R. Ivanov

Two-colour pump–probe experiments with a twin-pulse-seed extreme ultraviolet free-electron laser

Exploring the dynamics of matter driven to extreme non-equilibrium states by an intense ultrashort X-ray pulse is becoming reality, thanks to the advent of free-electron laser technology that allows development of different schemes for probing the response at variable time delay with a second pulse. Here we report the generation of two-colour extreme ultraviolet pulses of controlled wavelengths, intensity and timing by seeding of high-gain harmonic generation free-electron laser with multiple independent laser pulses. The potential of this new scheme is demonstrated by the time evolution of a titanium-grating diffraction pattern, tuning the two coherent pulses to the titanium M-resonance and varying their intensities. This reveals that an intense pulse induces abrupt pattern changes on a time scale shorter than hydrodynamic expansion and ablation. This result exemplifies the essential capabilities of the jitter-free multiple-colour free-electron laser pulse sequences to study evolving states of matter with element sensitivity.

Determining the polarization state of an extreme ultraviolet free-electron laser beam using atomic circular dichroism

Ultrafast extreme ultraviolet and X-ray free-electron lasers are set to revolutionize many domains such as bio-photonics and materials science, in a manner similar to optical lasers over the past two decades. Although their number will grow steadily over the coming decade, their complete characterization remains an elusive goal. This represents a significant barrier to their wider adoption and hence to the full realization of their potential in modern photon sciences. Although a great deal of progress has been made on temporal characterization and wavefront measurements at ultrahigh extreme ultraviolet and X-ray intensities, only few, if any progress on accurately measuring other key parameters such as the state of polarization has emerged. Here we show that by combining ultra-short extreme ultraviolet free electron laser pulses from FERMI with near-infrared laser pulses, we can accurately measure the polarization state of a free electron laser beam in an elegant, non-invasive and straightforward manner using circular dichroism.

CITIUS: an infrared-extreme ultraviolet light source for fundamental and applied ultrafast science.

We present the main features of CITIUS, a new light source for ultrafast science, generating tunable, intense, femtosecond pulses in the spectral range from infrared to extreme ultraviolet (XUV). The XUV pulses (about 10(5)-10(8) photons/pulse in the range 14-80 eV) are produced by laser-induced high-order harmonic generation in gas. This radiation is monochromatized by a time-preserving monochromator, also allowing one to work with high-resolution bandwidth selection. The tunable IR-UV pulses (10(12)-10(15) photons/pulse in the range 0.4-5.6 eV) are generated by an optical parametric amplifier, which is driven by a fraction of the same laser pulse that generates high order harmonics. The IR-UV and XUV pulses follow different optical paths and are eventually recombined on the sample for pump-probe experiments. We also present the results of two pump-probe experiments: with the first one, we fully characterized the temporal duration of harmonic pulses in the time-preserving configuration; with the second one, we demonstrated the possibility of using CITIUS for selective investigation of the ultra-fast dynamics of different elements in a magnetic compound.

Ultrafast laser synchronization at the FERMI@Elettra FEL

Modern VUV and X-ray Free Electron Laser (FEL) facilities contain a number of ultrafast lasers (like photoinjector, seed and pump-probe lasers) whose performance is crucial for the generated FEL light quality as well as for the accuracy of the time resolved measurements performed using the FEL pulses. One of the very important laser related aspects, especially at seeded FELs, is the ability to precisely lock the ultrafast laser systems to the master clock signal, keeping the timing jitter and drifts of the generated pulses with respect to the machine timing as low as possible. The aim of this work is to review the main sources of timing jitter and drifts and present the schemes and solutions developed at FERMI for their characterization and compensation. The paper will first introduce a general scheme showing the architecture of the laser locking system developed for FERMI. Both the radio-frequency (RF) locking and the advanced balanced optical cross correlator electronics and optical setup design are described, together with data on the laser oscillator locking performance obtained in different modalities. Cross correlation measurements indicating the contribution of the ultrafast regenerative amplifier and optical beam transport part to the overall temporal jitter of the amplified ultrashort pulses arriving at destination are presented. The paper also includes examples of the influence of improved laser timing jitter and drifts on the seeded FEL performance and discusses foreseen future developments.

FERMI@Elettra, a seeded free electron laser source for a broad scientific user program

After less than two years of commissioning the FERMI@Elettra free electron laser is now entering into the operation phase and is providing light to the first user experiments. To reach the final ambitious goals of providing high power coherent pulses with fundamental wavelengths down to 4 nm, the system will need further studies and additional commissioning time in 2011 when fine tuning of the major systems such as the electron gun and the main accelerator will take place. Nevertheless, FERMI is already able to provide light with unique characteristics allowing Users to perform experiments not possible with other facilities. Based on a 1.5 GeV electron linear accelerator, FERMI@Elettra has two seeded FEL lines that cover the whole spectral range from 100 nm down to 4 nm with fully coherent pulses. The use of the high gain harmonic generation scheme initiated by a tunable laser in the UV allows FERMI to produce light characterized by both transverse and full temporal coherence. The use of specially designed undulators allows full control of the FEL polarization and can be continuously varied from linear to circular in any orientation or ellipticity. Here we will report about the first results and the future plans for FERMI@Elettra.

Optically induced Fe magnetization reversal in Fe/MnAs/GaAs(001)

Magnetization control without applying magnetic fields has potential for applications in sensors and devices. In Fe/MnAs/GaAs(001), the Fe magnetization can be modified by acting on the MnAs microstructure via temperature control, without applying external magnetic fields. Here we use an optical laser pulse to vary the local temperature and an x-ray free-electron laser pulse to probe the induced magnetic and structural dynamics in a time-resolved resonant scattering experiment, both pulses having ~100 fs duration. Modifications of the MnAs microstructure take place within a few ps, followed by a slower dynamics driven by thermal diffusion. We show that a single optical laser pulse can reverse the Fe magnetization locally, the process being driven not by the fast modifications of the MnAs structure, but rather by its slower return to equilibrium.

Monochromatic extreme-ultraviolet ultrafast beamline

Summary form only given. CITIUS is a multi-partner and multi-disciplinary project lead by University of Nova Gorica (Slovenia) to develop a facility based on a high repetition rate and ultra-short tunable laser source that is used to produce ultrafast extreme-ultraviolet (XUV) pulses through high-order harmonic (HH) generation. The XUV radiation is monochromatized and can be focused on different end-stations for materials and surface science and atomic and molecular physics and chemistry. We present here the characterization of the monochromatic XUV source. The HHs are generated in a gas cell using a Ti:Sa laser operated at 5-Khz repetition rate with an energy of 2 mJ/pulse. The XUV beam is monochromatized and focused in the experimental chamber. Since the beam is handled by a grating monochromator, a temporal broadening has to be accepted at the output due to the pulse front-tilt given by the diffraction [2]. In the case of the CITIUS beamline, an innovative single-grating configuration has been adopted, that combines in a single instrument two different grating geometries: the classical-diffraction mount (CDM) and the off-plane mount (OPM), as shown in Fig. 1. It has been demonstrated that the two geometries are complementary [3]: the CDM is used for relatively long instrumental response in the 100-200 fs range, and high spectral resolution, i.e. λ/Δλ > 200; the OPM is used for ultrashort responses in the 10-50 fs range and low spectral resolution, i.e. λ/Δλ <; 200 [4].