Rafael Salas-Montiel

Efficient Directional Coupling between Silicon and Copper Plasmonic Nanoslot Waveguides: toward Metal−Oxide−Silicon Nanophotonics

Coupling plasmonics and silicon photonics is the best way to bridge the size gap between macroscopic optics and nanodevices in general and especially nanoelectronic devices. We report on the realization of key blocks for future plasmonic planar integrated optics, nano-optical couplers, and nanoslot waveguides that are compatible both with the silicon photonics and the CMOS microelectronics. Copper-based devices provide for very efficient optical coupling, unexpectedly low propagation losses and a broadband sub-50 nm optical confinement. The fabrication in a standard frontline microelectronic facilities hints broad possibilities of hybrid opto-electronic very large scale integration.

On-chip hybrid photonic-plasmonic light concentrator for nanofocusing in an integrated silicon photonics platform.

The enhancement and confinement of electromagnetic radiation to nanometer scale have improved the performances and decreased the dimensions of optical sources and detectors for several applications including spectroscopy, medical applications, and quantum information. Realization of on-chip nanofocusing devices compatible with silicon photonics platform adds a key functionality and provides opportunities for sensing, trapping, on-chip signal processing, and communications. Here, we discuss the design, fabrication, and experimental demonstration of light nanofocusing in a hybrid plasmonic-photonic nanotaper structure. We discuss the physical mechanisms behind the operation of this device, the coupling mechanisms, and how to engineer the energy transfer from a propagating guided mode to a trapped plasmonic mode at the apex of the plasmonic nanotaper with minimal radiation loss. Optical near-field measurements and Fourier modal analysis carried out using a near-field scanning optical microscope (NSOM) show a tight nanofocusing of light in this structure to an extremely small spot of 0.00563(λ/(2n(rmax)))(3) confined in 3D and an exquisite power input conversion of 92%. Our experiments also verify the mode selectivity of the device (low transmission of a TM-like input mode and high transmission of a TE-like input mode). A large field concentration factor (FCF) of about 4.9 is estimated from our NSOM measurement with a radius of curvature of about 20 nm at the apex of the nanotaper. The agreement between our theory and experimental results reveals helpful insights about the operation mechanism of the device, the interplay of the modes, and the gradual power transfer to the nanotaper apex.

Observation of Near-Field Dipolar Interactions Involved in a Metal Nanoparticle Chain Waveguide

We present near-field measurements of transverse plasmonic wave propagation in a chain of gold elliptical nanocylinders fed by a silicon refractive waveguide at optical telecommunication wavelengths. Eigenmode amplitude and phase imaging by apertureless scanning near-field optical microscopy allows us to measure the local out-of-plane electric field components and to reveal the exact nature of the excited localized surface plasmon resonances. Furthermore, the coupling mechanism between subsequent metal nanoparticles along the chain is experimentally analyzed by spatial Fourier transformation on the complex near-field cartography, giving a direct experimental proof of plasmonic Bloch mode propagation along array of localized surface plasmons. Our work demonstrates the possibility to characterize multielement plasmonic nanostructures coupled to a photonic waveguide with a spatial resolution of less than 30 nm. This experimental work constitutes a prerequisite for the development of integrated nanophotonic devices.

Quantitative analysis and near-field observation of strong coupling between plasmonic nanogap and silicon waveguides

We present a near field optical study of a plasmonic gap waveguide vertically integrated on silicon. The experimental study is based on a near field scanning optical microscope configured in perturbation mode. This operation mode is described and modeled to give a physical insight into the measured signal. A high spatial resolution allows for the characteristics of the plasmonic gap modes, such as near field distributions, effective indices, direction of propagation, and coupling between perpendicularly polarized modes, to be imaged and analyzed with accuracy. This experimental work is supported by numerical simulations based on finite element optical mode solvers and by the application of the strongly coupled-mode theory to the device.

Waveguide-coupled nanowire as an optical antenna

We study the optical coupling between a gold nanowire and a silver ion-exchanged waveguide, with special emphasis on the nanowire antenna radiation pattern. We measure the radiation patterns of waveguide-coupled gold nanowires with a height of 70 nm and width of 50 or 150 nm in the 450-700 nm spectral range for TE and TM polarizations. We perform a systematic theoretical study on the wavelength, polarization, nanowire size, and material dependences on the properties of the radiation pattern. We also give some elements concerning absorption and near-field. Experiments and calculations show localized plasmon resonance for the polarization orthogonal to the wire (far-field resonance at 580 nm for the smallest wire and 670 nm for the widest). It is shown that a great variety of radiation patterns can be obtained, together with a high sensitivity to a change of one parameter, particularly near-resonance.

