Soon-Ung Park

Nitrogen budgets for the Republic of Korea and the Yellow Sea region

Growing populations in northeast Asia have greatly altered the nitrogencycle, with increases in agricultural production to feed the population, andwith increases in N emissions and transboundary air pollution. For example,during the 1900s over 50% of the N deposition over Republic of Korea wasimported from abroad. In this paper, we present biogeochemical budgets ofN for the South Korean peninsula (the Republic of Korea) and for the YellowSea region. We quantify N inputs from atmospheric deposition, fertilizers,biological fixation, and imports of food, feed, and products. We quantifyoutputs in riverine export, crop uptake, denitrification, volatilization,runoff, sedimentation and sea water exchange. Calculations were conductedusing mean values from 1994–1997. All of the nitrogen budgets werepositive, with N inputs exceeding outputs. The excess N inputs gave rise toincreases in N storage in landfills and in groundwater. Annual accumulationof N in the Yellow sea, including inputs from South Korea and otherdrainage areas, was 1229 kt yr−1 with a residence time for N ofapproximately 1.5 years, thus doubling N content in marine waters every 3years during 1994–1997. The human derived N inputs leads to excessiveeutrophication and pollution of the Yellow Sea.

Turbulence Structure In Unstable Conditions Over Various Surfaces

A comprehensive study of the turbulent structure of the atmospheric boundary layer in unstable conditions has been carried out using turbulence data obtained from the Gobi desert, grassland, suburban and urban sites based on the same instrumentation, data acquisition and data processing systems. The normalized standard deviations of u and v over the suburban and urban sites are systematically smaller than those over the Gobi desert and grassland sites. However, the normalized standard deviations of w, temperature θ and humidity q over the suburban and urban sites are quite close to those over the Gobi desert and grassland sites. The normalized humidity standard deviations are quite similar to those of temperature over the grassland and suburban sites. The temperature and humidity spectra are found to be independentof atmospheric stability in all frequency ranges, but spectra obtained from the Gobi desert and grassland sites reveal flatter peaks than those of the suburban and urban sites in the lower frequency range. The normalized spectral curves of temperature and humidity are independent of atmospheric stability both at high and low frequencies. The spectral characteristics of humidity over the grassland and suburban sites aresimilar to those of temperature, but the humidity spectra over the Gobi desert site are quite different from temperature spectra due to evaporation and/or large eddies in the boundary layer.

Effect of Direct Radiative Forcing of Asian Dust on the Meteorological Fields in East Asia during an Asian Dust Event Period

Abstract Coupled and noncoupled models in a grid of 60 × 60 km2 in the eastern Asian domain have been employed to examine the effect of the direct radiative forcing of the Asian dust aerosol on meteorological fields for an intense Asian dust event observed in eastern Asia on 18–23 March 2002. The coupled model consists of the modified fifth-generation Pennsylvania State University–National Center for Atmospheric Research (NCAR) Mesoscale Model (MM5) with direct radiative forcing of the Asian dust aerosol through the NCAR Column Radiation Model and the Asian Dust Aerosol Model. The noncoupled model is MM5 without the direct radiative forcing of the Asian dust aerosol. The results indicate that the radiative cooling of the dust aerosol over the high-dust-concentration (HDC) region induces sinking motion and positive pressure perturbation near the surface, whereas the radiative warming of the aerosol near the top of the HDC layer induces rising motion and negative pressure perturbation, thereby enhancing the...

Interaction of gaseous pollutants with aerosols in Asia during March 2002.

The Asian Dust Aerosol Model (ADAM) and the aerosol dynamic model with the output of the fifth generation of mesoscale model (MM5) in a grid of 60x60 km2 over the Asian domain have been performed with and without the heterogeneous reaction (gas-aerosol interaction) to estimate the effect of the gas-aerosol interaction on the formation of aerosol for the period of 1-31 March 2002 when a severe Asian dust event has been observed during this period. The simulated gas-phase pollutants concentrations and aerosols are compared with those observed in South Korea and the East Asia Network (EANET). The results indicate that the present modeling system including ADAM, aerosol dynamic model and MM5 model simulates quite well and the gas-phase pollutants concentrations observed in South Korea and the simulated aerosol concentrations with the gas-aerosol interaction yield much better results in concentrations than those without the gas-aerosol interaction. It is found that the favorable regions for the gas-aerosol interaction in Asia are eastern China (high pollutants emissions), Korea, Japan and the East China Sea that are downstream regions of the Asian dust sources and relatively high relative humidity. In these regions the concentrations of SO2 and O3 decrease whereas the concentrations of sulfate and nitrate increase significantly due to the gas-aerosol interaction. In particular, the increase of sulfate concentration due to the interaction is more than 30% of the corresponding concentration without the gas-aerosol interaction. It is also found that the time-area mean column concentrations of PM10, sulfate, nitrate in the model domain are respectively to be 154.9, 3.2, 3.6 mg m(-2) without the gas-aerosol interaction. However, with the gas-aerosol interaction these values have been increased to 0.6% (155.8 mg m(-2)), 16% (3.7 mg m(-2)), and 14% (4.1 mg m(-2)) of the corresponding concentration without the gas-aerosol interaction. On the other hand, the time-area mean concentration of ammonium is found to decrease about 13% (1.8 mg m(-2) to 1.6 mg m(-2)) due to the gas-aerosol interaction. The result clearly indicates the importance of the gas-aerosol interaction on the tropospheric chemistry during the long-range transport period.

