Michael Geiselmann

Photonic chip based optical frequency comb using soliton induced Cherenkov radiation

Timing on a chip Laser-induced optical frequency combs allow precision measurements and affect a broad range of technologies. Brasch et al. generated optical frequency combs on an optical chip (see the Perspective by Akhmediev and Devine). They induced an optical soliton, or optical bullet, and propagated it in an engineered microcavity waveguide. The emitted output light formed a coherent comb of frequencies spanning two-thirds of an octave. Such an on-chip demonstration bodes well for miniaturization of metrological technology and its adaption for widespread application. Science, this issue p. 357; see also p. 340 A broadband and coherent frequency comb is generated with an optical microresonator. [Also see Perspective by Akhmediev and Devine] Optical solitons are propagating pulses of light that retain their shape because nonlinearity and dispersion balance each other. In the presence of higher-order dispersion, optical solitons can emit dispersive waves via the process of soliton Cherenkov radiation. This process underlies supercontinuum generation and is of critical importance in frequency metrology. Using a continuous wave–pumped, dispersion-engineered, integrated silicon nitride microresonator, we generated continuously circulating temporal dissipative Kerr solitons. The presence of higher-order dispersion led to the emission of red-shifted soliton Cherenkov radiation. The output corresponds to a fully coherent optical frequency comb that spans two-thirds of an octave and whose phase we were able to stabilize to the sub-Hertz level. By preserving coherence over a broad spectral bandwidth, our device offers the opportunity to develop compact on-chip frequency combs for frequency metrology or spectroscopy.

Three-dimensional optical manipulation of a single electron spin

Nitrogen vacancy (NV) centres in diamond are promising elemental blocks for quantum optics, spin-based quantum information processing and high-resolution sensing. However, fully exploiting the capabilities of these NV centres requires suitable strategies to accurately manipulate them. Here, we use optical tweezers as a tool to achieve deterministic trapping and three-dimensional spatial manipulation of individual nanodiamonds hosting a single NV spin. Remarkably, we find that the NV axis is nearly fixed inside the trap and can be controlled in situ by adjusting the polarization of the trapping light. By combining this unique spatial and angular control with coherent manipulation of the NV spin and fluorescence lifetime measurements near an integrated photonic system, we demonstrate individual optically trapped NV centres as a novel route for both three-dimensional vectorial magnetometry and sensing of the local density of optical states.

Coupling of individual quantum emitters to channel plasmons

Efficient light-matter interaction lies at the heart of many emerging technologies that seek on-chip integration of solid-state photonic systems. Plasmonic waveguides, which guide the radiation in the form of strongly confined surface plasmon-polariton modes, represent a promising solution to manipulate single photons in coplanar architectures with unprecedented small footprints. Here we demonstrate coupling of the emission from a single quantum emitter to the channel plasmon polaritons supported by a V-groove plasmonic waveguide. Extensive theoretical simulations enable us to determine the position and orientation of the quantum emitter for optimum coupling. Concomitantly with these predictions, we demonstrate experimentally that 42% of a single nitrogen-vacancy centre emission efficiently couples into the supported modes of the V-groove. This work paves the way towards practical realization of efficient and long distance transfer of energy for integrated solid-state quantum systems.

Photonic Damascene process for integrated high-Q microresonator based nonlinear photonics

High confinement, integrated silicon nitride (SiN) waveguides have recently emerged as an attractive platform for on-chip nonlinear optical devices. The fabrication of high-Q SiN microresonators with anomalous group velocity dispersion has enabled broadband nonlinear optical frequency comb generation. Such frequency combs have been successfully applied in coherent communication and ultrashort pulse generation. However, the reliable fabrication of high confinement waveguides from stoichiometric, high stress SiN remains challenging. Here we present a novel photonic Damascene fabrication process enabling the use of substrate topography for stress control and thin film crack prevention. With close to unity sample yield we fabricate microresonators with 1.35 mu m thick waveguides and optical Q-factors of 3.7 x 10(6) and demonstrate single temporal dissipative Kerr soliton based coherent optical frequency comb generation. Our newly developed process is also interesting for other material platforms, photonic integration, and mid-infrared Kerr comb generation

Raman Self-Frequency Shift of Dissipative Kerr Solitons in an Optical Microresonator.

