O. J. Luiten

Compression of subrelativistic space-charge-dominated electron bunches for single-shot femtosecond electron diffraction.

We demonstrate the compression of 95 keV, space-charge-dominated electron bunches to sub-100 fs durations. These bunches have sufficient charge (200 fC) and are of sufficient quality to capture a diffraction pattern with a single shot, which we demonstrate by a diffraction experiment on a polycrystalline gold foil. Compression is realized by means of velocity bunching by inverting the positive space-charge-induced velocity chirp. This inversion is induced by the oscillatory longitudinal electric field of a 3 GHz radio-frequency cavity. The arrival time jitter is measured to be 80 fs.

Electron source concept for single-shot sub-100 fs electron diffraction in the 100 keV range

We present a method for producing sub-100 fs electron bunches that are suitable for single-shot ultrafast electron diffraction experiments in the 100 keV energy range. A combination of analytical estimates and state-of-the-art particle tracking simulations show that it is possible to create 100 keV, 0.1 pC, 30 fs electron bunches with a spot size smaller than 500u2002μm and a transverse coherence length of 3 nm, using established technologies in a table-top setup. The system operates in the space-charge dominated regime to produce energy-correlated bunches that are recompressed by radio-frequency techniques. With this approach we overcome the Coulomb expansion of the bunch, providing a single-shot, ultrafast electron diffraction source concept.

High-coherence electron bunches produced by femtosecond photoionization

With the development of ultrafast electron and X-ray sources it is becoming possible to study structural dynamics with atomic-level spatial and temporal resolution. Because of their short mean free path, electrons are particularly well suited for investigating surfaces and thin films, such as the challenging and important class of membrane proteins. To perform single-shot diffraction experiments on protein crystals, an ultracold electron source was proposed, based on near-threshold photoionization of laser-cooled atoms, which is capable of producing electron pulses of both high intensity and high coherence. Here we show that high coherence electron pulses can be produced by femtosecond photoionization, opening up a new regime of ultrafast structural dynamics experiments. The transverse coherence turns out to be much better than expected on the basis of the large bandwidth of the femtosecond ionization laser pulses. This surprising result can be explained by analysis of classical electron trajectories.

Optical cooling of atomic hydrogen in a magnetic trap

We describe the prospects for optical cooling of magnetically trapped atomic hydrogen. We analyze the performance of an optical system currently under development in our laboratory and present calculations for the optical cooling rate. We conclude that by using optical techniques hydrogen can be cooled to below 10 mK while the density is simultaneously boosted to approximately 1014 cm−3. The same system can be used for thermometry down to temperatures well into the microkelvin regime.

Simulated performance of an ultracold ion source

At present, the smallest spot size which can be achieved with state-of-the-art focused ion beam (FIB) technology is mainly limited by the chromatic aberrations associated with the 4.5 eV energy spread of the liquid-metal ion source. Here we numerically investigate the performance of an ultracold ion source which has the potential for generating ion beams which combine high brightness with small energy spread. The source is based on creating very cold ion beams by near-threshold photoionization of a laser-cooled and trapped atomic gas. We present ab initio numerical calculations of the generation of ultracold beams in a realistic acceleration field and including all Coulomb interactions, i.e., both space charge effects and statistical Coulomb effects. These simulations demonstrate that with existing technology reduced brightness values exceeding 105u2002Au2009m−2u2009sr−1u2009V−1 are feasible at an energy spread as low as 0.1 eV. The estimated spot size of the ultracold ion source in a FIB instrument ranges from 10 nm at ...

Cold electron and ion beams generated from trapped atoms

A novel way of creating low-temperature electron and ion beams is demonstrated. The beams are generated by converting a laser-cooled atom cloud to a highly excited Rydberg gas, which subsequently develops into an ultracold plasma. Charged particles are extracted from the Rydberg gas and the plasma by a pulsed electric field. The properties of the resulting electron and ion pulses are experimentally studied. Pulses of a few hundred ns duration containing a few pC of charge were observed. Upper limits for the temperature of such beams (60K for ions and 500K for electrons) are obtained, and the beams are shown to have low emittance. Further development of the method may lead to the generation of high-brightness charged-particle beams from ultracold plasmas.

Ultracold electron source for single-shot, ultrafast electron diffraction

Ultrafast electron diffraction (UED) enables studies of structural dynamics at atomic length and timescales, i.e., 0.1 nm and 0.1 ps, in single-shot mode. At present UED experiments are based on femtosecond laser photoemission from solid state cathodes. These photoemission sources perform excellently, but are not sufficiently bright for single-shot studies of, for example, biomolecular samples. We propose a new type of electron source, based on near-threshold photoionization of a laser-cooled and trapped atomic gas. The electron temperature of these sources can be as low as 10 K, implying an increase in brightness by orders of magnitude. We investigate a setup consisting of an ultracold electron source and standard radio-frequency acceleration techniques by GPT tracking simulations. The simulations use realistic fields and include all pairwise Coulomb interactions. We show that in this setup 120 keV, 0.1 pC electron bunches can be produced with a longitudinal emittance sufficiently small for enabling sub-100 fs bunch lengths at 1% relative energy spread. A transverse root-mean-square normalized emittance of epsilon(x) = 10 nm is obtained, significantly better than from photoemission sources. Correlations in transverse phase-space indicate that the transverse emittance can be improved even further, enabling single-shot studies of biomolecular samples.

High-brightness, narrowband, and compact soft x-ray Cherenkov sources in the water window

Narrowband, soft x-ray Cherenkov radiation at energies of 453 and 512 eV has been generated by 10 MeV electrons in, respectively, titanium and vanadium foils. The measured spectral and angular distribution of the radiation, and the measured total yield (≈10−4 photon per electron) are in agreement with theoretical predictions based on refractive index data. We show that the brightness that can be achieved using a small electron accelerator is sufficient for practical x-ray microscopy in the water-window spectral region.

Ultracold electron source for single-shot diffraction studies

Ultracold electron sources, which are based on near-threshold photo- and field-ionization of a cloud of laser-cooled atoms, offer the unique combination of low emittance and extended size that is essential for achieving single-shot, ultrafast electron diffraction of macromolecules. Here we present measurements of the effective temperature of such a pulsed electron source employing rubidium atoms that are magneto-optically trapped at the center of an accelerator structure. Transverse source temperatures ranging from 200u2009K down to 10u2009K are demonstrated, controllable with the wavelength of the ionization laser. Together with the 50u2009μm source size, the achievable temperature enables a transverse coherence length of ≈20u2009nm for a 100u2009μm sample size.

Effective temperature of an ultracold electron source based on near-threshold photoionization

We present a detailed description of measurements of the effective temperature of a pulsed electron source, based on near-threshold photoionization of laser-cooled atoms. The temperature is determined by electron beam waist scans, source size measurements with ion beams, and analysis with an accurate beam line model. Experimental data is presented for the source temperature as a function of the wavelength of the photoionization laser, for both nanosecond and femtosecond ionization pulses. For the nanosecond laser, temperatures as low as 14 ± 3 K were found; for femtosecond photoionization, 30 ± 5 K is possible. With a typical source size of 25 μm, this results in electron bunches with a relative transverse coherence length in the 10⁻⁴ range and an emittance of a few nm rad.