Estimates of Asian dust deposition over the Asian region by using ADAM2 in 2007

The Asian Dust Aerosol Model 2 (ADAM2) with the MM5 meteorological model has been employed to estimate the dust concentration, and wet and dry depositions of dust in the Asian region for the year of 2007. It is found that the model simulates quite reasonably the dust (PM(10)) concentrations both in the dust source region (100-110 degrees E and 37-43 degrees N) and the downstream region of Korea. The starting and ending times of most of dust events and their peak concentration occurring times are well simulated. The annual average dust (PM(10)) concentration near the surface is found to be 171microgm(-3) over the dust source area, 39microgm(-3) over the Yellow Sea, 25microgm(-3) over the Korean peninsula and 17microgm(-3) over the East Sea. It is also found that the annual total deposition of dust is about 118.1tkm(-2) (dry deposition, 101.4tkm(-2); wet deposition, 16.7tkm(-2)) in the dust source region, 19.0tkm(-2) (dry deposition, 7.8tkm(-2); wet deposition, 11.2tkm(-2)) in the Yellow Sea, 12.6tkm(-2) (dry deposition, 6.5tkm(-2); wet deposition, 6.1tkm(-2)) in the Korean peninsula and 10.7tkm(-2) (dry deposition, 2.1tkm(-2); wet deposition, 8.6tkm(-2)) in the East Sea. Their ratios of wet deposition to total deposition of dust in the respective regions are 14%, 59%, 48% and 80%. This clearly indicates that the main dust removal mechanism from the atmosphere is dry deposition over the source region whereas wet deposition predominates in the downstream region of the sea. The estimated dust deposition could adversely impact the eco-environmental system in the downstream regions of the dust source region significantly.

Estimation of ammonia emission in South Korea

The importance of ammonia (NH3) in the atmosphere andits role in acidification is increasingly recognized. Adetailed emission inventory of NH3 for South Korea iscarried out for different sources using emission factors.Results indicate that the emission of ammonia has increasedby 21% over the last 11 yr from 143 000 t yr-1 in1988 to 181 000 t yr-1 in 1998. The major contributorsto the NH3 emission in South Korea are livestock andfertilizer application that account for 70 and 26% oftotal NH3 emission, respectively. The 11 × 14 km (0.125° long. × 0.125° lat.) grid distribution of emission of ammonia shows an maximum in the Yochon area due to the largest fertilizer factory and relatively wide regions of high NH3 emission in thenorthwestern part of South Korea due to a great number of livestock. It is found that the nitrogen ratio of wet deposition of NH4+ to emission of NH3 in SouthKorea is averaged to be 0.45.

Estimation of soil respiration using automated chamber systems in an oak (Quercus mongolica) forest at the Nam-San site in Seoul, Korea.

Soil respiration (R(soil)) is the largest component of ecosystem respiration produced by the autotrophic and heterotrophic respirations. Its variability on multiple time scales strongly depends on environmental variables such as temperature and moisture. To investigate the temporal variations of R(soil) in a cool-temperate oak (Quercus mongolica) forest at the Nam-San site in Seoul, Korea, continuous measurements of R(soil) using the automated chamber systems, air and soil temperatures and soil moisture are made for the period from April 2010 to March 2011. The observed data indicate that the R(soil) shows a remarkable seasonal variation in accordance with temperatures with high in summer and low in winter. The R(soil) is found to be strongly correlated with soil temperature (T(s)) at the 5cm depth throughout the year. However, the high fluctuation of R(soil) is found to be related with soil moisture content (M(s)) during the forest growing season. The estimated annual Q(10) value using the 1.5m-high air temperature is found to be 2.4 that is comparable with other studies in temperate forest ecosystems. The optimal regression equation of R(soil) with the T(s) at 5cm depth and the M(s) at 15cm depth is found to be R(soil)=124.3 exp (0.097T(s))-55.3 (M(s))(2)+2931.9 (M(s))-38516 for T(s)≥0°C and R(soil)=0 for T(s)<0°C with r(2)=0.97, P<0.01, suggesting the importance of T(s) and M(s) for R(soil). The annual total soil respiration estimated by the optimal regression equation is found to be 1264gCm(-2) with a maximum of 685gCm(-2) in the summer season and a minimum of 33gCm(-2) in the winter season. The present study can be implemented for the determination of the carbon balance of a cool-temperate Q. mongolica forest with the provision of photosynthesis.

