Y. Okamura

Observation of magnetic excitations of Skyrmion crystal in a helimagnetic insulator Cu2OSeO3.

We have investigated the low-energy dynamics of the triangular lattice of Skyrmions in a helimagnetic insulator Cu2OSeO3 in terms of microwave response. We have observed two elementary excitations of the Skyrmion with different polarization characteristics: the counterclockwise circulating mode at 1 GHz with the magnetic field polarization parallel to the Skyrmion plane and the breathing mode at 1.5 GHz with a perpendicular magnetic field polarization. These modes reflect the topological nature of Skyrmions and may play a central role in the Skyrmion dynamics.

Microwave magnetoelectric effect via skyrmion resonance modes in a helimagnetic multiferroic

Magnetic skyrmion, a topologically stable spin-swirling object, can host emergent electromagnetism, as exemplified by the topological Hall effect and electric-current-driven skyrmion motion. To achieve efficient manipulation of nano-sized functional spin textures, it is imperative to exploit the resonant motion of skyrmions, analogously to the role of the ferromagnetic resonance in spintronics. The magnetic resonance of skyrmions has recently been detected with oscillating magnetic fields at 1-2 GHz, launching a search for new skyrmion functionality operating at microwave frequencies. Here we show a microwave magnetoelectric effect in resonant skyrmion dynamics. Through microwave transmittance spectroscopy on the skyrmion-hosting multiferroic crystal Cu₂OSeO₃ combined with theoretical simulations, we reveal nonreciprocal directional dichroism (NDD) at the resonant mode, that is, oppositely propagating microwaves exhibit different absorption. The microscopic mechanism of the present NDD is not associated with the conventional Faraday effect but with the skyrmion magnetoelectric resonance instead, suggesting a conceptually new microwave functionality.

Magnetochiral nonreciprocity of volume spin wave propagation in chiral-lattice ferromagnets

Spin current, i.e. the flow of spin angular momentum or magnetic moment, has recently attracted much attention as the promising alternative for charge current with better energy efficiency. Genuine spin current is generally carried by the spin wave (propagating spin precession) in insulating ferromagnets, and should hold the chiral symmetry when it propagates along the spin direction. Here, we experimentally demonstrate that such a spin wave spin current (SWSC) shows nonreciprocal propagation characters in a chiral-lattice ferromagnet. This phenomenon originates from the interference of chirality between the SWSC and crystal-lattice, which is mediated by the relativistic spin-orbit interaction. The present finding enables the design of perfect spin current diode, and highlights the importance of the chiral aspect in SWSC.

Transition to and from the skyrmion lattice phase by electric fields in a magnetoelectric compound

Dissipation-less electric control of magnetic state variable is an important target of contemporary spintronics. The non-volatile control of magnetic skyrmions, nanometre-sized spin-swirling objects, with electric fields may exemplify this goal. The skyrmion-hosting magnetoelectric chiral magnet Cu2OSeO3 provides a unique platform for the implementation of such control; however, the hysteresis that accompanies the first-order transition associated with the skyrmion phase is negligibly narrow in practice. Here we demonstrate another method that functions irrespective of the transition boundary. Combination of magnetic-susceptibility measurements and microwave spectroscopy reveals that although the metastable skyrmion lattice is normally hidden behind a more thermodynamically stable conical phase, it emerges under electric fields and persists down to the lowest temperature. Once created, this metastable skyrmion lattice remains without electric fields, establishing a bistability distinct from the transition hysteresis. This bistability thus enables non-volatile electric-field control of the skyrmion lattice even in temperature/magnetic-field regions far from the transition boundary.

Current-induced viscoelastic topological unwinding of metastable skyrmion strings

In the MnSi bulk chiral magnet, magnetic skyrmion strings of 17 nm in diameter appear in the form of a lattice, penetrating the sample thickness, 10–1000 μm. Although such a bundle of skyrmion strings may exhibit complex soft-matter-like dynamics when starting to move under the influence of a random pinning potential, the details remain highly elusive. Here, we show that a metastable skyrmion-string lattice is subject to topological unwinding under the application of pulsed currents of 3–5 × 106 A m–2 rather than being transported, as evidenced by measurements of the topological Hall effect. The critical current density above which the topological unwinding occurs is larger for a shorter pulse width, reminiscent of the viscoelastic characteristics accompanying the pinning-creep transition observed in domain-wall motion. Numerical simulations reveal that current-induced depinning of already segmented skyrmion strings initiates the topological unwinding. Thus, the skyrmion-string length is an element to consider when studying current-induced motion.Understanding the dynamics of the skyrmion string lattice is the prerequisite for its potential application as next-generation information carriers. Here, the authors explore the topological unwinding of skyrmion string lattice under the application of current pulses.

Determination of the Lowest Unoccupied Orbital in the Layered Perovskite LaSrMnO4 Using Polarized Oxygen K Edge Absorption Spectroscopy.

Using polarized oxygen K edge spectroscopy, the first unoccupied orbital of LaSrMnO 4 was investigated. The lowest unoccupied orbital is of minority spin d x z , d y z character instead of the majority spin d x 2 - y 2 character. The d x 2 - y 2 orbital would be expected based on Hunds rule and the strong exchange interaction of the one-electron addition d 5 system. The explanation is a strong ligand field splitting caused by the strong local site distortion of the Mn site which raises the energy of the majority spin d x 2 - y 2 orbital and lowers the energy of the d x z , d y z orbitals. At the same time the two-electron integrals, which are responsible for the exchange interaction, are screened because of covalency.