The formation of temporal dissipative solitons in continuous wave laser driven microresonators enables the generation of coherent, broadband and spectrally smooth optical frequency combs as well as femtosecond pulses with compact form factor. Here we report for the first time on the observation of a Raman-induced soliton self-frequency shift for a microresonator soliton. The Raman effect manifests itself in amorphous SiN microresonator based single soliton states by a spectrum that is hyperbolic secant in shape, but whose center is spectrally red-shifted (i.e. offset) from the continuous wave pump laser. The shift is theoretically described by the first order shock term of the material’s Raman response, and we infer a Raman shock time of 20 fs for amorphous SiN. Moreover, we observe that the Raman induced frequency shift can lead to a cancellation or overcompensation of the soliton recoil caused by the formation of a (coherent) dispersive wave. The observations are in excellent agreement with numerical simulations based on the Lugiato-Lefever equation (LLE) with a Raman shock term. Our results contribute to the understanding of Kerr frequency combs in the soliton regime, enable to substantially improve the accuracy of modeling and are relevant to the fundamental timing jitter of microresonator solitons.We experimentally observed the Raman-induced self-frequency shift of high-intensity dissipative Kerr solitons in high-Q silicon nitride microresonators. The Raman redshift is linearly dependent on the pump-frequency-detuning, associated with the tunability of the soliton pulse duration.

Deterministic Optical-Near-Field-Assisted Positioning of Nitrogen-Vacancy Centers

Nanopositioning of single quantum emitters to control their coupling to integrated photonic structures is a crucial step in the fabrication of solid-state quantum optics devices. We use the optical near-field enhancement produced by nanofabricated gold antennas subject to near-infrared illumination to deterministically trap and position single nanodiamonds (NDs) hosting nitrogen-vacancy (NV) centers. The positioning of the NDs at the antenna regions of maximum field intensity is first characterized using both fluorescence and electron microscopy imaging. We further study the interaction between the nanoantenna and the delivered NV center by analyzing its change in fluorescence lifetime, which is driven by the increase in the local density of optical states at the trapping positions. Additionally, the plasmonic enhancement of the near-field intensity allows us to optically control the NV excited lifetime using relatively low NIR illumination intensities, some 20 times lower than in the absence of the antennas.

Self-referenced photonic chip soliton Kerr frequency comb

Self-referencing turns pulsed laser systems into self-referenced frequency combs. Such frequency combs allow counting of optical frequencies and have a wide range of applications. The required optical bandwidth to implement self-referencing is typically obtained via nonlinear broadening in optical fibers. Recent advances in the field of Kerr frequency combs have provided a path towards the development of compact frequency comb sources that provide broadband frequency combs, exhibit microwave repetition rates and that are compatible with on-chip photonic integration. These devices have the potential to significantly expand the use of frequency combs. Yet to date self-referencing of such Kerr frequency combs has only been attained by applying conventional, fiber based broadening techniques. Here we demonstrate external broadening-free self-referencing of a Kerr frequency comb. An optical spectrum that spans two-thirds of an octave is directly synthesized from a continuous wave laser-driven silicon nitride microresonator using temporal dissipative Kerr soliton formation and soliton Cherenkov radiation. Using this coherent bandwidth and two continuous wave transfer lasers in a 2f-3f self-referencing scheme, we are able to detect the offset frequency of the soliton Kerr frequency comb. By stabilizing the repetition rate to a radio frequency reference the self-referenced frequency comb is used to count and track the continuous wave pump laser’s frequency. This work demonstrates the principal ability of soliton Kerr frequency combs to provide microwave-to-optical clockworks on a chip.Self-referencing turns pulsed laser systems into self-referenced frequency combs. Such frequency combs allow counting of optical frequencies and have a wide range of applications. The required optical bandwidth to implement self-referencing is typically obtained via nonlinear broadening in optical fibers. Recent advances in the field of Kerr frequency combs have provided a path toward the development of compact frequency comb sources that provide broadband frequency combs, exhibit microwave repetition rates and are compatible with on-chip photonic integration. These devices have the potential to significantly expand the use of frequency combs. Yet to date, self-referencing of such Kerr frequency combs has only been attained by applying conventional, fiber-based broadening techniques. Here we demonstrate external broadening-free self-referencing of a Kerr frequency comb. An optical spectrum spanning two-thirds of an octave is directly synthesized from a continuous wave laser-driven silicon nitride microresonator using temporal dissipative Kerr soliton formation and soliton Cherenkov radiation. Using this coherent bandwidth and two continuous wave transfer lasers in a 2f–3f self-referencing scheme, we are able to detect the offset frequency of the soliton Kerr frequency comb. By stabilizing the repetition rate to a radio frequency reference, the self-referenced frequency comb is used to count and track the continuous wave pump laser’s frequency. This work demonstrates the principal ability of soliton Kerr frequency combs to provide microwave-to-optical clockworks on a chip.

