R. Haight

Nuclear energy generation and waste transmutation using an accelerator-driven intense thermal neutron source

We describe a new approach for commercial nuclear energy production without a long-term high-level waste stream and for transmutation of both fission product and higher actinide commercial nuclear waste using a thermal flux of accelerator-produced neutrons in the 1016 n/cm2s range. Continuous neutron fluxes at this intensity, which is approximately 100 times larger than is typically available in a large scale thermal reactor, appear practical, owing to recent advances in proton linear accelerator technology and to the spallation target-moderator design presented here. This large flux of thermal neutrons makes possible a waste inventory in the transmutation system which is smaller by about a factor of 100 than competing concepts. The accelerator allows the system to operate well below criticality so that the possibility for a criticality accident is eliminated. No control rods are required. The successful implementation of this new method for energy generation and waste transmutation would eliminate the need for nuclear waste storage on a geologic time scale. The production of nuclear energy from 232Th or 238U is used to illustrate the general principles of commercial nuclear energy, production without long-term high-level waste. There appears to be sufficient thorium to meet the worlds energy needs for many millenia.

A fission ionization detector for neutron flux measurements at a spallation source

Abstract The construction of a neutron flux monitor that can measure absolute neutron intensities in the neutron energy range from below 1 MeV to over 500 MeV is described. The detector consists of an ionization chamber with several thin deposits of fissionable material. The ionization chamber is thin enough that it does not significantly affect the neutron beam and may be left in the neutron flight path during experimental measurements to continuously monitor the beam flux. The use of this monitor at the continuous-energy spallation neutron source at the WNR target area at LAMPF is described.

A detector for (n,γ) cross-section measurements at a spallation neutron source

Abstract The quest for improved neutron capture cross-sections for advanced reactor concepts, transmutation of radioactive wastes as well as for astrophysical scenarios of neutron capture nucleosynthesis has motivated new experimental efforts based on modern techniques. Recent measurements in the keV region have shown that a 4 π BaF 2 detector represents an accurate and versatile instrument for such studies. The present work deals with the potential of such a 4 π BaF 2 detector in combination with spallation neutron sources, which offer large neutron fluxes over a wide energy range. Detailed Monte Carlo simulations with the GEANT package have been performed to investigate the critical backgrounds at a spallation facility, to optimize the detector design, and to discuss alternative solutions.

Background identification and suppression for the measurement of (n,γ) reactions with the DANCE array at LANSCE

Abstract In the commissioning phase of the DANCE project (Detector for Advanced Neutron Capture Experiments) measurements have been performed with special emphasis on the identification and suppression of possible backgrounds for the planned (n,γ) experiments. This report describes several background sources, observed in the experiment or anticipated from simulations, which will need to be suppressed in this and in similar detectors that are planned at other facilities. First successes are documented in the suppression of background from scattered neutrons captured in the detector as well as from the internal radiation. Experimental results and simulations using the GEANT code are compared.

Acquisition-analysis system for the DANCE (detector for advanced neutron capture experiments) BaF/sub 2/ gamma-ray calorimeter

The DANCE detector is a segmented 4/spl pi/ gamma-ray calorimeter for measuring (n, /spl gamma/) and (n,fission) cross-sections of stable and long-lived radioactive isotopes. DANCE uses waveform digitization to acquire the basic gamma-ray data, which maximizes the information available for event reconstruction, but has necessitated the development of several techniques for handling the resulting high data rates. This paper describes the basic experimental requirements for acquisition and analysis and how we have satisfied these requirements primarily by extending existing acquisition and analysis frameworks.

The C 14 ( n , γ ) cross section between 10 keV and 1 MeV

The neutron capture cross section of 14C is of relevance for several nucleosynthesis scenarios such as inhomogeneous Big Bang models, neutron induced CNO cycles, and neutrino driven wind models for the r process. The 14C(n,gamma) reaction is also important for the validation of the Coulomb dissociation method, where the (n,gamma) cross section can be indirectly obtained via the time-reversed process. So far, the example of 14C is the only case with neutrons where both, direct measurement and indirect Coulomb dissociation, have been applied. Unfortunately, the interpretation is obscured by discrepancies between several experiments and theory. Therefore, we report on new direct measurements of the 14C(n,gamma) reaction with neutron energies ranging from 20 to 800 keV.

Characterization of a novel, short pulse laser-driven neutron source

We present a full characterization of a short pulse laser-driven neutron source. Neutrons are produced by nuclear reactions of laser-driven ions deposited in a secondary target. The emission of neutrons is a superposition of an isotropic component into 4π and a forward directed, jet-like contribution, with energies ranging up to 80 MeV. A maximum flux of 4.4 × 109 neutrons/sr has been observed and used for fast neutron radiography. On-shot characterization of the ion driver and neutron beam has been done with a variety of different diagnostics, including particle detectors, nuclear reaction, and time-of-flight methods. The results are of great value for future optimization of this novel technique and implementation in advanced applications.

Correlated neutron emissions from 252Cf

Abstract This paper presents new experimental results of correlated, prompt neutron emission from the spontaneous fission of 252Cf. Specifically, we present correlated-neutron emission probabilities and average energies for two detected neutrons as a function of the angle between the two neutrons. Experimental results are compared to several Monte Carlo models that include the number, energy, and angular distributions of prompt neutrons from fission.

Neutron imaging with the short-pulse laser driven neutron source at the Trident laser facility

Emerging approaches to short-pulse laser-driven neutron production offer a possible gateway to compact, low cost, and intense broad spectrum sources for a wide variety of applications. They are based on energetic ions, driven by an intense short-pulse laser, interacting with a converter material to produce neutrons via breakup and nuclear reactions. Recent experiments performed with the high-contrast laser at the Trident laser facility of Los Alamos National Laboratory have demonstrated a laser-driven ion acceleration mechanism operating in the regime of relativistic transparency, featuring a volumetric laser-plasma interaction. This mechanism is distinct from previously studied ones that accelerate ions at the laser-target surface. The Trident experiments produced an intense beam of deuterons with an energy distribution extending above 100 MeV. This deuteron beam, when directed at a beryllium converter, produces a forward-directed neutron beam with ∼5 × 109 n/sr, in a single laser shot, primarily due to ...

The 59Co(n,xα) Reaction from 5 to 50 MeV

Alpha-particle production cross sections and spectra produced by neutron bombardment of 59Co are measured at 30, 60, 90, and 135 deg over the neutron energy range from 5 to 50 MeV. A source of neut...