Theoretical analysis of Bloch mode propagation in an integrated chain of gold nanowires

The eigenmodes analysis of Bloch modes in a chain of metallic nanowires (MNWs) provides a significant physical understanding about the light propagation phenomena involved in such structures. However, most of these analyses have been done above the light line in the dispersion relation, where the Bloch modes can only be excited with radiative modes. By making use of the Fourier modal method, in this paper we rigorously calculate the eigenmode and mode excitation of a chain of MNWs via the fundamental transverse magnetic (TM) mode of a dielectric waveguide. Quadrupolar and dipolar transversal Bloch modes were obtained in an MNW chain embedded in a dielectric material. These modes can be coupled efficiently with the fundamental TM mode of the waveguide. Since the eigenmodes supported by the integrated plasmonic structure exhibit strong localized surface plasmon (LSP) resonances, they could serve as a nanodevice for sensing applications. Also, the analysis opens a direction for novel nanostructures, potentially helpful for the efficient excitation of LSPs and strong field enhancement.

Topology assisted self-organization of colloidal nanoparticles: application to 2D large-scale nanomastering

Summary Our aim was to elaborate a novel method for fully controllable large-scale nanopatterning. We investigated the influence of the surface topology, i.e., a pre-pattern of hydrogen silsesquioxane (HSQ) posts, on the self-organization of polystyrene beads (PS) dispersed over a large surface. Depending on the post size and spacing, long-range ordering of self-organized polystyrene beads is observed wherein guide posts were used leading to single crystal structure. Topology assisted self-organization has proved to be one of the solutions to obtain large-scale ordering. Besides post size and spacing, the colloidal concentration and the nature of solvent were found to have a significant effect on the self-organization of the PS beads. Scanning electron microscope and associated Fourier transform analysis were used to characterize the morphology of the ordered surfaces. Finally, the production of silicon molds is demonstrated by using the beads as a template for dry etching.

Optimal length of ZnO nanorods for improving the light-extraction efficiency of blue InGaN light-emitting diodes.

Optimal length of ZnO nanorods (NRs) on blue InGaN light-emitting diodes (LEDs) was investigated to improve the light-extraction efficiency (LEE) of the LED. X-ray diffraction, photoluminescence spectroscopy, and micro-Raman spectroscopy were employed to determine the structural and optical properties of the ZnO NRs with length of 300 nm and 5 μm grown by a hydrothermal method. From the conventional light output power versus injection current (L-I) measurement, we found that the light output power of the LEDs with 300-nm- and 5-μm-long ZnO NRs was approximately 14.6% and 40.7% greater, respectively, than that of the LED without the ZnO NRs at an operating current of 20 mA. In addition, there were almost no changes to the electrical properties of the ZnO-NR-coated LEDs. The effect of the length of the ZnO NRs on the LEE of the LEDs was theoretically verified with three-dimensional finite-difference time-domain (FDTD) analysis. The FDTD images of the optical power and far-field radiation patterns of the LEDs showed that more photons were guided to the out of the LED by the longer ZnO NRs than by the shorter ZnO NRs grown on the LEDs.

Local density of electromagnetic states in plasmonic nanotapers: spatial resolution limits with nitrogen-vacancy centers in diamond nanospheres

One of the most explored single quantum emitters for the development of nanoscale fluorescence lifetime imaging is the nitrogen-vacancy (NV) color center in diamond. An NV center does not experience fluorescence bleaching or blinking at room temperature. Furthermore, its optical properties are preserved when embedded into nanodiamond hosts. This paper focuses on the modeling of the local density of states (LDOS) in a plasmonic nanofocusing structure with an NV center acting as local illumination sources. Numerical calculations of the LDOS near such a nanostructure were done with a classical electric dipole radiation placed inside a diamond sphere as well as near-field optical fluorescence lifetime imaging of the structure. We found that Purcell factors higher than ten can be reached with diamond nanospheres of radius less than 5 nm and at a distance of less than 20 nm from the surface of the structure. Although the spatial resolution of the experiment is limited by the size of the nanodiamond, our work supports the analysis and interpretation of a single NV color center in a nanodiamond as a probe for scanning near-field optical microscopy.

Light confinement and propagation characteristics in plasmonic gap waveguides on silicon

Plasmonic waveguiding structures have the ability to confine and propagate light over short distances, typically less than a hundred micrometers. This short propagation length is the price that is paid for confining light to dimensions on the order of a hundred of nanometers. With these scales in mind, several plasmonic devices can be proposed (e.g. wavelength multiplexors) and some of them have been already demonstrated such as Y junctions and directional couplers. Although the dimensions involved in such structures are below the diffraction limit, large-scale optical characterization techniques, such as transmitted power, are still employed. In this contribution, we present a characterization technique for the study of the guided modes in plasmonic gap waveguiding structures that resolves subwavelength-scale features, as it is based on atomic force microscope and on near field scattering optical microscope in guided detection.