James Keeley

Terahertz imaging using quantum cascade lasers—a review of systems and applications

The terahertz (THz) frequency quantum cascade laser (QCL) is a compact source of THz radiation offering high power, high spectral purity and moderate tunability. As such, these sources are particularly suited to the application of THz frequency imaging across a range of disciplines, and have motivated significant research interest in this area over the past decade. In this paper we review the technological approaches to THz QCL-based imaging and the key advancements within this field. We discuss in detail a number of imaging approaches targeted to application areas including multiple-frequency transmission and diffuse reflection imaging for the spectral mapping of targets; as well as coherent approaches based on the self-mixing phenomenon in THz QCLs for long-range imaging, three-dimensional imaging, materials analysis, and high-resolution inverse synthetic aperture radar imaging.

Coherent three-dimensional terahertz imaging through self-mixing in a quantum cascade laser

We demonstrate coherent terahertz (THz) frequency imaging using the self-mixing effect in a quantum cascade laser (QCL). Self-mixing voltage waveforms are acquired at each pixel of a two-dimensional image of etched GaAs structures and fitted to a three-mirror laser model, enabling extraction of the amplitude and phase parameters of the reflected field. From the phase, we reconstruct the depth of the sample surface, and we show that the amplitude can be related to the sample reflectance. Our approach is experimentally simple and compact, and does not require frequency stabilization of the THz QCL.

Apertureless near-field terahertz imaging using the self-mixing effect in a quantum cascade laser

We report two-dimensional apertureless near-field terahertz (THz) imaging using a quantum cascade laser(QCL)source and a scattering probe. A near-field enhancement of the scattered field amplitude is observed for small tip-sample separations, allowing image resolutions of ∼1 μm (∼λ/100) and ∼7 μm to be achieved along orthogonal directions on the sample surface. This represents the highest resolution demonstrated to date with a THz QCL. By employing a detection scheme based on self-mixing interferometry, our approach offers experimental simplicity by removing the need for an external detector and also provides sensitivity to the phase of the reinjected field.

Laser Feedback Interferometry as a Tool for Analysis of Granular Materials at Terahertz Frequencies: Towards Imaging and Identification of Plastic Explosives.

We propose a self-consistent method for the analysis of granular materials at terahertz (THz) frequencies using a quantum cascade laser. The method is designed for signals acquired from a laser feedback interferometer, and applied to non-contact reflection-mode sensing. Our technique is demonstrated using three plastic explosives, achieving good agreement with reference measurements obtained by THz time-domain spectroscopy in transmission geometry. The technique described in this study is readily scalable: replacing a single laser with a small laser array, with individual lasers operating at different frequencies will enable unambiguous identification of select materials. This paves the way towards non-contact, reflection-mode analysis and identification of granular materials at THz frequencies using quantum cascade lasers.

Origin of terminal voltage variations due to self-mixing in terahertz frequency quantum cascade lasers.

We explain the origin of voltage variations due to self-mixing in a terahertz (THz) frequency quantum cascade laser (QCL) using an extended density matrix (DM) approach. Our DM model allows calculation of both the current-voltage (I-V) and optical power characteristics of the QCL under optical feedback by changing the cavity loss, to which the gain of the active region is clamped. The variation of intra-cavity field strength necessary to achieve gain clamping, and the corresponding change in bias required to maintain a constant current density through the heterostructure is then calculated. Strong enhancement of the self-mixing voltage signal due to non-linearity of the (I-V) characteristics is predicted and confirmed experimentally in an exemplar 2.6 THz bound-to-continuum QCL.

Active phase-nulling of the self-mixing phase in a terahertz frequency quantum cascade laser

We demonstrate an active phase-nulling scheme for terahertz (THz) frequency quantum cascade lasers (QCLs) under optical feedback, by active electronic feedback control of the emission frequency. Using this scheme, the frequency tuning rate of a THz QCL is characterized, with significantly reduced experimental complexity compared to alternative approaches. Furthermore, we demonstrate real-time displacement sensing of targets, overcoming the resolution limits imposed by quantization in previously implemented fringe-counting methods. Our approach is readily applicable to high-frequency vibrometry and surface profiling of targets, as well as frequency-stabilization schemes for THz QCLs.

Measurement of the emission spectrum of a semiconductor laser using laser-feedback interferometry

The effects of optical feedback (OF) in lasers have been observed since the early days of laser development. While OF can result in undesirable and unpredictable operation in laser systems, it can also cause measurable perturbations to the operating parameters, which can be harnessed for metrological purposes. In this work we exploit this ‘self-mixing’ effect to infer the emission spectrum of a semiconductor laser using a laser-feedback interferometer, in which the terminal voltage of the laser is used to coherently sample the reinjected field. We demonstrate this approach using a terahertz frequency quantum cascade laser operating in both single- and multiple-longitudinal mode regimes, and are able to resolve spectral features not reliably resolved using traditional Fourier transform spectroscopy. We also investigate quantitatively the frequency perturbation of individual laser modes under OF, and find excellent agreement with predictions of the excess phase equation central to the theory of lasers under OF.

Optical feedback effects on terahertz quantum cascade lasers: modelling and applications

Terahertz (THz) quantum cascade lasers (QCLs) are compact sources of radiation in the 1–5 THz range with significant potential for applications in sensing and imaging. Laser feedback interferometry (LFI) with THz QCLs is a technique utilizing the sensitivity of the QCL to the radiation reflected back into the laser cavity from an external target. We will discuss modelling techniques and explore the applications of LFI in biological tissue imaging and will show that the confocal nature of the QCL in LFI systems, with their innate capacity for depth sectioning, makes them suitable for skin diagnostics with the well-known advantages of more conventional confocal microscopes. A demonstration of discrimination of neoplasia from healthy tissue using a THz, LFI-based system in the context of melanoma is presented using a transgenic mouse model.

Self-mixing effect in THz quantum cascade lasers: Applications in sensing and imaging

The paper introduces self-mixing interferometry in semiconductor lasers in general, and then discusses recent advancements in the coherent THz imaging and sensing systems based on the self-mixing effect in terahertz quantum cascade lasers. Two different imaging modalities are used to illustrate the coherent nature of this sensing technique and its applications to three-dimensional surface profiling and material identification.