P. Sigalotti

Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet

Researchers demonstrate the FERMI free-electron laser operating in the high-gain harmonic generation regime, allowing high stability, transverse and longitudinal coherence and polarization control.

Two-colour pump–probe experiments with a twin-pulse-seed extreme ultraviolet free-electron laser

Exploring the dynamics of matter driven to extreme non-equilibrium states by an intense ultrashort X-ray pulse is becoming reality, thanks to the advent of free-electron laser technology that allows development of different schemes for probing the response at variable time delay with a second pulse. Here we report the generation of two-colour extreme ultraviolet pulses of controlled wavelengths, intensity and timing by seeding of high-gain harmonic generation free-electron laser with multiple independent laser pulses. The potential of this new scheme is demonstrated by the time evolution of a titanium-grating diffraction pattern, tuning the two coherent pulses to the titanium M-resonance and varying their intensities. This reveals that an intense pulse induces abrupt pattern changes on a time scale shorter than hydrodynamic expansion and ablation. This result exemplifies the essential capabilities of the jitter-free multiple-colour free-electron laser pulse sequences to study evolving states of matter with element sensitivity.

Towards jitter-free pump-probe measurements at seeded free electron laser facilities.

X-ray free electron lasers (FEL) coupled with optical lasers have opened unprecedented opportunities for studying ultrafast dynamics in matter. The major challenge in pump-probe experiments using FEL and optical lasers is synchronizing the arrival time of the two pulses. Here we report a technique that benefits from the seeded-FEL scheme and uses the optical seed laser for nearly jitter-free pump-probe experiments. Timing jitter as small as 6 fs has been achieved and confirmed by measurements of FEL-induced transient reflectivity changes of Si3N4 using both collinear and non-collinear geometries. Planned improvements of the experimental set-up are expected to further reduce the timing jitter between the two pulses down to fs level.

The FERMI free-electron lasers

FERMI is a seeded free-electron laser (FEL) facility located at the Elettra laboratory in Trieste, Italy, and is now in user operation with its first FEL line, FEL-1, covering the wavelength range between 100 and 20 nm. The second FEL line, FEL-2, a high-gain harmonic generation double-stage cascade covering the wavelength range 20-4 nm, has also completed commissioning and the first user call has been recently opened. An overview of the typical operating modes of the facility is presented.

Single-shot spectro-temporal characterization of XUV pulses from a seeded free-electron laser

Intense ultrashort X-ray pulses produced by modern free-electron lasers (FELs) allow one to probe biological systems, inorganic materials and molecular reaction dynamics with nanoscale spatial and femtoscale temporal resolution. These experiments require the knowledge, and possibly the control, of the spectro-temporal content of individual pulses. FELs relying on seeding have the potential to produce spatially and temporally fully coherent pulses. Here we propose and implement an interferometric method, which allows us to carry out the first complete single-shot spectro-temporal characterization of the pulses, generated by an FEL in the extreme ultraviolet spectral range. Moreover, we provide the first direct evidence of the temporal coherence of a seeded FEL working in the extreme ultraviolet spectral range and show the way to control the light generation process to produce Fourier-limited pulses. Experiments are carried out at the FERMI FEL in Trieste.

Experimental setups for FEL-based four-wave mixing experiments at FERMI

The recent advent of free-electron laser (FEL) sources is driving the scientific community to extend table-top laser research to shorter wavelengths adding elemental selectivity and chemical state specificity. Both a compact setup (mini-TIMER) and a separate instrument (EIS-TIMER) dedicated to four-wave-mixing (FWM) experiments has been designed and constructed, to be operated as a branch of the Elastic and Inelastic Scattering beamline: EIS. The FWM experiments that are planned at EIS-TIMER are based on the transient grating approach, where two crossed FEL pulses create a controlled modulation of the sample excitations while a third time-delayed pulse is used to monitor the dynamics of the excited state. This manuscript describes such experimental facilities, showing the preliminary results of the commissioning of the EIS-TIMER beamline, and discusses original experimental strategies being developed to study the dynamics of matter at the fs-nm time-length scales. In the near future such experimental tools will allow more sophisticated FEL-based FWM applications, that also include the use of multiple and multi-color FEL pulses.

