Rupert F. Oulton

Plasmon lasers at deep subwavelength scale

Laser science has been successful in producing increasingly high-powered, faster and smaller coherent light sources. Examples of recent advances are microscopic lasers that can reach the diffraction limit, based on photonic crystals, metal-clad cavities and nanowires. However, such lasers are restricted, both in optical mode size and physical device dimension, to being larger than half the wavelength of the optical field, and it remains a key fundamental challenge to realize ultracompact lasers that can directly generate coherent optical fields at the nanometre scale, far beyond the diffraction limit. A way of addressing this issue is to make use of surface plasmons, which are capable of tightly localizing light, but so far ohmic losses at optical frequencies have inhibited the realization of truly nanometre-scale lasers based on such approaches. A recent theoretical work predicted that such losses could be significantly reduced while maintaining ultrasmall modes in a hybrid plasmonic waveguide. Here we report the experimental demonstration of nanometre-scale plasmonic lasers, generating optical modes a hundred times smaller than the diffraction limit. We realize such lasers using a hybrid plasmonic waveguide consisting of a high-gain cadmium sulphide semiconductor nanowire, separated from a silver surface by a 5-nm-thick insulating gap. Direct measurements of the emission lifetime reveal a broad-band enhancement of the nanowire’s exciton spontaneous emission rate by up to six times owing to the strong mode confinement and the signature of apparently threshold-less lasing. Because plasmonic modes have no cutoff, we are able to demonstrate downscaling of the lateral dimensions of both the device and the optical mode. Plasmonic lasers thus offer the possibility of exploring extreme interactions between light and matter, opening up new avenues in the fields of active photonic circuits, bio-sensing and quantum information technology.

Room-temperature sub-diffraction-limited plasmon laser by total internal reflection

Plasmon lasers are a new class of coherent optical amplifiers that generate and sustain light well below its diffraction limit. Their intense, coherent and confined optical fields can enhance significantly light-matter interactions and bring fundamentally new capabilities to bio-sensing, data storage, photolithography and optical communications. However, metallic plasmon laser cavities generally exhibit both high metal and radiation losses, limiting the operation of plasmon lasers to cryogenic temperatures, where sufficient gain can be attained. Here, we present a room-temperature semiconductor sub-diffraction-limited laser by adopting total internal reflection of surface plasmons to mitigate the radiation loss, while using hybrid semiconductor-insulator-metal nanosquares for strong confinement with low metal loss. High cavity quality factors, approaching 100, along with strong λ/20 mode confinement, lead to enhancements of spontaneous emission rate by up to 18-fold. By controlling the structural geometry we reduce the number of cavity modes to achieve single-mode lasing.

Confinement and propagation characteristics of subwavelength plasmonic modes

We have studied subwavelength confinement of the surface plasmon polariton modes of various plasmonic waveguides and examined their relative merits using a graphical parametric representation of their confinement and propagation characteristics. While the same plasmonic phenomenon governs mode confinement in all these waveguides, the various architectures can exhibit distinctive behavior in terms of effective mode area and propagation distance. We found that the waveguides based on metal and one dielectric material show a similar trade-off between energy confinement and propagation distance. However, a hybrid plasmon waveguide, incorporating metal, low index and high index dielectric materials, exhibits longer propagation distances for the same degree of confinement. We also point out that plasmonic waveguides with sharp features can provide an extremely strong local field enhancement, which is not necessarily accompanied by strong confinement of the total electromagnetic energy. In these waveguides, a mode may couple strongly to nearby atoms, but suffer relatively low propagation losses due to weak confinement.

On long-range plasmonic modes in metallic gaps

Satuby and Orenstein [Opt. Express 15, 4247-4252 (2007)] reported the discovery and numerical and experimental investigation of long-range surface plasmon-polariton eigenmodes guided by wide (6 to 12 mum) rectangular gaps in 400 nm thick gold films using excitation of vacuum wavelength lambda(vac) = 1.55 mum. In this paper, we carry out a detailed numerical analysis of the two different types of plasmonic modes in these structures. We show that no long-range eigenmodes exists for these gap plasmon waveguides, and that the reported modes are likely to be beams of bulk waves and surface plasmons, rather than guided modes of the considered structures.

