O. Jagutzki

Correlated electron emission in multiphoton double ionization

Electronic correlations govern the dynamics of many phenomena in nature, such as chemical reactions and solid state effects, including superconductivity. Such correlation effects can be most clearly investigated in processes involving single atoms. In particular, the emission of two electrons from an atom—induced by the impact of a single photon, a charged particle or by a short laser pulse—has become the standard process for studies of dynamical electron correlations. Atoms and molecules exposed to laser fields that are comparable in intensity to the nuclear fields have extremely high probabilities for double ionization; this has been attributed to electron–electron interaction. Here we report a strong correlation between the magnitude and the direction of the momentum of two electrons that are emitted from an argon atom, driven by a femtosecond laser pulse (at 38 TW cm-2). Increasing the laser intensity causes the momentum correlation between the electrons to be lost, implying that a transition in the laser–atom coupling mechanism takes place.

A broad-application microchannel-plate detector system for advanced particle or photon detection tasks: large area imaging, precise multi-hit timing information and high detection rate

New applications for single particle and photon detection in many fields require both large area imaging performance and precise time information on each detected particle. Moreover, a very high data acquisition rate is desirable for most applications and eventually the detection and imaging of more than one particle arriving within a microsecond is required. Commercial CCD systems lack the timing information whereas other electronic microchannel plate (MCP) read-out schemes usually suffer from a low acquisition rate and complicated and sometimes costly read-out electronics. We have designed and tested a complete imaging system consisting of an MCP position readout with helical wire delaylines, single-unit amplifier box and PC-controlled time-to-digital converter (TDC) readout. The system is very flexible and can detect and analyse position and timing information at single particle rates beyond 1 MHz. Alternatively, multihit events can be collected and analysed at about 20 kHz rate. We discuss the advantages and applications of this technique and then focus on the detector’s ability to detect and analyse multiple hits. r 2002 Elsevier Science B.V. All rights reserved.

Ultrafast Probing of Core Hole Localization in N2

Although valence electrons are clearly delocalized in molecular bonding frameworks, chemists and physicists have long debated the question of whether the core vacancy created in a homonuclear diatomic molecule by absorption of a single x-ray photon is localized on one atom or delocalized over both. We have been able to clarify this question with an experiment that uses Auger electron angular emission patterns from molecular nitrogen after inner-shell ionization as an ultrafast probe of hole localization. The experiment, along with the accompanying theory, shows that observation of symmetry breaking (localization) or preservation (delocalization) depends on how the quantum entangled Bell state created by Auger decay is detected by the measurement.

Position sensitive anodes for MCP read-out using induced charge measurement

Abstract We investigate the method of an indirect detection of a MCP charge avalanche projected onto a resistive layer (G. Battistoni, et al., Nucl. Instr. and Meth., 202 (1982) 459). If the sheet resistance is favourable one can detect the charge cloud by the capacitive coupling to an anode structure a few millimetres behind the layer. The anode structure can be, for example, a wedge-and-strip electrode pattern (M. Unverzagt, Diplomarbeit, Universitat Frankfurt 1992, private communication) as it is used for directly collecting the electron avalanche from a MCP. Detection of the induced charge is beneficial in several respects. Firstly, image distortions produced by secondary electron mediated charge redistribution are eliminated. Secondly, the noise component due to quantized charge collection, commonly referred to as partition noise, is not present. In addition, the dielectric substrate can function both as an element of the vacuum enclosure and HV insulator, making the electrical connections easily accessible and the pattern operable at ground potential, independently of detector operating voltages. This technique can be used to simplify the electronic design requirements where varying high voltages are required at the detector input face such as plasma analysers, etc. It also has application in the manufacture of intensifier tubes (J. Barnstedt, M. Grewing, Nucl. Instr. and Meth., these proceedings) where the inclusion of a readout pattern inside the intensifier body with associated electrical feed-throughs can prove problematic. We will present data on the performance of such detection geometries using several types of charge division anode, and discuss the advantages compared with the “traditional” charge collecting method.

Multi-hit detector system for complete momentum balance in spectroscopy in molecular fragmentation processes

A multi-hit detector system has been developed capable of measuring the complete momentum vectors of all ionic fragments after the dissociation of complex molecules induced by photon, electron or ion impact. The fragments are collected in an electrostatic field and detected with a position-sensitive micro-channel plate detector using a fast timing delay-line readout. The detector has a position resolution better than 0.2 mm and can resolve fragments with arrival times separated by at least 5 ns in time. We illustrate the features of this new detector with first measurements for the collision

Fragmentation dynamics of CO(2)(3+) investigated by multiple electron capture in collisions with slow highly charged ions.