COHERENT STRUCTURES NEAR THE SURFACE IN A STRONGLY SHEARED CONVECTIVE BOUNDARY LAYER GENERATED BY LARGE-EDDY SIMULATION

Well-developed low speed and high temperature streaks in association with the alignment of convection cells are observed in a large-eddy-simulation (LES) generated strongly sheared convective boundary-layer flow, which is driven by a geostrophic wind speed of 15 m s-1 and a surface kinematic heat flux of 0.05 K m s-1. Vortices that drive streaky structures are identified through an eigenvalue method (lambda;2method) near the surface. These vortices are highly elongated along the quasi-streamwise direction alternating sign of the x-component of vorticity (ωx). By conditional sampling of fully developed vortices, a statistically significant coherent structure is educed. The educed vortex is elongated to the streamwise direction with the elevation angle of about 17° above the horizontal surface. However, the horizontal tilting is not clearly demonstrated in the present simulation. Fluctuation fields in the domain of the educed vortex show the existence of a low speed and high temperature streak as a direct consequence of momentum and heat transport by vortical motions. The strong ejection(upward transport of low momentum or high temperature)occurring at the higher level than that of the strong sweep (downward transport of high momentum and low temperature) can be explained from the spatial distribution of the fluctuationfields of velocity and temperature. The contribution of ejection to the Reynolds stress at z/h1 = 0.18 is about 75%, which is slightly greater than that (70% at z/h1 = 0.173) for the neutrally stratified atmospheric boundary layer. Ejection is also found to be dominant for the turbulent heat flux.

Long-range transport contribution to dry deposition of acid pollutants in South Korea

Abstract Long-range transport for dry acidic deposition over South Korea has been estimated using a simplified chemical model and the K-mean clustering technique. The three consecutive daily mean National Center for Environmental Protection reanalyzed 850 hPa geopotential height fields without precipitation on the last day over South Korea are used for clustering of synoptic patterns for the period of 1994–1998. Two emission conditions are simulated for each cluster to estimate long-term impact by long-range transport for acidic dry deposition over South Korea. One condition takes all emissions within the simulated domain into account as a base case and the other condition excludes South Koreas emission and all oxidizers and considering all of the other emissions as a control case. The results of the present study indicate that the contribution of long-range transport to the annual total South Koreas dry deposition of sulfur is found to be about 30% (78 eq ha −1 yr −1 ) , of which 65% and 35% are contributed by SO2 and SO42−, respectively, whereas that of total nitrogen deposition is found to be 49% (240 eq ha −1 yr −1 ) , of which 80% and 20% are contributed by the transformed nitrogen species including HNO3, NH4+ and NO3−, and the primary pollutants of NOx and NH3, respectively, suggesting the importance of secondary pollutants of nitrogen species for long-range transport to South Koreas total dry deposition of nitrogen.

Estimation of Dust Emission Amount for a Dust Storm Event Occurred in April 1998 in China

The threshold friction velocities for dust rises in inland China are examined using WMO synoptic station data and the soil types in the source region to estimate dust emission amounts for a dust event occurred from 13 to 24 April 1998 in China. The dust-rise reports in the WMO synoptic data are used for the delineation of dust source regions that are found to be composed of the Gobi, Sand and Loess regions according to soil types in inland China. The estimated threshold friction velocities with the use of wind speeds observed in the Gobi, Sand and Loess regions are found to be about 60, 50, and 40 cm s-1, respectively. The estimated dust-rise occurrencegrids by both the grid interpolated observed wind and the MM5 model wind well coincide with the areas of strong wind speeds. However, the dust-rise areas estimated by the model are larger than those estimated by the observed wind, whereas the friction velocities estimated by the model in the dust-rise areas are much smaller than those estimated by the observed wind, which result in less amount of dust emission by the model in all source regions. The 10-day accumulated total dust emission estimated by the observed wind during the dust storm event is found to be 4.64 × 108 ton in the whole source region of 3.29 × 106 km2. Of which 85, 9 and 6% are, respectively, contributed by the Gobi, Sand and Loess regions,suggesting the dominant emission from the Gobi region for this event.The model estimated total dust emission is found to be about 56% of that estimated by the observed wind, indicating some improvement of the model being required.