Anomalous spectral scaling of light emission rates in low-dimensional metallic nanostructures

The strength of light emission near metallic nanostructures can scale anomalously with frequency and dimensionality. We find that light-matter interactions in plasmonic systems confined in two dimensions (e.g., near metal nanowires) strengthen with decreasing frequency owing to strong mode confinement away from the surface-plasmon frequency. The anomalous scaling also applies to the modulation speed of plasmonic light sources, including lasers, with modulation bandwidths growing at lower carrier frequencies. This allows developing optical devices that exhibit simultaneously femtosecond response times at the nanometer scale, even at longer wavelengths into the mid-IR, limited only by nonlocal effects and reversible light-matter coupling.

Active Plasmonics: Surface Plasmon Interaction With Optical Emitters

The interaction between surface plasmons and optical emitters is fundamentally important for engineering applications, especially surface plasmon amplification and controlled spontaneous emission. We investigate these phenomena in an active planar metal-film system comprising InGaN/GaN quantum wells and a silver film. First, we present a detailed study of the propagation and amplification of surface plasmon polaritons (SPPs) at visible frequencies. In doing so, we propose a multiple quantum well structure and present quantum well gain coefficient calculations accounting for SPP polarization, line broadening due to exciton damping, and particularly, the effects of finite temperature. Second, we show that the emission of an optical emitter into various channels (surface plasmons, lossy surface waves, and free radiation) can be precisely controlled by strategically positioning the emitters. Together, these could provide a range of photonic devices (for example, surface plasmon amplifiers, nanolasers, nanoemitters, plasmonic cavities) and a foundation for the study of cavity quantum electrodynamics associated with surface plasmons.

Extremely low-loss slow-light modes in plasmonic dielectric hybrid systems

A new class of optical modes arising from the hybridization between one localized plasmon and two orthogonal waveguide modes is described. Of particular interest is our observation that these hybrid modes simultaneously exhibit extremely low-loss and highly dispersive characteristics, which translate into slow light propagation. We propose that this is a new type of classical analogs of the electromagnetically induced transparency (EIT) in an atomic system. Based on a fine balance of geometric and material dispersion in the system, destructive interference of the waveguide modes cancels out the metal loss, resulting in a narrow transparent window within a broad absorption band. In accordance with the developed phenomenological model, we show that the dispersion characteristics of the hybrid modes can be entirely controlled by tuning the coupling strengths between the plasmon and waveguide modes while the mode losses remain the same.

Directionally emitting plasmon lasers with multiplexing and electrical modulation

We demonstrated the first directionally emitting deep sub-wavelength plasmon laser. The plasmon laser naturally integrates photonic and electronic functionality allowing both efficient electrical modulation and wavelength multiplexing.

Temperature stability of thin film refractory plasmonic materials

Materials such as W, TiN, and SrRuO3 (SRO) have been suggested as promising alternatives to Au and Ag in plasmonic applications owing to their stability at high operational temperatures. However, investigation of the reproducibility of the optical properties after thermal cycling between room and elevated temperatures is so far lacking. Here, thin films of W, Mo, Ti, TiN, TiON, Ag, Au, SrRuO3 and SrNbO3 are investigated to assess their viability for robust refractory plasmonic applications. These results are further compared to the performance of SrMoO3 reported in literature. Films ranging in thickness from 50 to 105 nm are deposited on MgO, SrTiO3 and Si substrates by e-beam evaporation, RF magnetron sputtering and pulsed laser deposition, prior to characterisation by means of AFM, XRD, spectroscopic ellipsometry, and DC resistivity. Measurements are conducted before and after annealing in air at temperatures ranging from 300 to 1000° C for one hour, to establish the maximum cycling temperature and potential longevity at elevated temperatures for each material. It is found that SrRuO3 retains metallic behaviour after annealing at 800° C, while SrNbO3 undergoes a phase transition resulting in a loss of metallic behaviour after annealing at 400° C. Importantly, the optical properties of TiN and TiON are degraded as a result of oxidation and show a loss of metallic behaviour after annealing at 500° C, while the same is not observed in Au until annealing at 600° C. Nevertheless, both TiN and TiON may be better suited than Au or SRO for high temperature applications operating under vacuum conditions.

Plasmon nanolaser and circuit

We will review our works on plasmon lasers and circuits. The scaling down of laser will experience ever-increasing radiation loss and stronger divergence. Plasmonics has emerged as one solution for these hurdles.