Ulrich Probst

Long term performance of metal seals for transport and storage casks

Abstract Dual purpose casks for the transportation and storage of spent nuclear fuel and other radioactive materials require very high leak tightness of lid closure systems under accident conditions as well as in the long term to prevent activity release. For that purpose metal seals of specific types with an inner helical spring and outer metal liners are widely used and have shown their excellent performance if certain quality assurance requirements for fabrication and assembling are satisfied. Well defined surface roughness, clean and dry inert conditions are therefore essential. No seal failure in a loaded cask happened under these conditions until today. Nevertheless, the considered and licensed operation period is limited and all safety assessments have been performed and approved for this period of time which is 40 years in Germany so far. However, in the meantime longer storage periods might be necessary for the future and therefore additional material data will be required. BAM is involved in the qualification and evaluation procedures of those seals from the early beginning. Because long term tests are always time consuming BAM has early decided to perform additional tests with specific test seal configurations to gain a better understanding of the long term behaviour with regard to seal pressure force, leakage rate and useable resilience which is safety relevant mainly in case of accidental mechanical loads inside a storage facility or during a subsequent transport. Main test parameters are the material of the outer seal jacket (silver or aluminium) and the temperature. This paper presents the BAM test program including an innovative test mock-up and most recent test results. Based on these data extrapolation models to extended time periods are discussed, and also future plans to continue tests and to investigate seal behaviour for additional test parameters are explained.

Aging management for long-term interim storage casks

Abstract The aging management system for the mechanical components of nuclear power plants (NPPs) must be established and used by the licensee in such a way that the quality of safety relevant components is guaranteed for the completely designed lifetime of the NPP. This demands an extensive plant life management with special emphases on the knowledge of the degradation in material properties. The basic safety concept in Germany observes this circumstance. Lifetime extension of the German NPPs is an aim of the current valid coalition agreement of the German government. Operational extension of interim storage facilities requires, in comparison to the aging management system for NPP, an aging management system adapted to the special circumstances of spent fuel storage casks. Extension of interim storage periods for spent fuel casks beyond the designed lifetime requires, in comparison to the components of an NPP, an increasing knowledge of material degradation with potential impact on cask integrity, e.g. leak tightness. Dry interim storage in Germany has been approved for 40 years. After that time, according to the present strategy, a final repository should be available. However, until now, such a final facility still does not exist, and the German exploration and licensing process is heavily delayed. Currently, discussions are continuing regarding further exploration of the Gorleben salt mine. There is willingness to overcome this situation that is clearly described in the available coalition agreement of the federal government. Anyway, however, the prediction is viewed; a repository for heat generating radioactive waste in Germany will not be available in the near future and may not be available when first storage facilities and casks reach their 40 years of approved lifetime, which will occur in ∼25 years starting from now. Therefore, the question must be asked: what has to be done with the existing storage casks in the interim facilities? May these casks be fit for continued use, with an extension of the storage period? One option is to have an aging management system, which creates enough information about the technical condition of safety relevant cask properties. This is the basis for safety evaluation for extended storage periods. In the present paper, possible aging mechanisms for high level waste storage casks are discussed, as well as the influence of the time dependent changes of the component properties.

Investigation of seal effects according to axial compression variation of metal seals for transport and storage casks

Abstract Casks for the transport and storage of heat generating radioactive waste in Germany are normally provided with screwed lid systems, which are in most cases equipped with double jacket metal seals with an inner spring wire to provide long term resistance to the seal compression force. Preservation of the high sealing quality of those seals under operational and accidental stress conditions is essentially important to the safety of those casks. Relative displacements of the lid system surfaces caused by specific impact scenarios cannot be excluded and have to be evaluated with respect to a possible increase in the leakage rate. To get representative data for such metal sealed lid systems, BAM has developed a special conceptualised flange system placed in an appropriate testing machine for relevant mechanical loading of the metal seals under static and cyclic conditions. Furthermore, the flange system enables continuous measurement of the standard helium leakage rate during each test. The primary aim of the investigation is to identify the correlation between variation of installation conditions (axial displacements) caused by external loads and the standard helium leakage rate. An essential parameter in this case is the useable resilience ru of a metal seal under relevant stress conditions. The useable resilience ru is the vertical difference in the cross-section between the seals assembling status and the point where the leakage rate, by means of external load relieving, exceeds the quality criterion of 10–8 Pa m3 s–1. Load relieving can instantly occur due to modification of the seal groove dimension caused by accident impacts and deformation of the lid system. Furthermore, component specific basis data for the development of finite element calculation models should be collected. In the tests, seals are subjected to static and cyclic loads. All tests are performed at ambient temperature. This paper presents the test configuration, different test series and results of the current experiments. Typical load–displacement–leakage rate correlations are presented and discussed.

