Alessandro Tredicucci

Terahertz semiconductor-heterostructure laser

Semiconductor devices have become indispensable for generating electromagnetic radiation in everyday applications. Visible and infrared diode lasers are at the core of information technology, and at the other end of the spectrum, microwave and radio-frequency emitters enable wireless communications. But the terahertz region (1–10 THz; 1 THz = 1012 Hz) between these ranges has remained largely underdeveloped, despite the identification of various possible applications—for example, chemical detection, astronomy and medical imaging. Progress in this area has been hampered by the lack of compact, low-consumption, solid-state terahertz sources. Here we report a monolithic terahertz injection laser that is based on interminiband transitions in the conduction band of a semiconductor (GaAs/AlGaAs) heterostructure. The prototype demonstrated emits a single mode at 4.4 THz, and already shows high output powers of more than 2 mW with low threshold current densities of about a few hundred A cm-2 up to 50 K. These results are very promising for extending the present laser concept to continuous-wave and high-temperature operation, which would lead to implementation in practical photonic systems.

Science and technology roadmap for graphene, related two-dimensional crystals, and hybrid systems

We present the science and technology roadmap for graphene, related two-dimensional crystals, and hybrid systems, targeting an evolution in technology, that might lead to impacts and benefits reaching into most areas of society. This roadmap was developed within the framework of the European Graphene Flagship and outlines the main targets and research areas as best understood at the start of this ambitious project. We provide an overview of the key aspects of graphene and related materials (GRMs), ranging from fundamental research challenges to a variety of applications in a large number of sectors, highlighting the steps necessary to take GRMs from a state of raw potential to a point where they might revolutionize multiple industries. We also define an extensive list of acronyms in an effort to standardize the nomenclature in this emerging field.

Sub-cycle switch-on of ultrastrong light-matter interaction

Controlling the way light interacts with material excitations is at the heart of cavity quantum electrodynamics (QED). In the strong-coupling regime, quantum emitters in a microresonator absorb and spontaneously re-emit a photon many times before dissipation becomes effective, giving rise to mixed light–matter eigenmodes. Recent experiments in semiconductor microcavities reached a new limit of ultrastrong coupling, where photon exchange occurs on timescales comparable to the oscillation period of light. In this limit, ultrafast modulation of the coupling strength has been suggested to lead to unconventional QED phenomena. Although sophisticated light–matter coupling has been achieved in all three spatial dimensions, control in the fourth dimension, time, is little developed. Here we use a quantum-well waveguide structure to optically tune light–matter interaction from weak to ultrastrong and turn on maximum coupling within less than one cycle of light. In this regime, a class of extremely non-adiabatic phenomena becomes observable. In particular, we directly monitor how a coherent photon population converts to cavity polaritons during abrupt switching. This system forms a promising laboratory in which to study novel sub-cycle QED effects and represents an efficient room-temperature switching device operating at unprecedented speed.

New frontiers in quantum cascade lasers and applications

Recent advances and new directions in quantum cascade (QC) lasers are discussed. Invented in 1994 following many years of research on band-structure engineered semiconductors and devices grown by molecular beam epitaxy, this fundamentally new laser has rapidly advanced to a leading position among midinfrared semiconductor lasers in terms of wavelength agility as well as power and temperature performance. Because of the cascaded structure, QC lasers have a slope efficiency proportional to the number of stages. Devices with 100 stages having a record peak power of 0.6 W at room temperature are reported. QC lasers in the AlInAs-GaInAs lattice matched to InP material system can now be designed to emit in the whole midinfrared range from 4 to 20 /spl mu/m by appropriately choosing the thickness of the quantum wells in the active region. Using strained AlInAs-GaInAs, wavelengths as short as 3.4 /spl mu/m have been produced. New results on QC lasers emitting at 19 /spl mu/m, the longest ever realized in a III-V semiconductor laser, are reported. These devices use innovative plasmon waveguides to greatly enhance the mode confinement factor, thereby reducing the thickness of the epitaxial material. By use of a distributed feedback (DFB) geometry, QC lasers show single-mode emission with a 30-dB side-mode suppression ratio. Broad continuous single-mode tuning by either temperature or current has been demonstrated in these DFB QC lasers at wavelengths in two atmospheric windows (3-5 and 8-13 /spl mu/m), with continuous-wave linewidths <1 MHz when free running and /spl sim/10 KHz with suitable locking to the side of a molecular transition. These devices have been used in a number of chemical sensing and spectroscopic applications, demonstrating the capability of detecting parts per billion in volume of several trace gases. Sophisticated band-structure engineering has allowed the design and demonstration of bidirectional lasers. These devices emit different wavelengths for opposite bias polarities. The last section of the paper deals with the high-speed operation of QC lasers. Gain switching with pulse widths /spl sim/50 ps and active modelocking with a few picosecond-long pulses have been demonstrated. Finally, a new type of passive modelocking has been demonstrated in QC lasers, which relies on the giant and ultrafast optical Kerr effect of intersubband transitions.

