Michael Scheibner

Stark effect and polarizability in a single CdSe/ZnSe quantum dot

The quantum-confined Stark effect in a single self-assembled CdSe/ZnSe quantum dot was studied by means of highly spatially resolved photoluminescence spectroscopy. A nanotechnological approach making use of a capacitor-like geometry enabled us to apply a well-defined lateral electric field on the quantum dots. Stark shifts of up to 1.1 meV were obtained, which can be well fitted by a purely quadratic dependence on an electric field. In quite good agreement with theoretical calculations, an exciton polarizability of 4.9×10−3 meV/(kV/cm)2 can be extracted, while the permanent dipole moment in the lateral direction is found to be negligible.

Engineering electron and hole tunneling with asymmetric InAs quantum dot molecules

Most self-assembled quantum dot molecules are intrinsically asymmetric with inequivalent dots resulting from imperfect control of crystal growth. The authors have grown vertically aligned pairs of InAs∕GaAs quantum dots by molecular beam epitaxy, introducing intentional asymmetry that limits the influence of intrinsic growth fluctuations and allows selective tunneling of electrons or holes. They present a systemic investigation of tunneling energies over a wide range of interdot barrier thickness. The concepts discussed here provide an important tool for the systematic design and characterization of more complicated quantum dot nanostructures.

Electrically Tunable g Factors in Quantum Dot Molecular Spin States

We present a magnetophotoluminescence study of individual vertically stacked InAs/GaAs quantum dot pairs separated by thin tunnel barriers. As an applied electric field tunes the relative energies of the two dots, we observe a strong resonant increase or decrease in the g factors of different spin states that have molecular wave functions distributed over both quantum dots. We propose a phenomenological model for the change in g factor based on resonant changes in the amplitude of the wave function in the barrier due to the formation of bonding and antibonding orbitals.

Spin fine structure of optically excited quantum dot molecules

The interaction between spins in coupled quantum dots is revealed in distinct fine structure patterns in the measured optical spectra of

Photoluminescence spectroscopy of the molecular biexciton in vertically stacked InAs-GaAs quantum dot pairs

\mathrm{In}\mathrm{As}∕\mathrm{Ga}\mathrm{As}

Optophononics with coupled quantum dots

double quantum dot molecules containing zero, one, or two excess holes. The fine structure is explained well in terms of a uniquely molecular interplay of spin-exchange interactions, Pauli exclusion, and orbital tunneling. This knowledge is critical for converting quantum dot molecule tunneling into a means of optically coupling not just orbitals but also spins.

Sign reversal and light controlled tuning of circular polarization in semimagnetic CdMnSe quantum dots

We present photoluminescence studies of the molecular neutral biexciton-exciton spectra of individual vertically stacked InAs/GaAs quantum dot pairs. We tune either the hole or the electron levels of the two dots into tunneling resonances. The spectra are described well within a few-level, few-particle molecular model. Their properties can be modified broadly by an electric field and by structural design, which makes them highly attractive for controlling nonlinear optical properties.

Quantum-confined Stark effects in coupled InAs/GaAs quantum dots

Modern technology is founded on the intimate understanding of how to utilize and control electrons. Next to electrons, nature uses phonons, quantized vibrations of an elastic structure, to carry energy, momentum and even information through solids. Phonons permeate the crystalline components of modern technology, yet in terms of technological utilization phonons are far from being on par with electrons. Here we demonstrate how phonons can be employed to render a single quantum dot pair optically transparent. This phonon-induced transparency is realized via the formation of a molecular polaron, the result of a Fano-type quantum interference, which proves that we have accomplished making typically incoherent and dissipative phonons behave in a coherent and non-dissipative manner. We find the transparency to be widely tunable by electronic and optical means. Thereby we show amplification of weakest coupling channels. We further outline the molecular polarons potential as a control element in phononic circuitry architecture.

Entanglement Dynamics of Molecular Exciton States in Coupled Quantum Dots

Circularly polarized luminescence of CdMnSe quantum dots in magnetic fields up to 5 T is studied for nominal Mn concentrations of 0%, 1%, and 2% by using a photoelastic modulator technique. The exciton g factors as well as spin relaxation times were determined from the polarized luminescence taking into account the exciton lifetimes, which were also extracted by means of time-resolved photoluminescence spectroscopy. For quantum dots without Mn and with 2% Mn exciton g factors of −1.62 and +1.32, respectively, were found. The quantum dots with 1% Mn show a vanishing small value of g for small excitation powers. For this structure the polarization properties are dominated by the optical orientation. Interestingly, for the 1% Mn quantum dots with increasing excitation power considerable changes of the polarization and the exciton g factor were observed which are interpreted in terms of heating effects. From the power dependence indirect heating via phonons and above a critical value direct heating due to pho...

Stabilization of the Cubic Crystalline Phase in Organometal Halide Perovskite Quantum Dots via Surface Energy Manipulation

We report the effects of tunnel coupling on the Quantum-Confined Stark Effect (QCSE) for excitons in InAs/GaAs coupled quantum dots (CQDs). As the barrier separating the dots is reduced, the zero-field dipole moment and the polarizability are both found to increase. This systematic variation as a function of barrier thickness is due to factors including the formation of molecular wavefunctions, the electron/hole effective masses, and the CQD structural properties. The dipole moment for the interdot exciton is found to be up to 100 times larger than that of the intradot exciton resulting in a predominantly linear shift with field. The ability to control the QCSE of the exciton in a single CQD could be useful for a new class of single photon optical switches and tunable emitters.