Warren J. Gore

Examining the impact of overlying aerosols on the retrieval of cloud optical properties from passive remote sensing

[1] Haywood et al. (2004) show that an aerosol layer above a cloud can cause a bias in the retrieved cloud optical thickness and effective radius. Monitoring for this potential bias is difficult because space‐based passive remote sensing cannot unambiguously detect or characterize aerosol above cloud. We show that cloud retrievals from aircraft measurements above cloud and below an overlying aerosol layer are a means to test this bias. The data were collected during the Intercontinental Chemical Transport Experiment (INTEX‐A) study based out of Portsmouth, New Hampshire, United States, above extensive, marine stratus cloud banks affected by industrial outflow. Solar Spectral Flux Radiometer (SSFR) irradiance measurements taken along a lower level flight leg above cloud and below aerosol were unaffected by the overlying aerosol. Along upper level flight legs, the irradiance reflected from cloud top was transmitted through an aerosol layer. We compare SSFR cloud retrievals from below‐aerosol legs to satellite retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) in order to detect an aerosol‐induced bias. In regions of small variation in cloud properties, we find that SSFR and MODIS‐retrieved cloud optical thickness compares within the uncertainty range for each instrument while SSFR effective radius tend to be smaller than MODIS values (by 1–2 mm) and at the low end of MODIS uncertainty estimates. In regions of large variation in cloud properties, differences in SSFR and MODIS‐retrieved cloud optical thickness and effective radius can reach values of 10 and 10 mm, respectively. We include aerosols in forward modeling to test the sensitivity of SSFR cloud retrievals to overlying aerosol layers. We find an overlying absorbing aerosol layer biases SSFR cloud retrievals to smaller effective radii and optical thickness while nonabsorbing aerosols had no impact.

Atmospheric Radiation Measurements Enhanced Shortwave Experiment (ARESE) : Experimental and data details

Atmospheric Radiation Measurements Enhanced Shortwave Experiment (ARESE) was conducted to study the magnitude and spectral characteristics of the absorption of solar radiation by the clear and cloudy atmosphere. Three aircraft platforms, a Grob Egrett, a NASA ER-2, and a Twin Otter, were used during ARESE in conjunction with the Atmospheric Radiation Measurements (ARM) central and extended facilities in north central Oklahoma. The aircraft were coordinated to simultaneously measure solar irradiances in the total spectral broadband (0.224-3.91 μm), near infrared broadband (0.678-3.3 μm), and in seven narrow band-pass (∼10 nm width) channels centered at 0.500, 0.862, 1.064, 1.249, 1.501, 1.651, and 1.750 μm. Instrumental calibration issues are discussed in some detail, in particular radiometric power, angular, and spectral responses. The data discussed in this paper are available at the ARM ARESE data archive via anonymous FTP to ftp.arm.gov.

Radiative flux measurements in the troposphere

The results of radiative flux-density measurements in the troposphere, made using an especially designed radiometer mounted on a Cessna 402B aircraft, are reported. The radiometer incorporates several well-known principles that result in highly accurate determinations of radiative fluxes in the atmosphere. Heating rates for gases and for aerosols are calculated, using measurements and radiosonde data. Instrument performance is verified by calculating the solar constant at the top of the atmosphere, using the radiative flux densities measured in the troposphere. Total heating rates of 0.175 and 0.377 K h(-1) are determined for hazy and foggy atmospheres, respectively. Aerosol heating rates of 0.065 and 0.235 K h(-1) are deduced from the total heating rates. Environmental noise measurements during data acquisition are presented. The solar constant value of 1387 +/- 21 W m(-2) derived from the experiments agrees within 4% of the standard value.

The effects of the Arctic haze as determined from airborne radiometric measurements during AGASP II

The interaction of the Aretic winter aerosol (Arctic haze) with solar radiation produces changes in the radiation field that result in the enhancement of scattering and absorption processes which alter the energy balance and solar energy distribution in the Arctic atmosphere-surface system. During the second Arctic Gas and Aerosols Sampling Project (AGASP II) field experiment, we measured radiation parameters using the NOAA WP-3D research aircraft as a platform. State-of-the-art instrumentation was used to measure in situ the absorption of solar radiation by the Arctic atmosphere during severe haze events. Simultaneously with the absorption measurements, we determined optical depths, and total, direct, and scattered radiation fields. All optical measurements were made at spectral bands centered at 412, 500, 675, and 778 nm and with a bandpass of 10 nm. With this selection of spectral regions we concentrated on the measurement of the radiative effects of the aerosol excluding most of the contributions by the gaseous components of the atmosphere. An additional measurement performed during these experiments was the determination of total solar spectrum fluxes. The experimentally determined parameters were used to define an aerosol model that was employed to deduce the absorption by the aerosols over the full solar spectrum and to calculate atmospheric heating rate profiles. The analyses summarized above allowed us to deduce the magnitude of the change in some important parameters. For example, we found changes in instantaneous heating rate of up to about 0.6 K/day. Besides the increased absorption (30 to 40%) and scattering of radiation by the atmosphere, the haze reduces the surface absorption of solar energy by 6 to 10% and the effective planetary albedo over ice surfaces by 3 to 6%. The vertical distribution of the absorbing aerosol is inferred from the flux measurements. Values for the specific absorption of carbon are found to be around 6 m2/g for externally mixed aerosol and about 11.7 m2/g for internally mixed aerosol. A complete study of the radiative effects of the Arctic haze should include infrared measurements and calculations as well as physics of the ice, snow, and water surfaces.