Verification of activity release compliance with regulatory limits within spent fuel transport cask assessment

Abstract Admissible limits for activity release from type B(U) packages for spent fuel transport specified in the International Atomic Energy Agency regulations (10−6 A2 h−1 for normal conditions of transport and A2 per week for accidental conditions of transport) have to be kept by an appropriate function of the cask body and its sealing system. Direct measurements of activity release from the transport casks are not feasible. Therefore, the most common method for the specification of leak tightness is to relate the admissible limits of activity release to equivalent standardised leakage rates. Applicable procedure and calculation methods are summarised in the International Standard ISO 12807 and the US standard ANSI N14·5. BAM as the German competent authority for mechanical, thermal and containment assessment of packages liable for approval verifies the activity release compliance with the regulatory limits. Two fundamental aspects in the assessment are the specification of conservative design leakage rates for normal and accidental conditions of transport and the determination of release fractions of radioactive gases, volatiles and particles from spent fuel rods. Design leakage rates identify the efficiency limits of the sealing system under normal and accidental transport conditions and are deduced from tests with real casks, cask models or components. The releasable radioactive content is primarily determined by the fraction of rods developing cladding breaches and the release fractions of radionuclides due to cladding breaches. The influence of higher burn-ups on the failure probability of the rods and on the release fractions are important questions. This paper gives an overview about methodology of activity release calculation and correlated boundary conditions for assessment.

Testing and Numerical Simulation of Elastomers: From Specimen Tests to Simulation of Seal Behavior Under Assembly Conditions

Due to delays in the siting procedure to establish a deep geological repository for spent nuclear fuel and high level radioactive waste as well as in construction of the already licensed Konrad repository for low and intermediate level radioactive waste, extended periods of interim storage become more relevant in Germany. BAM is involved in most of the cask licensing procedures and especially responsible for the evaluation of cask-related long-term safety issues. The long-term performance of elastomer seals for lid systems of transport and storage casks, whether used as auxiliary seals in spent fuel casks or as primary seals for low and intermediate level waste packages, is an important issue in this context. The polymeric structure of these seals causes a complex mechanical behavior with time-dependent sealing force reduction. The results of a comprehensive purpose-designed test program consisting of basic compression and tension tests as well as relaxation tests on unaged specimens of representative types of elastomers (fluorocarbon rubber (FKM) and ethylene propylene diene rubber (EPDM)) at different temperatures and strain rates are presented. They were used to identify the constitutive behavior and to obtain parameters for finite element material models provided by the computer code ABAQUS®. After estimating the influence of uncertainties such as Poisson’s ratio and friction coefficient by sensitivity analyses, the chosen parameters had to prove their suitability for the finite element simulation of the specimen tests themselves. Based on this preliminary work the simulation of a specific laboratory test configuration containing a typical elastomer seal with circular cross section is presented. The chosen finite element material model and the implemented parameters had to show that they are able to represent not only the specimen behavior under predominantly uniaxial load but also the more complex stress states in real components. Deviations between the measured and calculated results are pointed out and discussed. For the consideration of long-term effects in the simulation of elastomer behavior, test results of aged specimens are needed. First information about a new test program, started recently and planned to provide these data, are given.

Consideration of aging mechanism influence on transport safety of dual purpose casks for spent nuclear fuel or HLW

Abstract When storage of spent nuclear fuel or high level waste is carried out in dual purpose casks (DPC), the effects of aging on safety relevant DPC functions and properties have to be managed in a way that a safe transport after the storage period of several decades is capable and can be justified and certified permanently throughout that period. The effects of aging mechanisms (e.g. radiation, different corrosion mechanisms, stress relaxation, creep, structural changes and degradation) on the transport package design safety assessment features have to be evaluated. Consideration of these issues in the DPC transport safety case will be addressed. Special attention is given to all cask components that cannot be directly inspected or changed without opening the cask cavity, like the inner parts of the closure system and the cask internals, like baskets or spent fuel assemblies. The design criteria of that transport safety case have to consider the operational impacts during storage. Aging is not the subject of technical aspects only but also of ‘intellectual’ aspects, like changing standards, scientific/technical knowledge development and personal as well as institutional alterations. Those aspects are to be considered in the management system of license holders and in appropriate design approval update processes. The paper addresses issues that are subject of an actual International Atomic Energy Agency TECDOC draft ‘Preparation of a safety case for a dual purpose cask containing spent nuclear fuel’.

Analysis of Bolted Flange Joints for Lids of Packages for Radioactive Materials

The design of bolted flange joints for the German double barrier closure system of spent fuel and high-level waste transport and storage casks is described. Additionally, the basic load assumptions are presented for service conditions and for hypothetical accident scenarios. The modelling details and the results of numerical analyses are discussed with respect to those of experiments. The treatment of the numerical results for the bolts is presented considering safety factors derived by nominal stress concepts. The lids of the double barrier system are designed for a specified helium leak tightness. In addition to interior pressure, the accelerations during usual service and in particular during accidental drop tests are considered. The sliding and the gap formation at the gasket surfaces is analysed with respect to drop test loads. The consequences for the containment analysis are discussed on basis of the tightness characteristics. Concerning the bolts, the transfer of local stresses provided by numerical analysis to nominal stress values is presented. This transfer enables the use of safety factors based on nominal stress concepts for the local stresses given by numerical analysis.Copyright