Fast optical modulation of the fluorescence from a single nitrogen–vacancy centre

The intensity of optically-pumped fluorescence generated from a single atomic defect in diamond can be reduced by 80% in just 100 ns by applying infrared laser light. This result demonstrates the possibility of using these so-called nitrogen–vacancy centres to create optical switches that operate at room temperature.

Coupling ideality of integrated planar high-Q microresonators

Chip-scale optical microresonators with integrated planar optical waveguides are useful building blocks for linear, nonlinear, and quantum-optical photonic devices alike. Loss reduction through improving fabrication processes results in several integrated microresonator platforms attaining quality (Q) factors of several millions. Beyond the improvement of the quality factor, the ability to operate the microresonator with high coupling ideality in the overcoupled regime is of central importance. In this regime, the dominant source of loss constitutes the coupling to a single desired output channel, which is particularly important not only for quantum-optical applications such as the generation of squeezed light and correlated photon pairs but also for linear and nonlinear photonics. However, to date, the coupling ideality in integrated photonic microresonators is not well understood, in particular, design-dependent losses and their impact on the regime of high ideality. Here we investigate design-dependent parasitic losses described by the coupling ideality of the commonly employed microresonator design consisting of a microring-resonator waveguide side coupled to a straight bus waveguide, a system which is not properly described by the conventional input-output theory of open systems due to the presence of higher-order modes. By systematic characterization of multimode high-Q silicon nitride microresonator devices, we show that this design can suffer from low coupling ideality. By performing 3D simulations, we identify the coupling to higher-order bus waveguide modes as the dominant origin of parasitic losses which lead to the low coupling ideality. Using suitably designed bus waveguides, parasitic losses are mitigated with a nearly unity ideality and strong overcoupling (i.e., a ratio of external coupling to internal resonator loss rate > 9) are demonstrated. Moreover, we find that different resonator modes can exchange power through the coupler, which, therefore, constitutes a mechanism that induces modal coupling, a phenomenon known to distort resonator dispersion properties. Our results demonstrate the potential for significant performance improvements of integrated planar microresonators for applications in quantum optics and nonlinear photonics achievable by optimized coupler designs.

Intermode Breather Solitons in Optical Microresonators

Dissipative solitons can be found in a variety of systems resulting from the double balance between dispersion and nonlinearity, as well as gain and loss. Recently, they have been observed to spontaneously form in Kerr nonlinear microresonators driven by a continuous wave laser, providing a compact source of coherent optical frequency combs. As optical microresonators are commonly multimode, intermode interactions, which give rise to avoided mode crossings, frequently occur and can alter the soliton properties. Recent works have shown that avoided mode crossings cause the soliton to acquire a single-mode dispersive wave, a recoil in the spectrum, or lead to soliton decay. Here, we show that avoided mode crossings can also trigger the formation of breather solitons, solitons that undergo a periodic evolution in their amplitude and duration. This new breather soliton, referred to as an intermode breather soliton, occurs within a laser detuning range where conventionally stationary (i.e., stable) dissipative Kerr solitons are expected. We experimentally demonstrate the phenomenon in two microresonator platforms (crystalline magnesium fluoride and photonic chip-based silicon nitride microresonators) and theoretically describe the dynamics based on a pair of coupled Lugiato-Lefever equations. We show that the breathing is associated with a periodic energy exchange between the soliton and a second optical mode family, a behavior that can be modeled by a response function acting on dissipative solitons described by the Lugiato-Lefever model. The observation of breathing dynamics in the conventionally stable soliton regime is relevant to applications in metrology such as low-noise microwave generation, frequency synthesis, or spectroscopy.