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Dive into the research topics where Shu-Liang Zang is active.

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Featured researches published by Shu-Liang Zang.


Green Chemistry | 2015

Olefin epoxidation with hydrogen peroxide using octamolybdate-based self-separating catalysts

Ming-Dong Zhou; Mei-Ju Liu; Liangliang Huang; Jian Zhang; Jingyun Wang; Xuebing Li; Fritz E. Kühn; Shu-Liang Zang

Mo8O264− based organic polyoxomolybdate salts of general formula [Hmim]4Mo8O26 (Hmim = 1-hexyl-3-methylimidazolium), [Dhmim]4Mo8O26 (Dhmim = 1,2-dimethyl-3-hexylimidazolium) and [Hpy]4Mo8O26·H2O (Hpy = 1-hexylpyridinium) have been prepared and characterized. These compounds were applied as catalysts for olefin epoxidation using hydrogen peroxide (H2O2) as oxidant in CH3CN. The polyoxomolybdate salts exhibit excellent catalytic performance and are also self-separating, a great advantage for catalyst recycling. The catalysts can be reused for at least 10 runs without significant loss of activity.


Chemistry-an Asian Journal | 2009

(N-Salicylidene)aniline Derived Schiff Base Complexes of Methyltrioxorhenium(VII): Ligand Influence and Catalytic Performance

Ming-Dong Zhou; Yang Yu; Alejandro Capapé; Kavita R. Jain; Eberhardt Herdtweck; Xiao‐Rong Li; Jun Li; Shu-Liang Zang; Fritz E. Kühn

Methyltrioxorhenium(VII) (MTO) readily forms 1:1 adducts with several N-(salicylidene)aniline derived Schiff bases. If the aromatic rings of the N-(salicylidene)aniline ligands display non-donating or electron withdrawing substituent groups, the resulting MTO adducts show good activities in olefin epoxidations. However, steric effects seem to play a major role, leading often to instable o- and m-Schiff base-MTO adducts, while p-substituted Schiff bases usually lead to more stable adducts. In catalysis, electron-withdrawing substituents on the aniline moiety lead to better catalysts than electron donating ones. The gap between good catalysts and instable or non-existing compounds, however, is small. The general tendency, however, that good donors on the Schiff base ligands lead to shorter Re-O(Schiff base) bridges and lower catalytic activity, while the opposite is true with acceptor ligands on the Schiff bases, seems to be quite clear.


Zeitschrift für Naturforschung B | 2013

Oxidation Reactions Catalyzed by Polyoxomolybdate Salts

Bo Zhang; Su Li; Alexander Pöthig; Mirza Cokoja; Shu-Liang Zang; Wolfgang A. Herrmann; Fritz E. Kühn

Ionic compounds containing the polyoxomolybdate anion [Mo6O19]2- and [(n-C4H9)4P]+ (tetrabutylphosphonium), [(n-C4H9)3P(n-C14H29)]+ (tributyl (tetradecyl)phosphonium), [Bmim]+ (1- butyl-3-methylimidazolium) and [Dbmim]+ (1,2-dimethyl-3-butylimidazolium) cations were prepared and characterized, including the determination of three of the solid state structures by singlecrystal X-ray diffraction. These compounds were applied as catalysts for the epoxidation of olefins with urea hydrogen peroxide (UHP) as oxidant in the ionic liquid [Bmim]PF6. Additionally, the oxidation of sulfides to sulfoxides with hydrogen peroxide (H2O2) in several solvents was investigated. The polyoxomolybdate catalysts showed a good performance for epoxidation of olefins as well as for oxidation of sulfides. Furthermore, the catalysts can be recycled several times in oxidation reactions. We present this methodology for the oxidation reaction in a simple, economically, technically, and environmentally benign manner Graphical Abstract Oxidation Reactions Catalyzed by Polyoxomolybdate Salts


Zeitschrift für Naturforschung B | 2013

Synthesis and Characterization of Imidazolium Perrhenate Ionic Liquids

Shuang Yue; Da-Wei Fang; Jun Li; Shu-Liang Zang; Ming-Dong Zhou; Bo Zhang; Iulius I. E. Markovits; Mirza Cokoja; Fritz E. Kühn

A series of air- and water-stable imidazolium perrhenate-based room-temperature ionic liquids [(RT)ILs] of the type [Cnmim][ReO4] (Cnmim = 1-CnH2n+1-3-methylimidazolium, n = 2, 4, 5, 6, 8, 10, 12) have been synthesized and characterized by 1H and 13C NMR spectroscopy, IR spectroscopy, electrospray ionization mass spectrometry (ESI-MS), and elemental analysis (EA). The effect of the variation of the alkyl chain length on physical properties such as melting point, thermal stability, density, and conductivity was examined Graphical Abstract Synthesis and Characterization of Imidazolium Perrhenate Ionic Liquids


Inorganic Chemistry | 2002

Synthesis and Catalytic Application of Octahedral Lewis Base Adducts of Dichloro and Dialkyl Dioxotungsten(VI)

Fritz E. Kühn; Wen-Mei Xue; Ahmad M. Al-Ajlouni; Ana M. Santos; Shu-Liang Zang; Carlos C. Romão; Georg Eickerling; Eberhardt Herdtweck


Journal of Organometallic Chemistry | 2013

Imidazolium perrhenate ionic liquids as efficient catalysts for the selective oxidation of sulfides to sulfones

Bo Zhang; Su Li; Shuang Yue; Mirza Cokoja; Ming-Dong Zhou; Shu-Liang Zang; Fritz E. Kühn


Journal of Organometallic Chemistry | 2008

((2-Hydroxynapthalen-1-yl)methylene)aniline derived Schiff base adducts of MTO: Synthesis and catalytic application

Alejandro Capapé; Ming-Dong Zhou; Shu-Liang Zang; Fritz E. Kühn


Journal of Organometallic Chemistry | 2008

A (salicylidene)aniline derived Schiff-base adduct of methyltrioxorhenium(VII)–Cis-and trans-coordination of the ligand

Ming-Dong Zhou; Shu-Liang Zang; Eberhardt Herdtweck; Fritz E. Kühn


Journal of Solid State Chemistry | 2013

Synthesis, structure and characterization of two new open-framework gallium phosphite-oxalates of varying dimensionality

Caixia Li; Liangliang Huang; Ming-Dong Zhou; Jing Xia; Hongwei Ma; Shu-Liang Zang; Li Wang


Catalysis Communications | 2017

C-S cross-coupling of aryl halides with alkyl thiols catalyzed by in-situ generated nickel(II) N-heterocyclic carbene complexes

Fang-Jie Guo; Jing Sun; Zhaoqing Xu; Fritz E. Kühn; Shu-Liang Zang; Ming-Dong Zhou

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Bo Zhang

Dalian Institute of Chemical Physics

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Jun Li

Liaoning University

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Xuebing Li

Chinese Academy of Sciences

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