Fragmentation of highly charged molecular ions or clusters consisting of more than two atoms can proceed in a one step synchronous manner where all bonds break simultaneously or sequentially by emitting one ion after the other. We separated these decay channels for the fragmentation of CO(2)(3+) ions by measuring the momenta of the ionic fragments. We show that the total energy deposited in the molecular ion is a control parameter which switches between three distinct fragmentation pathways: the sequential fragmentation in which the emission of an O(+) ion leaves a rotating CO(2+) ion behind that fragments after a time delay, the Coulomb explosion and an in-between fragmentation--the asynchronous dissociation. These mechanisms are directly distinguishable in Dalitz plots and Newton diagrams of the fragment momenta. The CO(2)(3+) ions are produced by multiple electron capture in collisions with 3.2 keV/u Ar(8+) ions.

Complete photo-fragmentation of the deuterium molecule

All properties of molecules—from binding and excitation energies to their geometry—are determined by the highly correlated initial-state wavefunction of the electrons and nuclei. Details of these correlations can be revealed by studying the break-up of these systems into their constituents. The fragmentation might be initiated by the absorption of a single photon, by collision with a charged particle or by exposure to a strong laser pulse: if the interaction causing the excitation is sufficiently understood, the fragmentation process can then be used as a tool to investigate the bound initial state. The interaction and resulting fragment motions therefore pose formidable challenges to quantum theory. Here we report the coincident measurement of the momenta of both nuclei and both electrons from the single-photon-induced fragmentation of the deuterium molecule. The results reveal that the correlated motion of the electrons is strongly dependent on the inter-nuclear separation in the molecular ground state at the instant of photon absorption.

Fast position and time-resolved read-out of micro-channelplates with the delay-line technique for single-particle and photon-detection

Based on delay-line read-out methods of micro-channelplate (MCP) stacks we develop imaging system for single particle and photon spectroscopy. A complete system consists of an open MCP-detector with helical wire anode, specially designed front-end electronics and a stand alone PC-based TDC-system. We achieve a position resolution better than 0.1 mm and excellent linearity for open dimensions up to 100 mm, multi-hit operation, and detection rates up to 20 kiloEvents/sec in an event-listing mode or over 1 MegaCount/sec in a histogram mode. Both modes allow 2D position and time-of-flight (TOF) spectroscopy with approximately 1 nanosec TOF resolution. Furthermore, we currently test a delay-line anode on printed circuit that operates with image charge pick-up from a high-resistive collecting anode. With an image charge detection method this 3D-imaging technique can be applied to commercial sealed MCP single-photon detectors. While a simple high-resistive collection anode is placed inside the tube, a position sensitive pick-up electrode can be mounted next to it outside the vacuum wall.

K-shell photoionization of CO and N2: is there a link between the photoelectron angular distribution and the molecular decay dynamics?

We have used COLTRIMS to measure the angular distribution of electrons released from the K-shell of N2 and the carbon K-shell of CO by absorption of one linear polarized photon. For each ionization event which leads to two charged fragments we determine the angle of the photoelectron with respect to the fragment ion momenta. In addition we determine the charge state and energy of the molecular fragments. We find a breakdown of the axial recoil approximation for CO for kinetic energy releases below 10.2 eV, whereas for N2 that approximation is found to be valid for all fragment energies. Furthermore, the photoelectron emission spectrum for N2 is found to be the same for the molecular breakup channels producing N + N + and N + N ++ . (Some figures in this article are in colour only in the electronic version)

Sequential and nonsequential contributions to double ionization in strong laser fields

We demonstrate experimentally the difference between a sequential interaction of a femtosecond laser field with two electrons and a nonsequential process of double ionization mediated by electron-electron correlation. This is possible by observing the momentum distribution of doubly charged argon ions created in the laser field. In the regime of laser intensities where the nonsequential process dominates, an increase in laser power leads to an increase in the observed ion momenta. At the onset of the sequential process, however, a higher laser power leads to colder ions. The momentum distributions of the ions from the sequential process can be modelled by convolving the single-ionization distribution with itself.