Stephen J. Kindness

Graphene based plasmonic terahertz amplitude modulator operating above 100 MHz

The terahertz (THz) region of the electromagnetic spectrum holds great potential in many fields of study, from spectroscopy to biomedical imaging, remote gas sensing, and high speed communication. To fully exploit this potential, fast optoelectronic devices such as amplitude and phase modulators must be developed. In this work, we present a room temperature external THz amplitude modulator based on plasmonic bow-tie antenna arrays with graphene. By applying a modulating bias to a back gate electrode, the conductivity of graphene is changed, which modifies the reflection characteristics of the incoming THz radiation. The broadband response of the device was characterized by using THz time-domain spectroscopy, and the modulation characteristics such as the modulation depth and cut-off frequency were investigated with a 2.0 THz single frequency emission quantum cascade laser. An optical modulation cut-off frequency of 105 ± 15 MHz is reported. The results agree well with a lumped element circuit model developed to describe the device.

External amplitude and frequency modulation of a terahertz quantum cascade laser using metamaterial/graphene devices

Active control of the amplitude and frequency of terahertz sources is an essential prerequisite for exploiting a myriad of terahertz applications in imaging, spectroscopy, and communications. Here we present a optoelectronic, external modulation technique applied to a terahertz quantum cascade laser which holds the promise of addressing a number of important challenges in this research area. A hybrid metamaterial/graphene device is implemented into an external cavity set-up allowing for optoelectronic tuning of feedback into a quantum cascade laser. We demonstrate powerful, all-electronic, control over the amplitude and frequency of the laser output. Full laser switching is performed by electrostatic gating of the metamaterial/graphene device, demonstrating a modulation depth of 100%. External control of the emission spectrum is also achieved, highlighting the flexibility of this feedback method. By taking advantage of the frequency dispersive reflectivity of the metamaterial array, different modes of the QCL output are selectively suppressed using lithographic tuning and single mode operation of the multi-mode laser is enforced. Side mode suppression is electrically modulated from ~6 dB to ~21 dB, demonstrating active, optoelectronic modulation of the laser frequency content between multi-mode and single mode operation.

Amplitude stabilization and active control of a terahertz quantum cascade laser with a graphene loaded split-ring-resonator array

We demonstrate the amplitude stabilization of a 2.85 THz quantum cascade laser with a graphene loaded split-ring-resonator array acting as an external amplitude modulator. The transmittance of the modulator can be actively changed by modifying the graphene conductivity via electrostatic back-gating. The modulator operates at room temperature and is capable of actively modulating the quantum cascade laser power level and thus stabilizing the power output via a proportional-integral-derivative feedback control loop. The stability was enhanced by more than 10 times through actively tuning the modulation. Furthermore, this approach can be used to externally control the laser power with a high level of stability.We demonstrate the amplitude stabilization of a 2.85 THz quantum cascade laser with a graphene loaded split-ring-resonator array acting as an external amplitude modulator. The transmittance of the modulator can be actively changed by modifying the graphene conductivity via electrostatic back-gating. The modulator operates at room temperature and is capable of actively modulating the quantum cascade laser power level and thus stabilizing the power output via a proportional-integral-derivative feedback control loop. The stability was enhanced by more than 10 times through actively tuning the modulation. Furthermore, this approach can be used to externally control the laser power with a high level of stability.

Fast terahertz optoelectronic amplitude modulator based on plasmonic metamaterial antenna arrays and graphene

The growing interest in terahertz (THz) technologies in recent years has seen a wide range of demonstrated applications, spanning from security screening, non-destructive testing, gas sensing, to biomedical imaging and communication. Communication with THz radiation offers the advantage of much higher bandwidths than currently available, in an unallocated spectrum. For this to be realized, optoelectronic components capable of manipulating THz radiation at high speeds and high signal-to-noise ratios must be developed. In this work we demonstrate a room temperature frequency dependent optoelectronic amplitude modulator working at around 2 THz, which incorporates graphene as the tuning medium. The architecture of the modulator is an array of plasmonic dipole antennas surrounded by graphene. By electrostatically doping the graphene via a back gate electrode, the reflection characteristics of the modulator are modified. The modulator is electrically characterized to determine the graphene conductivity and optically characterization, by THz time-domain spectroscopy and a single-mode 2 THz quantum cascade laser, to determine the optical modulation depth and cut-off frequency. A maximum optical modulation depth of ~ 30% is estimated and is found to be most (least) sensitive when the electrical modulation is centered at the point of maximum (minimum) differential resistivity of the graphene. A 3 dB cut-off frequency > 5 MHz, limited only by the area of graphene on the device, is reported. The results agree well with theoretical calculations and numerical simulations, and demonstrate the first steps towards ultra-fast, graphene based THz optoelectronic devices.

