R. C. Pardo

Laser Spectroscopic Determination of the ^6He Nuclear Charge Radius

We have performed precision laser spectroscopy on individual 6He (t(1/2)=0.8 s) atoms confined and cooled in a magneto-optical trap, and measured the isotope shift between 6He and 4He to be 43 194.772+/-0.056 MHz for the 2(3)S1-3(3)P2 transition. Based on this measurement and atomic theory, the nuclear charge radius of 6He is determined for the first time in a method independent of nuclear models to be 2.054+/-0.014 fm. The result is compared with the values predicted by a number of nuclear structure calculations and tests their ability to characterize this loosely bound halo nucleus.

A Shorter 146Sm Half-Life Measured and Implications for 146Sm-142Nd Chronology in the Solar System

A New Lease on Half-Life Radiometric dating relies on measuring the abundance of long-lived radionuclides relative to the abundance of their radiogenic decay products—a process determined by the original radionuclides half-life. For primordial radionuclides that decay slowly, such as 146Sm decaying to 142Nd, this method provides the timing of some of the earliest processes in solar system history. Using accelerator mass spectrometry, Kinoshita et al. (p. 1614) provide a revised estimate for the 146Sm half-life of ∼68.7 million years, which is 30% shorter than the previously accepted value. This shorter half-life suggests that reductions need to be made in the estimated ages for differentiation of Earths mantle and the solidification of the Moons magma ocean and for other more recent processes. Mantle differentiation of Earth, the Moon, and Mars occurred earlier and over a shorter time scale than previously estimated. The extinct p-process nuclide 146Sm serves as an astrophysical and geochemical chronometer through measurements of isotopic anomalies of its α-decay daughter 142Nd. Based on analyses of 146Sm/147Sm α-activity and atom ratios, we determined the half-life of 146Sm to be 68 ± 7 (1σ) million years, which is shorter than the currently used value of 103 ± 5 million years. This half-life value implies a higher initial 146Sm abundance in the early solar system, (146Sm/144Sm)0 = 0.0094 ± 0.0005 (2σ), than previously estimated. Terrestrial, lunar, and martian planetary silicate mantle differentiation events dated with 146Sm-142Nd converge to a shorter time span and in general to earlier times, due to the combined effect of the new 146Sm half-life and (146Sm/144Sm)0 values.

81Kr in the Great Artesian Basin, Australia: a new method for dating very old groundwater

Abstract The measurement of cosmogenic 81Kr (t1/2=(2.29±0.11)×105 yr) has been proposed for many years as a reliable tool for groundwater dating in the range from 105 to 106 yr. In this paper, we report on the first use of 81Kr to determine the age of groundwater from four wells in the Great Artesian Basin in Australia. As the concentration of 81Kr in old groundwater is only a few hundred atoms per liter, krypton was extracted from large (16 000 l) groundwater samples and was analyzed for the isotopic abundance of 81Kr by accelerator mass spectrometry (AMS) with a cyclotron. 81Kr/Kr isotope ratios of (1.54±0.22)×10−13, (1.78±0.26)×10−13, (2.19±0.28)×10−13 and (2.63±0.32)×10−13, respectively, were measured for these samples. It is reasonable to assume that krypton dissolved in surface water in contact with the atmosphere has the known atmospheric 81Kr/Kr ratio of (5.20±0.40)×10−13. The observed reduction of isotope ratios in the groundwater samples can then be interpreted as being due to radioactive decay since recharge. This results in respective groundwater ages of: (4.02±0.51)×105 yr, (3.54±0.50)×105 yr, (2.87±0.38)×105 yr and (2.25±0.42)×105 yr. The main emphasis of this paper lies on the description of the analytic procedure to extract a reliable 81Kr signal from large groundwater samples. Although the uncertainties are still relatively large (primarily due to counting statistics caused by the low cyclotron AMS efficiency), the new technique enabled for the first time a definite determination of residence times for old groundwater with 81Kr. It thus confirms the hope that this radionuclide may become a very valuable tool for groundwater dating.

Influence of Nuclear Structure on Sub-Barrier Hindrance in Ni + Ni Fusion

Fusion-evaporation cross sections for

Production of radioactive ion beams using the in-flight technique

^{64}

Measurement of 81Kr in the atmosphere

Ni+

Half-life of 60Fe

^{64}

Ion plasma sputtering as a method of introducing solid material into an electron cyclotron resonance ion source

Ni have been measured down to the 10 nb level. For fusion between two open-shell nuclei, this is the first observation of a maximum in the

Long-lived noble gas radionuclides

S

Hindrance of heavy-ion fusion at extreme sub-barrier energies in open-shell colliding systems

-factor, which signals a strong sub-barrier hindrance. A comparison with the