R. M. Stevenson

Quantum memories : a review based on the European integrated project "Qubit Applications (QAP)"

AbstractWe perform a review of various approaches to the implementation of quantum memories, with an emphasis on activities within the quantum memory sub-project of the EU integrated project “Qubit Applications”. We begin with a brief overview over different applications for quantum memories and different types of quantum memories. We discuss the most important criteria for assessing quantum memory performance and the most important physical requirements. Then we review the different approaches represented in “Qubit Applications” in some detail. They include solid-state atomic ensembles, NV centers, quantum dots, single atoms, atomic gases and optical phonons in diamond. We compare the different approaches using the discussed criteria.

Inversion of exciton level splitting in quantum dots

The demonstration of degeneracy of exciton spin states is an important step toward the production of entangled photon pairs from the biexciton cascade. We measure the fine structure of exciton and biexciton states for a large number of single InAs quantum dots in a GaAs matrix; the energetic splitting of the horizontally and vertically polarized components of the exciton doublet is shown to decrease as the exciton confinement decreases, crucially passing through zero and changing sign. Thermal annealing is shown to reduce the exciton confinement, thereby increasing the number of dots with splitting close to zero.

Electric-field-induced coherent coupling of the exciton states in a single quantum dot

The ability to generate entangled photon pairs from a quantum dot critically depends on the size of the fine-structure splitting of its exciton states. A demonstration of the ability to tune this splitting with an electric field represents a promising step in the use of quantum dots to generate entangled photon pairs on demand.

Magnetic-field-induced reduction of the exciton polarization splitting in InAs quantum dots

By the application of an in-plane magnetic field, we demonstrate control of the fine structure polarization splitting of the exciton emission lines in individual InAs quantum dots. The selection of quantum dots with certain barrier composition and confinement energies is found to determine the magnetic field dependent increase or decrease of the separation of the bright exciton emission lines, and has enabled the splitting to be tuned to zero within the resolution of our experiments. Observed behavior allows us to determine g factors and exchange splittings for different types of dots.

Coherence of an entangled exciton-photon state.

We study the effect of the exciton fine-structure splitting on the polarization entanglement of photon pairs produced by the biexciton cascade in a quantum dot. Entanglement persists despite separations between the intermediate energy levels of up to 4 microeV. Measurements show that entanglement of the photon pair is robust to the dephasing of the intermediate exciton state responsible for the first-order coherence time of either single photon. We present a theoretical framework incorporating the effects of spin scattering, background light, and dephasing. We distinguish between the first-order coherence time, and a parameter which we measure for the first time and define as the cross-coherence time.

Control of fine-structure splitting of individual InAs quantum dots by rapid thermal annealing

Degeneracy of the bright single exciton spin state is a prerequisite for the production of triggered polarization-entangled photon pairs from the biexciton decay of a quantum dot. Normally, however, the exciton spin states are split due to in-plane asymmetries. Here the authors demonstrate that the exciton splitting of an individual dot can be tuned through zero by thermal annealing. Repeated annealing blueshifts the exciton emission line of the dot, accompanied by a reduction and inversion in polarization splitting. Annealing is also demonstrated to control the detuning between the exciton and biexciton transitions in any selected dot.

Modulation of single quantum dot energy levels by a surface-acoustic-wave

This letter presents an experimental investigation into the effect of a surface-acoustic-wave (SAW) on the emission of a single InAs quantum dot. The SAW causes the energy of the transitions within the dot to oscillate at the frequency of the SAW, producing a characteristic broadening of the emission lines in their time-averaged spectra. This periodic tuning of the transition energy is used as a method to regulate the output of a device containing a single quantum dot and we study the system as a high-frequency periodic source of single photons.

Enhancement and suppression of spontaneous emission by temperature tuning InAs quantum dots to photonic crystal cavities

We report on the control of the spontaneous emission rates in InAs self-assembled quantum dots weakly coupled to the mode of a modified H1 defect cavity in a two-dimensional photonic crystal slab. Changes in sample temperature are used to spectrally tune the exciton emission from a single quantum dot to the monopole mode of the microcavity. A Purcell enhancement of the spontaneous emission rate of up to a factor of 11.4 is seen on-resonance, while suppression by up to a factor of 4.4 is seen off-resonance. Also, a two orders of magnitude increase in the intensity of light detected from the exciton is measured when compared to a quantum dot in bulk GaAs.

Bell-inequality violation with a triggered photon-pair source.

Here we demonstrate, for the first time, violation of Bells inequality using a triggered quantum dot photon-pair source without post-selection. Furthermore, the fidelity to the expected Bell state is increased above 90% using temporal gating to reject photons emitted at times when collection of uncorrelated light is more probable. A direct measurement of a CHSH Bell inequality is made showing a clear violation, highlighting that a quantum dot entangled photon source is suitable for communication exploiting nonlocal quantum correlations.

Exciton-Spin Memory with a Semiconductor Quantum Dot Molecule

We report on a single photon and spin storage device based on a semiconductor quantum dot molecule. Optically excited single electron-hole pairs are trapped within the molecule, and their recombination rate is electrically controlled over 3 orders of magnitude. Single photons are stored up to 1 μs and read out on a subnanosecond time scale. By using resonant excitation, the circular polarization of individual photons is transferred into the spin state of electron-hole pairs with a fidelity above 80%, which does not degrade for storage times up to the 12.5 ns repetition period of the experiment.