A Comparison of In Situ Aircraft Measurements of Carbon Dioxide and Methane to GOSAT Data Measured Over Railroad Valley Playa, Nevada, USA

In this paper, we report the vertical profiles of CO2 and CH4 measured with a cavity ring-down spectrometer (CRDS) on a research aircraft from near-ground level to 8 km above mean sea level. The airborne platform employed in this paper is an Alpha Jet aircraft operated from NASAs Ames Research Center. Flights were undertaken to Railroad Valley, NV, USA, to coincide with overpasses of the Greenhouse Gases Observing Satellite (GOSAT). Ground-based CO2 and CH4 were simultaneously measured using CRDS, at the time and location of the airborne and satellite measurements. Results of three GOSAT coordinated aircraft profiles and ground-based measurements in June 2011 are presented and discussed in this paper. The accuracy of the CO2 and CH4 measurements has been determined based upon laboratory calibrations (World Meteorological Organisation traceable standard) and pressure/temperature flight simulations in a test chamber. The overall uncertainty for the airborne measurements ranged from 0.31 to 0.39 ppm for CO2 and from 3.5 to 5.6 ppb for CH4. Our column-averaged CO2 and CH4 measurements, which include about 61% of the total atmospheric mass, are extrapolated, using different techniques, to include the remainder of the tropospheric and stratospheric CO2 and CH4. The CO2 data are then analyzed using the Atmospheric CO2 Observations from Space 2.9 and 3.3 algorithms. For methane data, the RemoTeC v2.1 algorithm was used in its full physics setup. Column-averaged CO2 and XCO2, measured by GOSAT and analyzed from our data, ranged from 388.1 to 396.4 ppm, and XCH4 ranged from 1.743 to 1.822 ppm. The agreement of the satellite and aircraft CO2 mixing ratios, as well as ground measurements, falls within the uncertainties of the methods employed to acquire these numbers.

A New Instrumented Airborne Platform for Atmospheric Research

AbstractThe NASA Ames Research Center operates a new research platform for atmospheric studies: an instrumented Alpha Jet. The present complement of instruments allows for the determination of carbon dioxide, ozone, water vapor, and methane concentrations as well as measurements of three-dimensional wind speeds, temperature, and pressure. Planned future instrumentation includes an Air-Core sampler and an instrument to measure formaldehyde. We give examples of measurements that have been made, including measurements carried out during a downward spiral over an expected methane source. An attractive property of this airborne system is its ability to respond rapidly to unexpected atmospheric events such as large forest fires or severe air quality events.

Two-Year Comparison of Airborne Measurements of CO 2 and CH 4 With GOSAT at Railroad Valley, Nevada

The Alpha Jet Atmospheric eXperiment (AJAX) is a project to measure the atmospheric profiles of greenhouse gases (GHGs) and ozone (O3) regularly over California and Nevada. Airborne instruments measuring GHGs and O3 are installed in a wing pod of an Alpha Jet aircraft and operated from the National Aeronautics and Space Administration Ames Research Center at Moffett Field, CA. The instruments yield precise and accurate in situ vertical profiles of atmospheric carbon dioxide (CO2), methane (CH4), and O3. Measurements of vertical profiles of GHGs and O3 over Railroad Valley, NV have been conducted directly under the Greenhouse gases Observing SATellite (GOSAT) over passes on a monthly basis as part of the AJAX project since June 2011. The purpose of this work is to calculate aircraft-based dry-air mole fractions of the GHGs for the validation of GOSAT data products. This study expands and improves our previous comparisons by evaluating three algorithms against 24 months of in situ data collected over a Gain-M target. We used three different algorithms: Atmospheric CO2 Observations from Space (ACOS v3.4r3), Remote Sensing of Greenhouse Gases for Carbon Cycle Modeling (RemoteC v2.3.5FP), and National Institute for Environmental Studies (NIES v2.11). We find that the CO2 average differences of ACOS and RemoteC from AJAX are 0.26% and 0.24%, respectively. The difference between NIES and AJAX is 0.96%, which is higher than that of ACOS and RemoteC. The CH4 average differences for RemoteC and NIES are 2.1% and 1.7%, respectively.

An Assessment of Ground Level and Free Tropospheric Ozone Over California and Nevada

Increasing free tropospheric ozone (O3), combined with the high elevation and often deep boundary layers at western US surface stations, poses challenges in attaining the more stringent 70 ppb O3 National Ambient Air Quality Standard. As such, use of observational data to identify sources and mechanisms that contribute to surface O3 is increasingly important. This work analyzes surface and vertical O3 observations over California and Nevada from 1995 to 2015. Over this period, the number of high O3 events (95th percentile) at US EPA CASTNET sites has decreased during summer, as a result of decreasing US emissions. In contrast, an increase in springtime 5th percentile O3 indicates a general increase of baseline O3. During 2012 there was a peak in exceedances and in the average spring-summer O3 mixing ratios at CASTNET sites. GEOS-Chem results show that the surface O3 attributable to transport from the upper troposphere and stratosphere were increased in 2013 compared to 2012, highlighting the importance of measurements aloft. Vertical O3 measurements from aircraft, ozonesondes and lidar show distinct seasonal trends, with a high percentage of elevated O3 laminae (O3 >70 ppb, 3-8 km) during spring and summer. Analysis of the timing of high O3 surface events and correlation between surface and vertical O3 data is used to discuss varying sources of western US surface O3.

Calibration of infrared satellite images using high altitude aircraft measurements

The use of infrared radiance measurements made from high altitude aircraft for satellite image validation is discussed. Selected examples are presented to illustrate the techniques and the potentials of such validation studies.