Myriam Zerrad

Characterization of zirconia– and niobia–silica mixture coatings produced by ion-beam sputtering

ZrO2-SiO2 and Nb2O5-SiO2 mixture coatings as well as those of pure zirconia (ZrO2), niobia (Nb2O5), and silica (SiO2) deposited by ion-beam sputtering were investigated. Refractive-index dispersions, bandgaps, and volumetric fractions of materials in mixed coatings were analyzed from spectrophotometric data. Optical scattering, surface roughness, nanostructure, and optical resistance were also studied. Zirconia-silica mixtures experience the transition from crystalline to amorphous phase by increasing the content of SiO2. This also results in reduced surface roughness. All niobia and silica coatings and their mixtures were amorphous. The obtained laser-induced damage thresholds in the subpicosecond range also correlates with respect to the silica content in both zirconia- and niobia-silica mixtures.

A high accuracy femto-/picosecond laser damage test facility dedicated to the study of optical thin films

A laser damage test facility delivering pulses from 100 fs to 3 ps and designed to operate at 1030 nm is presented. The different details of its implementation and performances are given. The originality of this system relies the online damage detection system based on Nomarski microscopy and the use of a non-conventional energy detection method based on the utilization of a cooled CCD that offers the possibility to obtain the laser induced damage threshold (LIDT) with high accuracy. Applications of this instrument to study thin films under laser irradiation are presented. Particularly the deterministic behavior of the sub-picosecond damage is investigated in the case of fused silica and oxide films. It is demonstrated that the transition of 0-1 damage probability is very sharp and the LIDT is perfectly deterministic at few hundreds of femtoseconds. The damage process in dielectric materials being the results of electronic processes, specific information such as the material bandgap is needed for the interpretation of results and applications of scaling laws. A review of the different approaches for the estimation of the absorption gap of optical dielectric coatings is conducted and the results given by the different methods are compared and discussed. The LIDT and gap of several oxide materials are then measured with the presented instrument: Al(2)O(3), Nb(2)O(5), HfO(2), SiO(2), Ta(2)O(5), and ZrO(2). The obtained relation between the LIDT and gap at 1030 nm confirms the linear evolution of the threshold with the bandgap that exists at 800 nm, and our work expands the number of tested materials.

Laser-induced damage of hafnia coatings as a function of pulse duration in the femtosecond to nanosecond range

Laser-damage thresholds and morphologies of hafnia single layers exposed under femtosecond, picosecond, and nanosecond single pulses (1030/1064 nm) are reported. The samples were made with different deposition parameters in order to study how the damage behavior of the samples evolves with the pulse duration and how it is linked to the deposition process. In the femtosecond to picosecond regime, the scaling law of the laser-induced damage threshold as a function of pulse duration is in good agreement with the models of photo and avalanche ionization based on the rate equation for free electron generation. However, differences in the damage morphologies between samples are shown. No correlation between the nanosecond and femtosecond/picosecond laser-damage resistance of hafnia coatings could be established. We also report evidence of the transition in damage mechanisms for hafnia, from an ablation process linked to intrinsic properties of the material to a defect-induced process, that exists between a few picoseconds and a few tens of picoseconds.

Spectral effectiveness of engineered thermal cloaks in the frequency regime

We analyse basic thermal cloaks designed via different geometric transforms applied to thermal cloaking. We evaluate quantitatively the effectiveness of these heterogeneous anisotropic thermal cloaks through the calculation of the standard deviation of the isotherms. The study addresses the frequency regime and we point out the cloaks spectral effectiveness. We find that all these cloaks have comparable effectiveness irrespective of whether or not they have singular conductivity at their inner boundary. However, approximate cloaking with multi-layered cloak critically depends upon the homogenization algorithm and it is shown that the standard deviation varies linearly with the inverse of the number of layers.

Spatially resolved surface topography retrieved from far-field intensity scattering measurements

A far-field setup based on the fast and simultaneous recording of 1 million intensity angle-resolved-light-scattering patterns allows both to reconstruct surface topography and to cancel local defects in this topography. A spectral analysis is performed on measured data and allows to extract roughness and slopes mapping of a surface taking into account the spectral bandpass.

Light enpolarization by disordered media under partial polarized illumination: The role of cross-scattering coefficients

We show how disordered media allow to increase the local degree of polarization (DOP) of an arbitrary (partial) polarized incident beam. The role of cross-scattering coefficients is emphasized, together with the probability density functions (PDF) of the scattering DOP. The average DOP of scattering is calculated versus the incident illumination DOP.

Transformed Fourier and Fick equations for the control of heat and mass diffusion

We review recent advances in the control of diffusion processes in thermodynamics and life sciences through geometric transforms in the Fourier and Fick equations, which govern heat and mass diffusion, respectively. We propose to further encompass transport properties in the transformed equations, whereby the temperature is governed by a three-dimensional, time-dependent, anisotropic heterogeneous convection-diffusion equation, which is a parabolic partial differential equation combining the diffusion equation and the advection equation. We perform two dimensional finite element computations for cloaks, concentrators and rotators of a complex shape in the transient regime. We precise that in contrast to invisibility cloaks for waves, the temperature (or mass concentration) inside a diffusion cloak crucially depends upon time, its distance from the source, and the diffusivity of the invisibility region. However, heat (or mass) diffusion outside cloaks, concentrators and rotators is unaffected by their presence, whatever their shape or position. Finally, we propose simplified designs of layered cylindrical and spherical diffusion cloaks that might foster experimental efforts in thermal and biochemical metamaterials.

Coherence and polarization properties in speckle of totally depolarized light scattered by totally depolarizing media

When a totally unpolarized light is scattered by a medium that spatially totally depolarizes incident polarized light, the scattered field presents an increase of the order described by the temporal degree of polarization. We analyze the behavior of some polarization and coherence properties in such a physical situation.

Depolarization and enpolarization DOP histograms measured for surface and bulk speckle patterns

dop histograms are measured in the off-specular far field speckle of disordered media under polarized and unpolarized illumination. Three surface samples with increasing roughnesses, and three bulk samples with different absorption levels, are investigated. Results show that both rough surfaces and absorbing bulks hold the incident polarization, while transparent bulks allow to depolarize or to enpolarize the incident light. Hence we provide a first experimental evidence of such effects.

Enpolarization and depolarization of light scattered from chromatic complex media

Influence of the variations of the scattering properties of a disordered medium with respect to frequency on the polarization of scattered light is investigated. We focus on the strongly scattering regime with the sum of random phasors scattering model that is extended to chromatic media and made frequency-sensitive. It is numerically shown how the scattered polarization depends on the incident polarization and the incident light bandwidth to scattering coefficients chromatic length ratio. Under the presented approach, both phenomena of depolarization and enpolarization of light appear unified.