A. Giles Davies

Terahertz semiconductor-heterostructure laser

Semiconductor devices have become indispensable for generating electromagnetic radiation in everyday applications. Visible and infrared diode lasers are at the core of information technology, and at the other end of the spectrum, microwave and radio-frequency emitters enable wireless communications. But the terahertz region (1–10 THz; 1 THz = 1012 Hz) between these ranges has remained largely underdeveloped, despite the identification of various possible applications—for example, chemical detection, astronomy and medical imaging. Progress in this area has been hampered by the lack of compact, low-consumption, solid-state terahertz sources. Here we report a monolithic terahertz injection laser that is based on interminiband transitions in the conduction band of a semiconductor (GaAs/AlGaAs) heterostructure. The prototype demonstrated emits a single mode at 4.4 THz, and already shows high output powers of more than 2 mW with low threshold current densities of about a few hundred A cm-2 up to 50 K. These results are very promising for extending the present laser concept to continuous-wave and high-temperature operation, which would lead to implementation in practical photonic systems.

Terahertz spectroscopy of explosives and drugs

Terahertz frequency radiation possesses a unique combination of desirable properties for noninvasive imaging and spectroscopy of materials. This includes the ability to obtain chemical and structural information about substances concealed within dry packaging, such as paper, plastics, and cardboard. As a result, the application of terahertz frequency spectroscopy for the sensing and identification of materials of security interest, such as explosives and, to a lesser extent, drugs-of-abuse, has caught the attention of a number of researchers and security agencies. We describe terahertz time-domain spectroscopy and examine the terahertz spectra of a wide range of drugs-of-abuse, pure explosives, and plastic explosives.

Surface emitting terahertz quantum cascade laser with a double-metal waveguide

We investigate the implementation of surface emission via a second order grating in terahertz quantum cascade lasers with double-metal waveguides. Absorbing edge structures are designed to enforce anti-reflecting boundary conditions, which ensure distributed feedback in the cavity. The grating duty cycle is chosen in order to maximize slope efficiency. Fabricated devices demonstrate surface emission output powers that are comparable to those measured from edge-emitting double metal waveguide structures without gratings. The slope efficiency of surface emitting lasers is twice that of double-metal edge emitting structures. Surface emitting lasers show single mode behavior, with a beam divergence of approximately six degrees.

Terahertz imaging through self-mixing in a quantum cascade laser

We demonstrate terahertz (THz) frequency imaging using a single quantum cascade laser (QCL) device for both generation and sensing of THz radiation. Detection is achieved by utilizing the effect of self-mixing in the THz QCL, and, specifically, by monitoring perturbations to the voltage across the QCL, induced by light reflected from an external object back into the laser cavity. Self-mixing imaging offers high sensitivity, a potentially fast response, and a simple, compact optical design, and we show that it can be used to obtain high-resolution reflection images of exemplar structures.

Efficient power extraction in surface-emitting semiconductor lasers using graded photonic heterostructures

Symmetric and antisymmetric band-edge modes exist in distributed feedback surface-emitting semiconductor lasers, with the dominant difference being the radiation loss. Devices generally operate on the low-loss antisymmetric modes, although the power extraction efficiency is low. Here we develop graded photonic heterostructures, which localize the symmetric mode in the device centre and confine the antisymmetric modes close to the laser facet. This modal spatial separation is combined with absorbing boundaries to increase the antisymmetric mode loss, and force device operation on the symmetric mode, with elevated radiation efficiency. Application of this concept to terahertz quantum cascade lasers leads to record-high peak-power surface emission (>100 mW) and differential efficiencies (230 mW A(-1)), together with low-divergence, single-lobed emission patterns, and is also applicable to continuous-wave operation. Such flexible tuning of the radiation loss using graded photonic heterostructures, with only a minimal influence on threshold current, is highly desirable for optimizing second-order distributed feedback lasers.

High-performance continuous-wave operation of superlattice terahertz quantum-cascade lasers

The cw operation of chirped-superlattice quantum-cascade lasers emitting at λ∼67 μm (4.4 THz) is analyzed. Collected (min. 33% efficiency) output powers of 4 mW per facet are measured at liquid helium temperatures and a maximum operating temperature of 48 K is reached. Under pulsed excitation at duty cycles of 0.5%–1%, slightly higher (10%) peak powers are reached, and the device can be operated up to 67 K. Low threshold current densities of 165 and 185 A cm−2 are observed in pulsed and cw operation, respectively. The operation of the laser is examined using the Hakki–Paoli technique to estimate the net gain of the structure.

Demonstration of a self-mixing displacement sensor based on terahertz quantum cascade lasers

There has been growing interest in the use of terahertz (THz) quantum cascade lasers (QCLs) for sensing applications. However, the lack of compact and sensitive THz detectors has limited the potential for commercial exploitation of sensors based on these devices. We have developed a self-mixing sensing technique in which THz QCLs are used for both generation and interferometric sensing of THz radiation, eliminating the need for a separate detector. Using this technique, we have measured the displacement of a remote target, both with and without opaque (in the visible spectrum) materials in the beam path and demonstrated a stand-off distance of up to 7 m in air.

Swept-frequency feedback interferometry using terahertz frequency QCLs: a method for imaging and materials analysis

The terahertz (THz) frequency quantum cascade laser (QCL) is a compact source of high-power radiation with a narrow intrinsic linewidth. As such, THz QCLs are extremely promising sources for applications including high-resolution spectroscopy, heterodyne detection, and coherent imaging. We exploit the remarkable phase-stability of THz QCLs to create a coherent swept-frequency delayed self-homodyning method for both imaging and materials analysis, using laser feedback interferometry. Using our scheme we obtain amplitude-like and phase-like images with minimal signal processing. We determine the physical relationship between the operating parameters of the laser under feedback and the complex refractive index of the target and demonstrate that this coherent detection method enables extraction of complex refractive indices with high accuracy. This establishes an ultimately compact and easy-to-implement THz imaging and materials analysis system, in which the local oscillator, mixer, and detector are all combined into a single laser.

Surface-Immobilized Peptide Aptamers as Probe Molecules for Protein Detection

We demonstrate the use of surface-immobilized, oriented peptide aptamers for the detection of specific target proteins from complex biological solutions. These peptide aptamers are target-specific peptides expressed within a protein scaffold engineered from the human protease inhibitor stefin A. The scaffold provides stability to the inserted peptides and increases their binding affinity owing to the resulting three-dimensional constraints. A unique cysteine residue was introduced into the protein scaffold to allow orientation-specific surface immobilization of the peptide aptamer and to ensure exposure of the binding site to the target solution. Using dual-polarization interferometry, we demonstrate a strong relationship between binding affinity and aptamer orientation and determine the affinity constant KD for the interaction between an oriented peptide aptamer ST(cys+)_(pep9) and the target protein CDK2. Further, we demonstrate the high selectivity of the peptide aptamer STM_(pep9) by exposing surface-immobilized ST(cys+)_(pep9) to a complex biological solution containing small concentrations of the target protein CDK2.

Excitation-density-dependent generation of broadband terahertz radiation in an asymmetrically excited photoconductive antenna

The generation of terahertz (THz) transients in photoconductive emitters has been studied by varying the spatial extent and density of the optically excited photocarriers in asymmetrically excited, biased low-temperature-grown GaAs antenna structures. We find a pronounced dependence of the THz pulse intensity and broadband (>6.0 THz) spectral distribution on the pump excitation density and simulate this with a three-dimensional carrier dynamics model. We attribute the observed variation in THz emission to changes in the strength of the screening field.