Ultrafast laser synchronization at the FERMI@Elettra FEL

Modern VUV and X-ray Free Electron Laser (FEL) facilities contain a number of ultrafast lasers (like photoinjector, seed and pump-probe lasers) whose performance is crucial for the generated FEL light quality as well as for the accuracy of the time resolved measurements performed using the FEL pulses. One of the very important laser related aspects, especially at seeded FELs, is the ability to precisely lock the ultrafast laser systems to the master clock signal, keeping the timing jitter and drifts of the generated pulses with respect to the machine timing as low as possible. The aim of this work is to review the main sources of timing jitter and drifts and present the schemes and solutions developed at FERMI for their characterization and compensation. The paper will first introduce a general scheme showing the architecture of the laser locking system developed for FERMI. Both the radio-frequency (RF) locking and the advanced balanced optical cross correlator electronics and optical setup design are described, together with data on the laser oscillator locking performance obtained in different modalities. Cross correlation measurements indicating the contribution of the ultrafast regenerative amplifier and optical beam transport part to the overall temporal jitter of the amplified ultrashort pulses arriving at destination are presented. The paper also includes examples of the influence of improved laser timing jitter and drifts on the seeded FEL performance and discusses foreseen future developments.

DFG-based mid-IR laser system for muounic-hydrogen spectroscopy

The goal of this work is to prove the feasibility of building a laser system that can generate mid-infrared radiation with the parameters required for the measurement of the hyperfine splitting in the ground state of the mounic hydrogen spectroscopy. The first experimental results of a very straightforward scheme that, to our knowledge, has not been considered in the literature, are presented. We study a laser test bench system emitting nanosecond pulses of infrared tunable radiation in the spectral range 6.78 μm with high energy and narrow line-width, based on direct difference frequency generation (DFG), in non-oxide nonlinear crystals, using as pump lasers a single-mode Nd:YAG laser and tunable narrowbandwidth Cr:forsterite laser. The investigated system is based on lithium thioindate (LiInS2) and silver thiogallate (AgGaS2) crystals cut for type II difference frequency generation. The pulses of the Nd:YAG laser (1,064 μm) are combined with the pulses at ~ 1.262 μm of the Cr:forsterite laser through a dichroic mirror and sent to the nonlinear crystals in different optical geometries. The generated radiation reaches an output energy up to 80 μJ in a single pass optical geometry, has 10 ns long pulses at 50 Hz frequency repetition rate and is tunable in the range 6595 – 6895 nm. These first results prove the suitability of such an approach for building the laser system for the muonic-hydrogen experiment.

Status and achievements at FERMI@Elettra: the first double cascade seeded EUV-SXR FEL facility open to users

FERMI@Elettra is the first seeded VUV/soft X-ray FEL source. It is composed of two undulatory chains: the low energy branch (FELl) covering the wavelength range from 20 nm up to 100 nm, and the high energy branch (FEL2, employing a double stage cascade), covering the wavelength range from 4 nm up to 20 nm. At the end of 2012 FELl has been opened to external users while FEL2 has been turned on for the first time having demonstrated that a double cascade scheme is suitable for generating high intensity coherent FEL radiation. In this paper we will share our experience and will show our most recent results for both FERMI FELl and FEL2 sources. We will also present a brand new machine scheme that allows to perform two-colour pump and probe experiments as well as the first experimental results.

FERMI@Elettra, a seeded free electron laser source for a broad scientific user program

After less than two years of commissioning the FERMI@Elettra free electron laser is now entering into the operation phase and is providing light to the first user experiments. To reach the final ambitious goals of providing high power coherent pulses with fundamental wavelengths down to 4 nm, the system will need further studies and additional commissioning time in 2011 when fine tuning of the major systems such as the electron gun and the main accelerator will take place. Nevertheless, FERMI is already able to provide light with unique characteristics allowing Users to perform experiments not possible with other facilities. Based on a 1.5 GeV electron linear accelerator, FERMI@Elettra has two seeded FEL lines that cover the whole spectral range from 100 nm down to 4 nm with fully coherent pulses. The use of the high gain harmonic generation scheme initiated by a tunable laser in the UV allows FERMI to produce light characterized by both transverse and full temporal coherence. The use of specially designed undulators allows full control of the FEL polarization and can be continuously varied from linear to circular in any orientation or ellipticity. Here we will report about the first results and the future plans for FERMI@Elettra.