P. Ludwig

Time-resolved 2-million-year-old supernova activity discovered in Earth’s microfossil record

Significance Massive stars, which terminate their evolution in a cataclysmic explosion called a type-II supernova, are the nuclear engines of galactic nucleosynthesis. Among the elemental species known to be produced in these stars, the radioisotope 60Fe stands out: This radioisotope has no natural, terrestrial production mechanisms; thus, a detection of 60Fe atoms within terrestrial reservoirs is proof for the direct deposition of supernova material within our solar system. We report, in this work, the direct detection of live 60Fe atoms in biologically produced nanocrystals of magnetite, which we selectively extracted from two Pacific Ocean sediment cores. We find that the arrival of supernova material on Earth coincides with the lower Pleistocene boundary (2.7 Ma) and that it terminates around 1.7 Ma. Massive stars (M≳10 M⊙), which terminate their evolution as core-collapse supernovae, are theoretically predicted to eject >10−5M⊙ of the radioisotope 60Fe (half-life 2.61 Ma). If such an event occurs sufficiently close to our solar system, traces of the supernova debris could be deposited on Earth. Herein, we report a time-resolved 60Fe signal residing, at least partially, in a biogenic reservoir. Using accelerator mass spectrometry, this signal was found through the direct detection of live 60Fe atoms contained within secondary iron oxides, among which are magnetofossils, the fossilized chains of magnetite crystals produced by magnetotactic bacteria. The magnetofossils were chemically extracted from two Pacific Ocean sediment drill cores. Our results show that the 60Fe signal onset occurs around 2.6 Ma to 2.8 Ma, near the lower Pleistocene boundary, terminates around 1.7 Ma, and peaks at about 2.2 Ma.

Plutonium Isotopes (239–241Pu) Dissolved in Pacific Ocean Waters Detected by Accelerator Mass Spectrometry: No Effects of the Fukushima Accident Observed

The concentration of plutonium (Pu) and the isotopic ratios of 240Pu to 239Pu and 241Pu to 239Pu were determined by accelerator mass spectrometry (AMS) in Pacific Ocean water samples (20 L each) collected in late 2012. The isotopic Pu ratios are important indicators of different contamination sources and were used to identify a possible release of Pu into the ocean by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. In particular, 241Pu is a well-suited indicator for a recent entry of Pu because 241Pu from fallout of nuclear weapon testings has already significantly decayed. A total of 10 ocean water samples were prepared at the Radiochemie München of the TUM and analyzed at the Vienna Environmental Research Laboratory (VERA). Several samples showed a slightly elevated 240Pu/239Pu ratio of up to 0.22 ± 0.02 compared to global fallout (240Pu/239Pu = 0.180 ± 0.007), whereas all measured 241Pu-to-239Pu ratios were consistent with nuclear weapon fallout (241Pu/239Pu < 2.4 × 10-3), which means that no impact from the Fukushima accident was detected. From the average 241Pu-to-239Pu ratio of 8-2+3 ×10-4 at a sampling station located at a distance of 39.6 km to FDNPP, the 1-σ upper limit for the FDNPP contribution to the 239Pu inventory in the water column was estimated to be 0.2%. Pu, with the signature of weapon-grade Pu was found in a single sample collected around 770 km off the west coast of the United States.

Assessment of 53Mn deposition on Earth via accelerator mass spectrometry

The 53Mn flux onto Earth is a quantity relevant for different extraterrestrial and astrophysical questions. It is a proxy for related fluxes, such as supernova-produced material or interplanetary dust particles. In this work, we performed a first attempt to assess the 53Mn flux by measuring the 53Mn/10Be isotopic ratio in a 1400 L sample of molten Antarctic snow by AMS (Accelerator Mass Spectrometry). Using the 10Be production rate in the atmosphere, an upper limit of 5.5 × 103 atoms cm-2 yr-1 was estimated for the deposition of extraterrestrial 53Mn. This result is compatible with one of the two discrepant values existing in the literature.

Measurement of the stellar Ni 58 ( n , γ ) Ni 59 cross section with accelerator mass spectrometry

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Characterization of primary and secondary magnetite in marine sediment by combining chemical and magnetic unmixing techniques

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Interstellar Fe-60 on the Surface of the Moon

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InterstellarFe60on the Surface of the Moon

(n,\gamma)^{59}

Search for superheavy elements with 292 A 310 in nature with accelerator mass spectrometry

Ni cross section was measured with a combination of the activation technique and accelerator mass spectrometry (AMS). The neutron activations were performed at the Karlsruhe 3.7 MV Van de Graaff accelerator using the quasi-stellar neutron spectrum at

The Ksar Ghilane 002 shergottite-The 100th registered Martian meteorite fragment

kT=25

Analytical method for the determination of Np and Pu in sea water by AMS with respect to the Fukushima accident

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