Shigeaki Okajima

JENDL-4.0 Benchmarking for Fission Reactor Applications

Benchmark testing for the newly developed Japanese evaluated nuclear data library JENDL-4.0 is carried out by using a huge amount of integral data. Benchmark calculations are performed with a continuous-energy Monte Carlo code and with the deterministic procedure, which has been developed for fast reactor analyses in Japan. Through the present benchmark testing using a wide range of benchmark data, significant improvement in the performance of JENDL-4.0 for fission reactor applications is clearly demonstrated in comparison with the former library JENDL-3.3. Much more accurate and reliable prediction for neutronic parameters for both thermal and fast reactors becomes possible by using the library JENDL-4.0.

Benchmark models for criticalities of FCA-IX assemblies with systematically changed neutron spectra

New benchmark models with respect to criticality data are established on the basis of seven uranium-fueled assemblies constructed in the ninth experimental series at the fast critical assembly (FCA) facility. By virtue of these FCA-IX assemblies, where the simple combinations of uranium fuel and diluent (graphite and stainless steel) in their core regions were systematically varied, the neutron spectra of these benchmark models cover those of various reactor types, from fast to sub-moderated reactors. The sample calculations of the benchmark models by a continuous-energy Monte Carlo (MC) code showed obvious differences between even the latest versions of two major nuclear data libraries, JENDL-4.0 and ENDF/B-VII.1. The present benchmark models would be well suited for the assessment and improvement of the nuclear data for 235U, 238U, graphite, and stainless steel. In addition, the verification of the deterministic method was performed on the benchmark models by comparison with the MC calculations. The present benchmark models are also available to users of deterministic calculation codes for the assessment and improvement of nuclear data.

Prediction Accuracy Improvement of Neutronic Characteristics of a Breeding Light Water Reactor Core by Extended Bias Factor Methods with Use of FCA-XXII-1 Critical Experiments

Two extended bias factor methods, the LC and PE methods, were applied to the prediction accuracy evaluation of neutronic characteristics of a breeding light water reactor, using data of FCA-XXII-1 critical experiments, in order to investigate the features and effectiveness of these methods on the basis of an actual core design and existing experimental results. The present study confirms the following features of these methods. Both the LC and PE methods can improve the prediction accuracy the most when all the experimental results are used. The prediction accuracy improvement is achieved mainly by reducing uncertainty due to errors in cross sections. This is done by realizing a profile of sensitivity coefficients closer to that of the target core and suppressing the influence of errors in experiments and experimental analysis methods. The PE method always improves the prediction accuracy with the use of any combination of experimental results. It is always superior to the LC method in the improvement of the prediction accuracy. Concerning the effectiveness of using the extended bias factor methods with the data of FCA XXII-1 critical experiments, it is concluded that the experimental results regarding multiplication factor are more effective than the other experimental results, namely, reaction rate ratios of 238U capture to 239Pu fission (C28/F49) and void reactivity, in reducing prediction uncertainties of all the neutronic characteristics of the target core investigated: the multiplication factor, the C28/F49, and the void reactivity of the target core. This is due to the fact that the extended bias factor methods cannot fully utilize the potential that these experimental results have for the reduction of the uncertainties due to the errors in cross sections because of their strong correlations to the target core characteristics. This failure is due to large errors in the experiments and/or the experimental analysis methods.

Development of a calculation system for the estimation of decontamination effects

A calculation system for the estimation of decontamination effects (CDE) is developed in the present work to aid in the effective planning of decontamination procedures. This system calculates dose rate distribution before and after decontamination according to the distribution of radioactivity and the decontamination factor. A dose rate reduction factor is also used to estimate decontamination effects. Results obtained from CDE were compared with measurements and particle and heavy-ion transport code system (PHITS) simulations. The CDE successfully reproduced the measured and calculated dose rate distributions, requiring less than several seconds of calculation time.

Measurement and Analysis of Reactivity Worth of 237Np Sample in Cores of TCA and FCA

The reactivity worth of 22.87 grams of 237Np oxide sample was measured and analyzed in seven uranium cores in the Tank-Type Critical Assembly (TCA) and two uranium cores in the Fast Critical Assembly (FCA) at the Japan Atomic Energy Agency. The TCA cores provided a systematic variation in the neutron spectrum between the thermal and resonance energy regions. The FCA cores, XXI and XXV, provided a hard neutron spectrum of the fast reactor and a soft one of the resonance energy region, respectively. Analyses were carried out using the JENDL-3.3 nuclear data library with a Monte Carlo method for the TCA cores and a deterministic method for the FCA cores. The ratios of calculated to experimental (C/E) reactivity worth were between 0.97 and 0.91, and showed no apparent dependence on the neutron spectrum.

