R. A. Buhrman

Ultrafine metal particles

In this paper we present a novel and versatile technique for the production of ultrafine metal particles by evaporation from a temperature‐regulated oven containing a reduced atmosphere of an inert gas. An extensive investigation of particles of oxidized Al, with diameters of 3 to 6 nm, has been performed. We have also studied ultrafine particles of Mg, Zn, and Sn produced in the same manner. A supplementing investigation has been carried out for particles of Cr, Fe, Co, Ni, Cu, and Ga, as well as larger Al particles, produced by ’’conventional’’ inert‐gas evaporation from a resistive filament. Diameter as a function of evaporation rate, inert‐gas pressure, and the kind of inert gas are reported. Crystalline particles smaller than 20 nm look almost spherical in the electron microscope, while larger ones often display pronounced crystal habit. Size distributions have been investigated in detail, and consistently the logarithm of the particle diameter has a Gaussian distribution to a high precision for the ...

Current-driven magnetization reversal and spin-wave excitations in Co /Cu /Co pillars

Using thin film pillars approximately 100 nm in diameter, containing two Co layers of different thicknesses separated by a Cu spacer, we examine the process by which the scattering from the ferromagnetic layers of spin-polarized currents flowing perpendicular to the layers causes controlled reversal of the moment direction in the thin Co layer. The well-defined geometry permits a quantitative analysis of this spin-transfer effect, allowing tests of competing theories for the mechanism and also new insight concerning magnetic damping. When large magnetic fields are applied, the spin-polarized current no longer fully reverses the magnetic moment, but instead stimulates spin-wave excitations.

Microwave oscillations of a nanomagnet driven by a spin-polarized current

The recent discovery that a spin-polarized electrical current can apply a large torque to a ferromagnet, through direct transfer of spin angular momentum, offers the possibility of manipulating magnetic-device elements without applying cumbersome magnetic fields. However, a central question remains unresolved: what type of magnetic motions can be generated by this torque? Theory predicts that spin transfer may be able to drive a nanomagnet into types of oscillatory magnetic modes not attainable with magnetic fields alone, but existing measurement techniques have provided only indirect evidence for dynamical states. The nature of the possible motions has not been determined. Here we demonstrate a technique that allows direct electrical measurements of microwave-frequency dynamics in individual nanomagnets, propelled by a d.c. spin-polarized current. We show that spin transfer can produce several different types of magnetic excitation. Although there is no mechanical motion, a simple magnetic-multilayer structure acts like a nanoscale motor; it converts energy from a d.c. electrical current into high-frequency magnetic rotations that might be applied in new devices including microwave sources and resonators.

Spin-Torque Switching with the Giant Spin Hall Effect of Tantalum

Giant Spin Hall One of the primary challenges in the field of spin-electronics, which exploits the electrons spin rather than its charge, is to create strong currents of electrons with polarized spins. One way to do this is to use a ferromagnet as a polarizer, a principle used in magnetic tunnel junctions; however, these devices suffer from reliability problems. An alternative is the spin Hall effect, where running a charge current through a material generates a spin current in the transverse direction, but the efficiency of this process tends to be small. Liu et al. (p. 555) now show that the spin Hall effect in Tantalum in its high-resistance β phase generates spin currents strong enough to induce switching of the magnetization of an adjacent ferromagnet; at the same time, Ta does not cause energy dissipation in the ferromagnet. These properties allowed efficient and reliable operation of a prototype three-terminal device. Tantalum is found to generate strong spin currents that can induce switching of ferromagnets efficiently and reliably. Spin currents can apply useful torques in spintronic devices. The spin Hall effect has been proposed as a source of spin current, but its modest strength has limited its usefulness. We report a giant spin Hall effect (SHE) in β-tantalum that generates spin currents intense enough to induce efficient spin-torque switching of ferromagnets at room temperature. We quantify this SHE by three independent methods and demonstrate spin-torque switching of both out-of-plane and in-plane magnetized layers. We furthermore implement a three-terminal device that uses current passing through a tantalum-ferromagnet bilayer to switch a nanomagnet, with a magnetic tunnel junction for read-out. This simple, reliable, and efficient design may eliminate the main obstacles to the development of magnetic memory and nonvolatile spin logic technologies.

Current-induced switching of perpendicularly magnetized magnetic layers using spin torque from the spin Hall effect.

