Matthias Mulsow

Spatio-temporal evolution of the dust particle size distribution in dusty argon rf plasmas

An imaging Mie scattering technique has been developed to measure the spatially resolved size distribution of dust particles in extended dust clouds. For large dust clouds of micrometre-sized plastic particles confined in an radio frequency (rf) discharge, a segmentation of the dust cloud into populations of different sizes is observed, even though the size differences are very small. The dust size dispersion inside a population is much smaller than the difference between the populations. Furthermore, the dust size is found to be constantly decreasing over time while the particles are confined in an inert argon plasma. The processes responsible for the shrinking of the dust in the plasma have been addressed by mass spectrometry, ex situ microscopy of the dust size, dust resonance measurements, in situ determination of the dust surface temperature and Fourier transform infrared absorption (FT-IR). It is concluded that both a reduction of dust size and its mass density due to outgassing of water and other volatile constituents as well as chemical etching by oxygen impurities are responsible for the observations.

Crystal and fluid modes in three-dimensional finite dust clouds

The spectral properties of three-dimensional dust clusters confined in gaseous discharges are investigated using both a fluid mode description and the normal mode analysis (NMA). The modes are analysed for crystalline clusters as well as for laser-heated fluid-like clusters. It is shown that even for clusters with low particle numbers and under presence of damping fluid modes can be identified. Laser-heating leads to the excitation of several, mainly transverse, modes. The mode frequencies are found to be nearly independent of the coupling parameter and support the predictions of the underlying theory. The NMA and the fluid mode spectra demonstrate that the wakefield attraction is present for the experimentally observed Yukawa balls at low pressure. Both methods complement each other, since NMA is more suitable for crystalline clusters, whereas the fluid modes allow to explore even fluid-like dust clouds.

Stereoscopic imaging of dusty plasmas

The fundamentals of stereoscopy and their application to dusty plasmas are described. It is shown that stereoscopic methods allow us to measure the three-dimensional particle positions and trajectories with high spatial and temporal resolution. The underlying technical implications are presented and requirements and limitations are discussed. The stereoscopic method is demonstrated for dust particles in dust-density waves under microgravity conditions.

Correlation buildup during recrystallization in three-dimensional dusty plasma clusters

The recrystallization process of finite three-dimensional dust clouds after laser heating is studied experimentally. The time-dependent Coulomb coupling parameter is presented, showing that the recrystallization starts with an exponential cooling phase where cooling is slower than damping by the neutral gas friction. At later times, the coupling parameter oscillates into equilibrium. It is found that a large fraction of cluster states after recrystallization experiments is in metastable states. The temporal evolution of the correlation buildup shows that correlation occurs on even slower time scale than cooling.

Analysis of 3D vortex motion in a dusty plasma

Dust clusters of about 50–1000 particles have been confined near the sheath region of a gaseous radio-frequency plasma discharge. These compact clusters exhibit a vortex motion which has been reconstructed in full three dimensions from stereoscopy. Smaller clusters are found to show a competition between solid-like cluster structure and vortex motion, whereas larger clusters feature very pronounced vortices. From the three-dimensional analysis, the dust flow field has been found to be nearly incompressible. The vortices in all observed clusters are essentially poloidal. The dependence of the vorticity on the cluster size is discussed. Finally, the vortex motion has been quantitatively attributed to radial gradients of the ion drag force.

Recrystallization in Finite 3-D Dust Clouds

The recrystallization process of a finite dust cloud is studied experimentally on the kinetic level. The temporal evolution of the coupling parameter allows to reveal that the cluster is molten while laser heated and recrystallizes when heating is switched OFF. The cooling rate can be deduced from the initial stage of recrystallization.

Experimental determination of phase transitions by means of configurational entropies in finite Yukawa balls

The phase transition of finite Yukawa balls (ordered systems of microspheres in a gaseous plasma environment) with less than 100 particles is studied experimentally by means of configurational entropies. We have developed cylindrical two- and three-particle-correlation functions to measure these entropies for multiple cluster sizes over a wide temperature range. The cluster temperature is finely tuned using a stochastic laser heating setup. It is shown that the correlation functions give a detailed insight into the structural properties of the cluster. The derived configurational entropies give a clear indication of the transition temperature from a solid-like to a fluid-like state. Comparing the transition temperatures of different sized clusters it is found that the transition temperature increases with cluster size in general agreement with theoretical predictions.