilities for allowed and forbidden transitions among the levels of the ground configuration and first 23 excited configurations of fluorine-like Fe  have been calculated using the mul- ticonfigurational Dirac-Fock  code. A total of 379 lowest bound levels of Fe  is presented, and the energy levels are identified in spectroscopic notations. Transition probabilities, oscillator strengths and line strengths for electric dipole (E1), electric quadrupole (E2) and magnetic dipole (M1) transitions among these 379 levels are also presented. The calculated energy levels and transition probabilities are compared with experimental data.

Observation and control of shock waves in individual nanoplasmas.

Using an apparatus that images the momentum distribution of individual, isolated 100-nm-scale plasmas, we make the first experimental observation of shock waves in nanoplasmas. We demonstrate that the introduction of a heating pulse prior to the main laser pulse increases the intensity of the shock wave, producing a strong burst of quasimonoenergetic ions with an energy spread of less than 15%. Numerical hydrodynamic calculations confirm the appearance of accelerating shock waves and provide a mechanism for the generation and control of these shock waves. This observation of distinct shock waves in dense plasmas enables the control, study, and exploitation of nanoscale shock phenomena with tabletop-scale lasers.

Mapping Nanoscale Absorption of Femtosecond Laser Pulses Using Plasma Explosion Imaging

We make direct observations of localized light absorption in a single nanostructure irradiated by a strong femtosecond laser field, by developing and applying a technique that we refer to as plasma explosion imaging. By imaging the photoion momentum distribution resulting from plasma formation in a laser-irradiated nanostructure, we map the spatial location of the highly localized plasma and thereby image the nanoscale light absorption. Our method probes individual, isolated nanoparticles in vacuum, which allows us to observe how small variations in the composition, shape, and orientation of the nanostructures lead to vastly different light absorption. Here, we study four different nanoparticle samples with overall dimensions of ∼100 nm and find that each sample exhibits distinct light absorption mechanisms despite their similar size. Specifically, we observe subwavelength focusing in single NaCl crystals, symmetric absorption in TiO2 aggregates, surface enhancement in dielectric particles containing a single gold nanoparticle, and interparticle hot spots in dielectric particles containing multiple smaller gold nanoparticles. These observations demonstrate how plasma explosion imaging directly reveals the diverse ways in which nanoparticles respond to strong laser fields, a process that is notoriously challenging to model because of the rapid evolution of materials properties that takes place on the femtosecond time scale as a solid nanostructure is transformed into a dense plasma.

Laser-accelerated proton conversion efficiency thickness scaling

The conversion efficiency from laser energy into proton kinetic energy is measured with the 0.6ps, 9×1019W∕cm2 Titan laser at the Jupiter Laser Facility as a function of target thickness in Au foils. For targets thicker than 20μm, the conversion efficiency scales approximately as 1∕L, where L is the target thickness. This is explained by the domination of hot electron collisional losses over adiabatic cooling. In thinner targets, the two effects become comparable, causing the conversion efficiency to scale weaker than 1∕L; the measured conversion efficiency is constant within the scatter in the data for targets between 5 and 15μm, with a peak conversion efficiency of 4% into protons with energy greater than 3MeV. Depletion of the hydrocarbon contaminant layer is eliminated as an explanation for this plateau by using targets coated with 200nm of ErH3 on the rear surface. The proton acceleration is modeled with the hybrid-particle in cell code LSP, which reproduced the conversion efficiency scaling observed...