The spin Hall effect (SHE) generates spin currents within nonmagnetic materials. Previously, studies of the SHE have been motivated primarily to understand its fundamental origin and magnitude. Here we demonstrate, using measurement and modeling, that in a Pt/Co bilayer with perpendicular magnetic anisotropy the SHE can produce a spin transfer torque that is strong enough to efficiently rotate and reversibly switch the Co magnetization, thereby providing a new strategy both to understand the SHE and to manipulate magnets. We suggest that the SHE torque can have a similarly strong influence on current-driven magnetic domain wall motion in Pt/ferromagnet multilayers. We estimate that in optimized devices the SHE torque can switch magnetic moments using currents comparable to those in magnetic tunnel junctions operated by conventional spin-torque switching, meaning that the SHE can enable magnetic memory and logic devices with similar performance but simpler architecture than the current state of the art.

Spin transfer torque devices utilizing the giant spin Hall effect of tungsten

We report a giant spin Hall effect in β-W thin films. Using spin torque induced ferromagnetic resonance with a β-W/CoFeB bilayer microstrip, we determine the spin Hall angle to be |θSHβ-W|=0.30±0.02, large enough for an in-plane current to efficiently reverse the orientation of an in-plane magnetized CoFeB free layer of a nanoscale magnetic tunnel junction adjacent to a thin β-W layer. From switching data obtained with such 3-terminal devices, we independently determine |θSHβ-W|=0.33±0.06. We also report variation of the spin Hall switching efficiency with W layers of different resistivities and hence of variable (α and β) phase composition.

Spin-torque ferromagnetic resonance induced by the spin Hall effect.

We demonstrate that the spin Hall effect in a thin film with strong spin-orbit scattering can excite magnetic precession in an adjacent ferromagnetic film. The flow of alternating current through a Pt/NiFe bilayer generates an oscillating transverse spin current in the Pt, and the resultant transfer of spin angular momentum to the NiFe induces ferromagnetic resonance dynamics. The Oersted field from the current also generates a ferromagnetic resonance signal but with a different symmetry. The ratio of these two signals allows a quantitative determination of the spin current and the spin Hall angle.

Spin-polarized current switching of a Co thin film nanomagnet

A thin film Co nanomagnet in the shape of an elongated hexagon has been incorporated in a vertical device structure consisting of the nanomagnet and a thin Cu spacer layer formed on top of a thick Co film. The spin-polarized current flowing between the nanomagnet and the Co film is used to abruptly switch the magnetic alignment of the nanomagnet relative to that of the thick Co layer by the transfer of spin angular momentum from the conduction electrons to the nanomagnet moment. The shape anisotropy in the nanomagnet promotes the single domain behavior required for nonvolatile memory applications.

Magnetic vortex oscillator driven by d.c. spin-polarized current

Transfer of angular momentum from a spin-polarized current to a ferromagnet provides an efficient means to control the magnetization dynamics of nanomagnets. A peculiar consequence of this spin torque, the ability to induce persistent oscillations in a nanomagnet by applying a d.c. current, has previously been reported only for spatially uniform nanomagnets. Here, we demonstrate that a quintessentially non-uniform magnetic structure, a magnetic vortex, isolated within a nanoscale spin-valve structure, can be excited into persistent microwave-frequency oscillations by a spin-polarized d.c. current. Comparison with micromagnetic simulations leads to identification of the oscillations with a precession of the vortex core. The oscillations, which can be obtained in essentially zero magnetic field, exhibit linewidths that can be narrower than 300 kHz at ∼1.1 GHz, making these highly compact spin-torque vortex-oscillator devices potential candidates for microwave signal-processing applications, and a powerful new tool for fundamental studies of vortex dynamics in magnetic nanostructures.

Measurement of the spin-transfer-torque vector in magnetic tunnel junctions

The transfer of spin angular momentum from a spin-polarized current to a ferromagnet can generate sufficient torque to reorient the magnet’s moment. This torque could enable the development of efficient electrically actuated magnetic memories and nanoscale microwave oscillators. Yet difficulties in making quantitative measurements of the spin-torque vector have hampered understanding. Here we present direct measurements of both the magnitude and direction of the spin torque in magnetic tunnel junctions, the type of device of primary interest for applications. At low bias V, the differential torque dτ/dV lies in the plane defined by the electrode magnetizations, and its magnitude is in excellent agreement with recent predictions for near-perfect spin-polarized tunnelling. We find that the strength of the in-plane differential torque remains almost constant with increasing bias, despite a substantial decrease in the device magnetoresistance, and that with bias the torque vector also rotates out of the plane.