Pablo I. R. Pincheira

Observation of Lévy distribution and replica symmetry breaking in random lasers from a single set of measurements

Random lasers have been recently exploited as a photonic platform for studies of complex systems. This cross-disciplinary approach opened up new important avenues for the understanding of random-laser behavior, including Lévy-type distributions of strong intensity fluctuations and phase transitions to a photonic spin-glass phase. In this work, we employ the Nd:YBO random laser system to unveil, from a single set of measurements, the physical origin of the complex correspondence between the Lévy fluctuation regime and the replica-symmetry-breaking transition to the spin-glass phase. A novel unexpected finding is also reported: the trend to suppress the spin-glass behavior for high excitation pulse energies. The present description from first principles of this correspondence unfolds new possibilities to characterize other random lasers, such as random fiber lasers, nanolasers and small lasers, which include plasmonic-based, photonic-crystal and bio-derived nanodevices. The statistical nature of the emission provided by random lasers can also impact on their prominent use as sources for speckle-free laser imaging, which nowadays represents one of the most promising applications of random lasers, with expected progress even in cancer research.

Observation of photonic paramagnetic to spin-glass transition in a specially designed TiO 2 particle-based dye-colloidal random laser

Colloidal-based random lasers (RLs) are highly efficient and have been exploited in a wide range of geometries. However, in the particular case of ethanol solutions of rhodamines and TiO2 particles, the RL behavior is quite unstable due to the fast precipitation of the particles. In this Letter, specially designed amorphous TiO2 particles were synthesized by a sol-gel method, preventing the degradation of the RL for long operating lifetimes of over 105 shots. As a consequence, this modified colloidal RL allowed the observation of a clear replica-symmetry-breaking phase transition from the paramagnetic fluorescent to spin-glass RL behavior, which has not been observed in the system with nonfunctionalized TiO2 particles.By using specially designed nanoparticles scatterers which prevents photodegradation of the dye, we present clear demonstration of replica symmetry break and a photonic paramagnetic to spin-glass phase transition in a random laser operating in the incoherent feedback regime based on ethanol solution of Rhodamine 6G and amorphous TiO2 nanoparticles.

Turbulence hierarchy in a random fibre laser.

Turbulence is a challenging feature common to a wide range of complex phenomena. Random fibre lasers are a special class of lasers in which the feedback arises from multiple scattering in a one-dimensional disordered cavity-less medium. Here we report on statistical signatures of turbulence in the distribution of intensity fluctuations in a continuous-wave-pumped erbium-based random fibre laser, with random Bragg grating scatterers. The distribution of intensity fluctuations in an extensive data set exhibits three qualitatively distinct behaviours: a Gaussian regime below threshold, a mixture of two distributions with exponentially decaying tails near the threshold and a mixture of distributions with stretched-exponential tails above threshold. All distributions are well described by a hierarchical stochastic model that incorporates Kolmogorov’s theory of turbulence, which includes energy cascade and the intermittence phenomenon. Our findings have implications for explaining the remarkably challenging turbulent behaviour in photonics, using a random fibre laser as the experimental platform.

Tunable ultraviolet and blue light generation from Nd:YAB random laser bolstered by second-order nonlinear processes.

Ultraviolet and blue light were obtained by nonlinear frequency conversion in a random laser (RL) based on Nd0.10Y0.90Al3(BO3)4 nanocrystalline powder. RL operation at 1062 nm, due to the 4F3/2 → 4I11/2 transition of neodymium ions (Nd3+), was achieved by exciting the Nd3+ with a tunable beam from 680 to 920 nm covering the ground state absorption transitions to the 4F9/2, (4F7/2,4S3/2), (4F5/2,2H9/2), and 4F3/2 states. Light from 340 to 460 nm was obtained via the second-harmonic generation of the excitation beam while tunable blue light, from 417 to 486 nm, was generated by self-sum-frequency mixing between the excitation beam and the RL emission.

Glassy behavior in a one-dimensional continuous-wave erbium-doped random fiber laser

Anderson S. L. Gomes, ∗ Bismarck C. Lima, Pablo I. R. Pincheira, André L. Moura, 2 Mathieu Gagné, Raman Kashyap, Ernesto P. Raposo, and Cid B. de Araújo Departamento de F́ısica, Universidade Federal de Pernambuco, 50670-901, Recife-PE, Brazil Grupo de F́ısica da Matéria Condensada, Núcleo de Ciências Exatas NCEx, Campus Arapiraca, Universidade Federal de Alagoas, 57309-005, Arapiraca-AL, Brazil Fabulas Laboratory, Department of Engineering Physics, Department of Electrical Engineering, Polytechnique Montreal, Montreal, H3C 3A7, Canada Laboratório de F́ısica Teórica e Computacional, Departamento de F́ısica, Universidade Federal de Pernambuco, 50670-901, Recife-PE, Brazil (Dated: January 8, 2016)

Observation of Lévy statistics in one-dimensional erbium-based random fiber laser

We report on measurements of the statistical fluctuations of the output intensity in a continuous-wave-pumped erbium-doped one-dimensional random fiber laser (RFL), with specially designed Bragg grating scatterers. Transitions from Gaussian to Levy-like and back to the Gaussian regime, similar to those observed in three-dimensional random lasers, are described as the input excitation power increases from below to above the RFL threshold. Our results are consistent with theoretical predictions for the sequence of statistical regimes of output intensity in random laser systems. We also discuss experimental and theoretical connections with the photonic spin-glass behavior of the erbium-doped RFL, which displays a replica-symmetry-breaking phase above the threshold.

Replica Symmetry Breaking in the Photonic Ferromagneticlike Spontaneous Mode-Locking Phase of a Multimode Nd:YAG Laser

We demonstrate the replica symmetry breaking (RSB) phenomenon in the spontaneous mode-locking regime of a multimode Q-switched Nd:YAG laser. The underlying mechanism is quite distinct from that of the RSB recently observed in random lasers. Here, there is no random medium and the phase is not glassy with incoherently oscillating modes as in random lasers. Instead, in each pulse a specific subset of longitudinal modes are activated in a nondeterministic way, whose coherent oscillation dominates and frustrates the others. The emergence of RSB coincides with the onset of ultrashort pulse generation typical of the spontaneous mode-locking regime, both occurring at the laser threshold. On the other hand, when high losses are introduced, RSB is inhibited and only the amplified stimulated emission with replica symmetry is observed. Our results disclose the only theoretically predicted photonic phase with RSB that remained unobserved so far.The recent reports of the replica symmetry breaking (RSB) phenomenon in photonic experiments [1-5] boosted the understanding of the role of disorder in multimode lasers, as well as helped to settle enlightening connections [6-13] with the statistical physics of complex systems. RSB manifests when identically-prepared system replicas reach distinct states, yielding different measures of observable quantities [14]. Here we demonstrate the RSB in the spontaneous mode-locking regime of a conventional multimode Nd:YAG laser in a closed cavity. The underlying mechanism is quite distinct from that of the RSB spinglass phase in cavityless random lasers with incoherently-oscillating modes. Here, a specific nonuniform distribution of the gain takes place in each pulse, and frustration is induced since the coherent oscillation of a given subset of longitudinal modes dominates and simultaneously inhibits the others. Nevertheless, when high losses are introduced only the replica-symmetric amplified stimulation emission is observed. We therefore suggest that the RSB transition can be used as an identifier of the threshold in standard multimode lasers, as recently proposed and demonstrated for random lasers [1,2].