Evaluation of Delayed Neutron Data for JENDL-3.3

Delayed neutron data of 235U, 238U and 239Pu have been evaluated and recommended for JENDL-3.3. Adjustment of Vd was carried out on the basis of the ßeff measurements at FCA, MASURCA and TCA using the JENDL-3.2 data as the initial guess. Through this adjustment the vd value for 238U below 3.5 MeV was decreased by about 3 % from 0.0481 to 0.0466. The vd values of 235U and 239Pu were also determined in this way. Further appropriate six group constants, the decay constants λi and the group yields αi, were determined from experimental data of the delayed neutron emission rates, which were collected and compiled by Spriggs through the SG6 activity of WPEC. Applicability of the resultant group constants was validated through the analyses of the reactivity measurements based on the period or the rod-drop methods.

Analyses with latest major nuclear data libraries of the fission rate ratios for several TRU nuclides in the FCA-IX experiments

ABSTRACT In the 1980s, a series of integral experiments was conducted in FCA-IX assemblies with systematically changed neutron spectra covering from the intermediate to fast ones. The experiments provide systematic data of central fission rates for TRU nuclides containing minor actinides, 237Np, 238Pu, 239Pu, 242Pu, 241Am, 243Am, and 244Cm. Regarding the fission rate ratios relative to 239Pu, benchmark models had been recently developed for validation of nuclear data for the TRUs fission cross sections. In this paper, the latest major nuclear data libraries, JENDL-4.0, ENDF/B-VII.1, and JEFF-3.2, are compared on the benchmark models. For the libraries, the analyses by a Monte Carlo calculation code show obvious overestimations particularly for the fission rate ratios of  244Cm to 239Pu. Additionally, a large discrepancy about by 20% between the libraries is revealed for the fission rate ratio of  238Pu to 239Pu measured in the intermediate neutron spectrum. The causes of discrepancies are furthermore clarified by sensitivity analyses.

Intra-pellet neutron flux distribution measurements in LWR critical lattices

We have developed inexpensive and easy-handling measurement methods on intra-pellet neutron flux. A foil activation method with metallic foils, which were fabricated by punching out technique and etching technique to reduce fabrication error and positioning error, was used for the intra-pellet neutron flux distribution measurement. The developed method was applied to measure intra-pellet neutron flux distributions in a reduced–moderation light water reactor (LWR) lattices, and uncertainty of the distributions was estimated to be 1% to 2%. Measured values were analyzed with a continuous energy Monte Carlo code. Comparison of measurements and analyses revealed that the developed method is useful for the validation of an advanced fuel design method considering neutron behavior in fuel pellets.

Measurement and Analysis of Reactivity Worth of 241Am Sample in Water-Moderated Low-Enriched UO2 Fuel Lattices at TCA

The reactivity worths of 22.82 grams of 241Am oxide sample were measured and theoretically analyzed in water-moderated UO2 fuel lattices in seven cores of the Tank-Type Critical Assembly (TCA) at the Japan Atomic Energy Agency for an integral test of 241Am nuclear data. These cores provided a systematic variation in the neutron spectrum between the thermal and resonance energy regions. The sample reactivity worth was measured with an uncertainty of 2.1% or less. The theoretical analysis was performed using the JENDL-3.3 nuclear data by a Monte Carlo calculation method. Ratios of calculation to experiment (C/Es) of the reactivity worth were between 0.91 and 0.97, and showed no apparent dependence on the neutron spectrum. In addition, sensitivity analysis based on the deterministic calculation method was carried out to obtain the impact of changing the 241Am capture cross section on the sample reactivity worth. The result of this analysis showed that the C/E could be significantly improved by almost uniformly increasing the 241Am capture cross section of JENDL-3.3 by 25–30%.

Measurement and analysis of 238U doppler reactivity effect in FCA cores simulating light-water-moderated MOX fuel lattices

The Doppler reactivity effect of 238U was measured in simulated MOX fuel using the FCA facility for the purpose of obtaining data on the 238U Doppler reactivity effect in light-water-moderated MOX fuel and evaluating the prediction accuracy of the current analysis code systems and nuclear data library. Experimental data on the Doppler reactivity effect from room temperature up to 800°C were obtained for a uranium fueled core and mockup cores for MOX-fueled LWR using cylindrical natural-uranium samples. With the use of various samples with various neutron spectra, 238U Doppler reactivity effects at energies generally in the low range below 1 keV were evaluated. Analyses were performed using the current standard analysis code systems for fast and thermal reactors, with the JENDL-3.3 data library. Both analyses yielded calculated/experimental value (C/E) ratios of 0.96 to 1.06 for the MOX cores, a good agreement within the experimental error, and those in the uranium core were similar.