Metamaterial/graphene amplitude and frequency modulators for the active control of terahertz quantum cascade lasers

Hybrid metamaterial/graphene amplitude and frequency modulators have been implemented as external optoelectronic mirrors in external cavity configurations with terahertz quantum cascade lasers (QCLs). These devices’ tunability is accomplished via the interplay between metamaterial resonant units, normally engineered in mm-size arrays, and graphene. The integration of these devices in external cavity QCLs offers unique emission features and realizes an unprecedented studied regime. The implementation of an external amplitude modulation allows the full switching of laser emission in single mode operation by electrostatically gating graphene. The introduction of more dispersive tunable architectures in frequency modulators yields additionally an all-electronic spectral laser bistability.

100 % Amplitude modulation of an external cavity terahertz QCL using an optoelectronic chopper based on metamaterials and graphene

The continuous development of terahertz (THz) sources has opened up many potential applications in spectroscopy, imaging and communications. One popular THz source is the quantum cascade laser (QCL), which has many desirable properties including compactness and high output power with a narrow emission frequency. For such a source to be successfully integrated into a THz communication system, it is necessary to have control over the amplitude, frequency and phase. For wireless communication purposes, amplitude modulators must have a reasonable modulation depth and be capable of fast modulation speeds to take full advantage of the greater bandwidth opened up by using a THz carrier wave. To this purpose, we have developed optoelectronic split ring resonator (SRR) and graphene amplitude modulators which have been combined with a THz QCL thus realising an external cavity set-up which uses the SRR/graphene devices to efficiently modulate the light feedback into the laser cavity. The SRR/graphene device is lithographically designed to have maximum reflectivity at the QCL emission frequency (2.9 THz) and the graphene acts as a variable dampener, capable of electrically modulating the reflectivity. Similar SRR/graphene device architectures have been used previously for amplitude modulation by varying the reflection from a standard CW QCL output, achieving modulation speeds >100 MHz with a modulation depth limited to around 20 % [1].

Terahertz s-SNOM with > λ/1000 resolution based on self-mixing in quantum cascade lasers

Near-field imaging techniques have great potential in many applications, ranging from the investigation of the optical properties of solid state and 2D materials to the excitation and direct retrieval of plasmonic resonant modes, to the mapping of carrier concentrations in semiconductor devices. Further to this, the capability of performing imaging with non-ionizing terahertz (THz) radiation on a subwavelength scale is of fundamental importance in biological applications and healthcare. The implementation of stable, compact solid state sources such as quantum cascade lasers (QCLs) in apertureless scanning near field optical microscopes (s-SNOM), instead of bulkier gas lasers, has been already reported with a resolution ≥ 1 μm [1] based on metallic tips. Here we report on the realization of an s-SNOM, based on tuning fork sensors [2], to maintain a constant sample/tip distance in tapping mode, and using quantum cascade lasers emitting around 3 THz as both source and detector in a self-mixing scheme [3]. The implementation of a fast and efficient feedback mechanism allowed the achievement of a spatial resolution lower than 100 nm, as shown in Fig. 1, thus achieving the record resolution with a QCL better than λ/1000. The self-mixing approach allows an extremely sensitive and fast detection scheme, which overcomes the slow response of traditional THz detectors, by monitoring the scattered signal fed back into the QCL cavity, modulating the power or the bias. In order to enhance the sensitivity of the whole apparatus, as well as the collection of the scattered light, silicon lenses have been attached to the QCLs with an antireflection parylene coating which was thick enough to strongly reduce the laser emission, but still allowed enough power for alignment. Figure 1 reports the topography a) and the THz voltage signal on the QCL b) of Au square features (top-left square corner) over a Si substrate, exhibiting an enhanced scattering. As the reference voltage used for subtraction from the QCL voltage was placed lower than the QCL voltage, the THz signal dropped on the Au square.

Research data supporting "THz nanoscopy of plasmonic resonances with a quantum cascade laser"

The dataset contains all the experimental data required to reproduce the Figures. The profiles can be extracted from the original files.

Fast graphene based plasmonic terahertz amplitude modulators

We present two graphene based plasmonic devices for the external optoelectronic amplitude modulation of THz radiation. Modulation depths as high as 8% and up to 50 MHz, for a 10 V potential difference are reported.

Bow-tie plasmonic arrays loaded with graphene for the fast room temperature detection of terahertz quantum cascade lasers

We present a fast room temperature terahertz detector based on interdigitated bow-tie antennas asymmetrically doping and contacting graphene. The device was tested with a 2 THz quantum cascade laser yielding a responsivity of 0.5 μA/W.