Terahertz quantum cascade laser as local oscillator in a heterodyne receiver

Terahertz quantum cascade lasers have been investigated with respect to their performance as a local oscillator in a heterodyne receiver. The beam profile has been measured and transformed in to a close to Gaussian profile resulting in a good matching between the field patterns of the quantum cascade laser and the antenna of a superconducting hot electron bolometric mixer. Noise temperature measurements with the hot electron bolometer and a 2.5 THz quantum cascade laser yielded the same result as with a gas laser as local oscillator.

High-resolution gas phase spectroscopy with a distributed feedback terahertz quantum cascade laser

The quantum cascade laser is a powerful, narrow linewidth, and continuous wave source of terahertz radiation. The authors have implemented a distributed feedback device in a spectrometer for high-resolution gas phase spectroscopy. Amplitude as well as frequency modulation schemes have been realized. The absolute frequency was determined by mixing the radiation from the quantum cascade laser with that from a gas laser. The pressure broadening and the pressure shift of a rotational transition of methanol at 2.519THz were measured in order to demonstrate the performance of the spectrometer.The quantum cascade laser is a powerful, narrow linewidth, and continuous wave source of terahertz radiation. The authors have implemented a distributed feedback device in a spectrometer for high-resolution gas phase spectroscopy. Amplitude as well as frequency modulation schemes have been realized. The absolute frequency was determined by mixing the radiation from the quantum cascade laser with that from a gas laser. The pressure broadening and the pressure shift of a rotational transition of methanol at 2.519THz were measured in order to demonstrate the performance of the spectrometer.

Controlled photon emission in porous silicon microcavities

We demonstrate the preparation of narrow‐band porous‐silicon reflectors integrated on porous‐silicon layers by electrochemical etching. By carefully tuning the resulting photon cavity mode around the maximum of the porous silicon photoluminescence, we have obtained both a narrowing and enhancement of the emission line, and a highly concentrated radiation pattern. These results show that the porous silicon spontaneous emission is modified because of the coupling with the photon cavity mode.

Design and simulation of terahertz quantum cascade lasers

Strategies and concepts for the design of THz emitters based on the quantum cascade scheme are analyzed and modeled in terms of a fully three-dimensional Monte Carlo approach; this allows for a proper inclusion of both carrier–carrier and carrier–phonon scattering mechanisms. Starting from the simulation of previously published far-infrared emitters, where no population inversion is achieved, two designs are proposed. The first one follows the well-established chirped-superlattice scheme whereas the second one employs a double-quantum well superlattice to allow energy relaxation through optical phonon emission. For both cases a significant population inversion is predicted at temperatures up to 80 K.

Signatures of the ultrastrong light-matter coupling regime

Aji A. Anappara, Simone De Liberato, 3 Alessandro Tredicucci, ∗ Cristiano Ciuti, Giorgio Biasiol, Lucia Sorba, and Fabio Beltram NEST CNR-INFM and Scuola Normale Superiore, Piazza dei Cavalieri 7, I-56126 Pisa (Italy) Laboratoire Matériaux et Phénomènes Quantiques, Université Paris Diderot Paris 7 and CNRS, UMR 7162, Bâtiment Condorcet, 75013 Paris (France) Laboratoire Pierre Aigrain, Ecole Normale Supérieure and CNRS, UMR 8551, 75005 Paris (France) Laboratorio Nazionale TASC CNR-INFM, Area Science Park, SS 14 Km 163.5, Basovizza, I-34012 Trieste (Italy) (Dated: March 10, 2009)

High-performance operation of single-mode terahertz quantum cascade lasers with metallic gratings

A periodic array of thin slits opened on a metallic surface can act as a one-dimensional photonic crystal for the propagation of surface-plasmon waves. We have used such structure for the implementation of distributed feedback resonators in quantum cascade lasers emitting near 2.5THz. Single-mode emission, stable at all injection currents and operating temperatures, was achieved both in pulsed and continuous wave. The devices exhibited output powers of several milliwatts with low threshold current densities of ∼100A∕cm2.A periodic array of thin slits opened on a metallic surface can act as a one-dimensional photonic crystal for the propagation of surface-plasmon waves. We have used such structure for the implementation of distributed feedback resonators in quantum cascade lasers emitting near 2.5THz. Single-mode emission, stable at all injection currents and operating temperatures, was achieved both in pulsed and continuous wave. The devices exhibited output powers of several milliwatts with low threshold current densities of ∼100A∕cm2.