Timo A. Nieminen

Optical alignment and spinning of laser-trapped microscopic particles

Light-induced rotation of absorbing microscopic particles by transfer of angular momentum from light to the material raises the possibility of optically driven micromachines. The phenomenon has been observed using elliptically polarized laser beams or beams with helical phase structure,. But it is difficult to develop high power in such experiments because of overheating and unwanted axial forces, limiting the achievable rotation rates to a few hertz. This problem can in principle be overcome by using transparent particles, transferring angular momentum by a mechanism first observed by Beth in 1936, when he reported a tiny torque developed in a quartz ‘wave-plate’ owing to the change in polarization of transmitted light. Here we show that an optical torque can be induced on microscopic birefringent particles of calcite held by optical tweezers. Depending on the polarization of the incident beam, the particles either become aligned with the plane of polarization (and thus can be rotated through specified angles) or spin with constant rotation frequency. Because these microscopic particles are transparent, they can be held in three-dimensional optical traps at very high power without heating, leading to rotation rates of over 350 Hz.

Optical tweezers computational toolbox

We describe a toolbox, implemented in Matlab, for the computational modelling of optical tweezers. The toolbox is designed for the calculation of optical forces and torques, and can be used for both spherical and nonspherical particles, in both Gaussian and other beams. The toolbox might also be useful for light scattering using either Lorenz–Mie theory or the T-matrix method.

Optical microrheology using rotating laser-trapped particles

We demonstrate an optical system that can apply and accurately measure the torque exerted by the trapping beam on a rotating birefringent probe particle. This allows the viscosity and surface effects within liquid media to be measured quantitatively on a micron-size scale using a trapped rotating spherical probe particle. We use the system to measure the viscosity inside a prototype cellular structure.

Optical application and measurement of torque on microparticles of isotropic nonabsorbing material

We show how it is possible to controllably rotate or align microscopic particles of isotropic nonabsorbing material in a TEM00 Gaussian beam trap, with simultaneous measurement of the applied torque using purely optical means. This is a simple and general method of rotation, requiring only that the particle is elongated along one direction. Thus, this method can be used to rotate or align a wide range of naturally occurring particles. The ability to measure the applied torque enables the use of this method as a quantitative tool - the rotational equivalent of optical tweezers based force measurement. As well as being of particular value for the rotation of biological specimens, this method is also suitable for the development of optically-driven micromachines.

Forces in optical tweezers with radially and azimuthally polarized trapping beams.

It has been suggested that radially polarized beams can be used to improve the performance of optical tweezers, with reduced scattering force resulting from both the polarization and the dark center of the beam [Opt. Lett. 32, 1839 (2007)]. We calculate the forces on particles in such traps, using rigorous electromagnetic theory, comparing the results with azimuthally polarized beam, circularly polarized LG 01 beams, and Gaussian beams. Our results agree qualitatively with Opt. Lett. 32, 1839 (2007), but differ quantitatively.

Optical torque controlled by elliptical polarization.

We show theoretically and demonstrate experimentally that highly absorbing particles can be trapped and manipulated in a single highly focused Gaussian beam. Our studies of the effects of polarized light on such particles show that they can be set into rotation by elliptically polarized light and that both the sense and the speed of their rotation can be smoothly controlled.

Angular momentum of a strongly focused Gaussian beam

A circularly polarized paraxial Gaussian laser beam carries ± ¯ h angular momentum per photon as spin, with zero orbital angular momentum. Focusing the beam with a rotationally symmetric lens cannot change this angular momentum flux, yet the focused beam must have spin |Sz| < ¯ h per photon. The remainder of the original spin is converted to orbital angular momentum, manifesting itself as a longitudinal optical vortex at the focus. We investigate the nature of this orbital angular momentum.

Multipole expansion of strongly focussed laser beams

Multipole expansion of an incident radiation field-that is, representation of the fields as sums of vector spherical wavefunctions-is essential for theoretical light scattering methods such as the T-matrix method and generalised Lorenz-Mie theory (GLMT). In general, it is theoretically straightforward to find a vector spherical wavefunction representation of an arbitrary radiation field. For example, a simple formula results in the useful case of an incident plane wave. Laser beams present some difficulties. These problems are not a result of any deficiency in the basic process of spherical wavefunction expansion, but are due to the fact that laser beams, in their standard representations, are not radiation fields, but only approximations of radiation fields. This results from the standard laser beam representations being solutions to the paraxial scalar wave equation. We present an efficient method for determining the multipole representation of an arbitrary focussed beam

Calculation of the T-matrix: General Considerations and Application of the Point-Matching Method

The T-matrix method is widely used for the calculation of scattering by particles of sizes on the order of the illuminating wavelength. Although the extended boundary condition method (EBCM) is the most commonly used technique for calculating the T-matrix, a variety of methods can be used. We consider some general principles of calculating T-matrices, and apply the point-matching method to calculate the T-matrix for particles devoid of symmetry. This method avoids the time-consuming surface integrals required by the EBCM.

Calculation and optical measurement of laser trapping forces on non-spherical particles

Optical trapping, where microscopic particles are trapped and manipulated by light is a powerful and widespread technique, with the single-beam gradient trap (also known as optical tweezers) in use for a large number of biological and other applications. The forces and torques acting on a trapped particle result from the transfer of momentum and angular momentum from the trapping beam to the particle. Despite the apparent simplicity of a laser trap, with a single particle in a single beam, exact calculation of the optical forces and torques acting on particles is difficult. Calculations can be performed using approximate methods, but are only applicable within their ranges of validity, such as for particles much larger than, or much smaller than, the trapping wavelength, and for spherical isotropic particles. This leaves unfortunate gaps, since wavelength-scale particles are of great practical interest because they are readily and strongly trapped and are used to probe interesting microscopic and macroscopic phenomena, and non-spherical or anisotropic particles, biological, crystalline, or other, due to their frequent occurance in nature, and the possibility of rotating such objects or controlling or sensing their orientation. The systematic application of electromagnetic scattering theory can provide a general theory of laser trapping, and render results missing from existing theory. We present here calculations of force and torque on a trapped particle obtained from this theory and discuss the possible applications, including the optical measurement of the force and torque.