M.P. Reijnders

Simulated performance of an ultracold ion source

At present, the smallest spot size which can be achieved with state-of-the-art focused ion beam (FIB) technology is mainly limited by the chromatic aberrations associated with the 4.5 eV energy spread of the liquid-metal ion source. Here we numerically investigate the performance of an ultracold ion source which has the potential for generating ion beams which combine high brightness with small energy spread. The source is based on creating very cold ion beams by near-threshold photoionization of a laser-cooled and trapped atomic gas. We present ab initio numerical calculations of the generation of ultracold beams in a realistic acceleration field and including all Coulomb interactions, i.e., both space charge effects and statistical Coulomb effects. These simulations demonstrate that with existing technology reduced brightness values exceeding 105 A m−2 sr−1 V−1 are feasible at an energy spread as low as 0.1 eV. The estimated spot size of the ultracold ion source in a FIB instrument ranges from 10 nm at ...

Ultracold electron source for single-shot diffraction studies

Ultracold electron sources, which are based on near-threshold photo- and field-ionization of a cloud of laser-cooled atoms, offer the unique combination of low emittance and extended size that is essential for achieving single-shot, ultrafast electron diffraction of macromolecules. Here we present measurements of the effective temperature of such a pulsed electron source employing rubidium atoms that are magneto-optically trapped at the center of an accelerator structure. Transverse source temperatures ranging from 200 K down to 10 K are demonstrated, controllable with the wavelength of the ionization laser. Together with the 50 μm source size, the achievable temperature enables a transverse coherence length of ≈20 nm for a 100 μm sample size.

Optimization of the current extracted from an ultracold ion source

Photoionization of trapped atoms is a recent technique for creating ion beams with low transverse temperature. The temporal behavior of the current that can be extracted from such an ultracold ion source is measured when operating in the pulsed mode. A number of experimental parameters are varied to find the conditions under which the time-averaged current is maximized. A dynamic model of the source is developed that agrees quite well with the experimental observations. The radiation pressure exerted by the excitation laser beam is found to substantially increase the extracted current. For a source volume with a typical root-mean-square radius of 20µm, a maximum peak current of 88pA is observed, limited by the available ionization laser power of 46mW. The optimum time-averaged current is 13pA at a 36% duty cycle. Particle-tracking simulations show that stochastic heating strongly reduces the brightness of the ion beam at higher current for the experimental conditions.

Measurement of the temperature of an ultracold ion source using time-dependent electric fields

We report on a measurement of the characteristic temperature of an ultracold rubidium ion source, in which a cloud of laser-cooled atoms is converted to ions by photo-ionization. Extracted ion pulses are focused on a detector with a pulsed-field technique. The resulting experimental spot sizes are compared to particle-tracking simulations, from which an effective source temperature T = (3 ± 2) mK and the corresponding transversal reduced emittance er = 1.4 × 10−8 m rad eV are determined. Space charge effects that may affect the measurement are also discussed.

Ultracold electron sources

Ultra-cold plasmas with electron temperatures of ~10 K can be created by photo-ionization just above threshold of a cloud of laser-cooled atoms. Recently it was shown 7 by GPT particle tracking simulations that an ultra-cold plasma has an enormous potential as a pulsed bright electron source. Here we discuss these results in the framework of normalized 6D brightness, which allows us to make a proper comparison both with the performance of pulsed, radio-frequency photo-emission sources and with the performance of continuous, needle-like field-emission sources. In addition we speculate on the possibility of using ultra-cold plasmas to realize quantum degenerate electron beams, constituting the ultimate limit in electron beam brightness.

Time-dependent manipulation of ultracold ion bunches

The combination of an ultracold ion source based on photoionization of a laser-cooled gas and time-dependent acceleration fields enables precise manipulation of ion beams. We demonstrate reduction in the longitudinal energy spread and transverse (de)focusing of the beam by applying time-dependent acceleration voltages. In addition, we show how time-dependent acceleration fields can be used to control both the sign and strength of the spherical aberrations. The experimental results are in close agreement with detailed charged particle tracking simulations and can be explained in terms of a simple analytical model.