M. Roncadelli

Effects of Nitrogen contamination in liquid Argon

A dedicated test of the effects of Nitrogen contamination in liquid Argon has been performed at the INFN-Gran Sasso Laboratory (LNGS, Italy) within the WArP R&D program. A detector has been designed and assembled for this specific task and connected to a system for the injection of controlled amounts of gaseous Nitrogen into the liquid Argon. The purpose of the test is to detect the reduction of the Ar scintillation light emission as a function of the amount of the Nitrogen contaminant injected in the Argon volume. A wide concentration range, spanning from ~ 10?1 ppm up to ~ 103 ppm, has been explored. Measurements have been done with electrons in the energy range of minimum ionizing particles (?-conversion from radioactive sources). Source spectra at different Nitrogen contaminations are analyzed, showing sensitive reduction of the scintillation yield at increasing concentrations. Direct PMT signal acquisition exploiting high time resolution by fast waveform recording allowed high precision extraction of the main characteristics of the scintillation light emission in contaminated LAr. In particular, the decreasing behavior in lifetime and relative amplitude of the slow component is found to be appreciable starting from (1 ppm) of Nitrogen concentrations. The rate constant of the quenching process induced by Nitrogen in liquid Ar has been found to be kQ(N2) = 0.11 ? 0.01 ?s?1ppm?1, consistent with a previous measurement of this quantity but with significant improvement in precision. On the other hand, no evidence for absorption by N2 impurities has been found up to the higher concentrations here explored.

Oxygen contamination in liquid Argon: combined effects on ionization electron charge and scintillation light

A dedicated test of the effects of Oxygen contamination in liquid Argon has been performed at the INFN-Gran Sasso Laboratory (LNGS, Italy) within the WArP R&D program. Two detectors have been used: the WArP2.3 lt prototype and a small (0.7 lt) dedicated detector, coupled with a system for the injection of controlled amounts of gaseous Oxygen. O2 contamination in LAr leads to depletion of both the free electron charge (via attachment process) and the scintillation light (via quenching and absorption mechanisms) available for ionization signal detection. Purpose of the test with the 0.7 lt detector was to detect the reduction of the long-lived component lifetime of the Argon scintillation light emission and of the overall light yield at increasing O2 concentration. Data from the WArP prototype were used for determining the behavior of both the ionization electron lifetime and the scintillation long-lived component lifetime at decreasing O2 concentration by the purification process activated in closed loop during the acquisition run. The electron lifetime measurements allowed to infer the O2 content of the Argon and correlate it with the long-lived scintillation lifetime data. The effects of Oxygen contamination on the scintillation light have been thus extensively measured over a wide range of O2 concentration, spanning from ~ 10−3 ppm up to ~ 10 ppm.

The WArP experiment

Cryogenic noble liquid detectors are presently considered one of the best options for WIMP Dark Matter searches, especially when extensions to multi ton scale sensitive masses are foreseen. The WArP experiment is the first one that exploits the unique characteristics of liquid Argon to make a highly sensitive search for WIMP Dark Matter candidates. In 2008, a double phase detector has been assembled in the Gran Sasso National Laboratory with 140 kg sensitive mass and a discovery potential in the range of 5 × 10−45 cm2 in the spin-independent WIMP-nucleon cross-section. In addition to standard neutrons and gamma-rays passive shields, WArP implements an 8 ton liquid Argon active shield with 4π coverage. The detector was commissioned and put into operation during the first half of 2009 for a first technical run. This first run lasted about three months and then it was stopped for some detector repairs and modifications in the summer of 2009. A second run was started at the beginning of 2010. Detector design, construction and assembly are described, together with the results of the technical run and the very first results of the 2010 run.

Discovery of underground argon with a low level of radioactive 39Ar and possible applications to WIMP dark matter detectors

We report on the first measurement of 39Ar in argon from underground natural gas reservoirs. The gas stored in the US National Helium Reserve was found to contain a low level of 39Ar. The ratio of 39Ar to stable argon was found to be ≤4×10-17 (84% C.L.), less than 5% the value in atmospheric argon (39Ar/Ar=8×10-16). The total quantity of argon currently stored in the National Helium Reserve is estimated at 1000 tons. 39Ar represents one of the most important backgrounds in argon detectors for WIMP dark matter searches. The findings reported demonstrate the possibility of constructing large multi-ton argon detectors with low radioactivity suitable for WIMP dark matter searches.